Turbulent Flow Mixing for Organolithium Polymerization

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Existing methods for polymerizing conjugated diene or aromatic vinyl monomers with organolithium compounds suffer from insufficient uniformity in mixing, leading to gel generation in the polymerization tank and incorporation of gels into the polymer product.

Innovation Solution

A method involving the mixing of an organolithium compound solution with a non-polar solvent in a pipe-system to create a turbulent flow, characterized by a Reynolds number of 500,000 or more, which suppresses gel generation and incorporation into the polymer product.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of operation

If organolithium compound solution and non-polar solvent are mixed in a storage tank with stirring blade, then mixing operation is simple, but concentration uniformity is poor causing gel generation

Engineering Contradiction:
Improvemixing operation simplicityVSAvoidconcentration uniformity
Core Design Contradiction:
Ease of operationVSStability of the object's composition

Solution Approach 1:

The patent replaces the mechanical stirring blade system with a fluid dynamic system using turbulent flow. By designing the mixing pipe with specific geometry (narrow section) to generate high Reynolds number turbulent flow (Re≥500,000), the mixing process transitions from mechanical agitation to chaotic fluid mixing, achieving superior concentration uniformity without mechanical moving parts in the mixing zone.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The invention utilizes hydraulic principles by employing turbulent flow of liquids (organolithium compound solution and non-polar solvent) through a specifically designed mixing pipe. The hydraulic design creates intense mixing through turbulent eddies and chaotic flow patterns, eliminating the need for mechanical stirrers and preventing concentration stratification that leads to gel formation.

Inventive Principle:
Principle #29Pneumatics and hydraulics

2Stability of the object's composition

If mixing is performed in a pipe-system with turbulent flow, then concentration uniformity is improved suppressing gel generation, but device complexity increases

Engineering Contradiction:
Improveconcentration uniformityVSAvoidmixing system complexity
Core Design Contradiction:
Stability of the object's compositionVSDevice complexity

Solution Approach 1:

The patent extracts the mixing function from a complex mechanical stirring system and implements it within the existing fluid transport pipeline. By incorporating a narrow section directly into the mixing pipe, the system achieves turbulent flow mixing without adding separate mixing devices, motors, or mechanical components, thus minimizing device complexity while maximizing mixing effectiveness.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention merges the mixing function with the fluid transport function by designing the mixing pipe as an integrated component. The narrow section is incorporated directly into the pipeline, combining transportation and mixing operations in a single element, thereby avoiding additional equipment and reducing overall system complexity.

Inventive Principle:
Principle #5Merging (Combining)

3Productivity

If high concentration organolithium compound is used, then productivity is improved, but gel generation occurs due to concentration distribution

Engineering Contradiction:
Improvepolymerization productivityVSAvoidgel generation
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

The patent changes the flow regime parameter (Reynolds number) to extremely high values (Re≥500,000) by incorporating a narrow section in the mixing pipe. This parameter change transforms the mixing mechanism from laminar to turbulent flow, enabling rapid and uniform dispersion of high concentration organolithium compound with non-polar solvent, thereby maintaining high productivity while eliminating concentration distribution that causes gel formation.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method effectively prevents gel generation in the polymerization tank and reduces gel incorporation into the polymer product, ensuring more stable and uniform polymer production.

Implementation Method 1

at least one selected from the group consisting of the organolithium compound solution I, the organolithium compound solution II and the non-polar solvent is in the state of turbulent flow in step (1), said turbulent flow being characterized by a Reynolds number (Re) of 500000 or more

Methodology Applied
Scientific EffectTurbulent flow: Turbulence

Data Source

PatentEP3023440B1Polymer manufacturing method
Publication Date: 2020.09.09 ASAHI KASEI KOGYO KABUSHIKI KAISHA
  • EP3023440B1 patent drawingFigure 1
  • EP3023440B1 patent drawingFigure 2
  • EP3023440B1 patent drawingFigure 3

AI summary

The method for producing a polymer of the present invention is a method for producing a polymer by polymerization of a monomer comprising a conjugated diene compound and/or an aromatic vinyl compound by use of an organolithium compound as a polymerization initiator, comprising step (1) of mixing an organolithium compound solution I and a non-polar solvent to provide an organolithium compound solution II and step (2) of feeding the organolithium compound solution II to a polymerization tank, wherein at least one selected from the group consisting of the organolithium compound solution I, the organolithium compound solution II and the non-polar solvent is in the state of turbulent flow in step (1).