Co-rotating Twin-Screw Extruder for Reactive Polyamide Synthesis

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Current polyamide production processes are lengthy, require multiple steps, and involve complex transfers, making them inefficient and difficult to scale industrially, as they often necessitate the preparation of pre-polymers and salts, and subsequent heat treatment steps.

Innovation Solution

A process where diamine and dicarboxylic acid monomers are directly introduced into a co-rotating twin-screw extruder for polycondensation, eliminating the need for prior salt formation and additional heat treatment, with continuous operation in a single extruder to achieve high molar mass polyamides.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If conventional polycondensation process with multiple steps is used, then polyamide can be produced, but production time is long and process complexity increases

Engineering Contradiction:
Improveproduction timeVSAvoidprocess complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent combines salt formation, polycondensation, and post-condensation steps into a single continuous reactor system. The reactor integrates multiple functional zones (mixing zone, reaction zone, post-condensation zone) that perform sequentially different operations within one vessel, eliminating the need for separate reactors and intermediate transfer steps for salt preparation and heat treatment.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The process operates continuously with monomers being fed constantly into the reactor and polyamide product being discharged continuously. The reaction proceeds without interruption through all stages (salt formation, polycondensation, post-condensation) in a single pass, eliminating batch-to-batch cycles and idle transfer times between operations.

Inventive Principle:
Principle #20Continuity of useful action

2Manufacturing precision

If pre-polymer preparation and additional heat treatment steps are included, then high molar mass polyamide is achieved, but the number of steps increases

Engineering Contradiction:
Improvemolar mass controlVSAvoidnumber of steps
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The reactor design merges the functions of pre-polymerization and post-condensation heat treatment into a single integrated system. The reaction zone performs polycondensation to build molar mass, while the post-condensation zone continues the reaction under different conditions (reduced pressure, higher temperature) to achieve final high molar mass and extrusion-grade viscosity, all within one continuous process.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The process utilizes parameter changes along the reactor length to achieve different reaction stages. Temperature increases from the mixing zone to the reaction zone and further to the post-condensation zone. Pressure conditions are modified in the post-condensation zone (reduced pressure applied) to facilitate water removal and drive the polycondensation reaction to completion for high molar mass product.

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If material transfer between different stages is required, then complete polycondensation is achieved, but transfer operations become difficult to scale industrially

Engineering Contradiction:
Improvepolycondensation completionVSAvoidindustrial scalability
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The patent eliminates material transfer between stages by combining all polycondensation operations within a single continuous reactor. The material flows continuously through mixing, reaction, and post-condensation zones without being discharged and re-fed. This eliminates transfer operations entirely, making the process inherently scalable from pilot to industrial production.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The continuous flow through the reactor ensures that polycondensation completion is achieved without interruption or transfer. The residence time in the reactor is controlled to ensure complete reaction, and the continuous operation allows for easy scaling by simply increasing production rate or reactor size without changing the fundamental process architecture or adding transfer equipment.

Inventive Principle:
Principle #20Continuity of useful action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process significantly reduces production time, eliminates the need for pre-polymer preparation and heat treatment, and enhances productivity by confining the reaction in a metal envelope, allowing for easier scale-up from pilot to production and improving the resistance to pressure and temperature.

Implementation Method 1

A process for the polycondensation of a polyamide polymer by reactive extrusion

Methodology Applied
Scientific EffectPolycondensation: Chemical Bonding

Implementation Method 2

confining the reaction in a metal envelope, allowing for easier scale-up from pilot to production and improving the resistance to pressure and temperature

Methodology Applied
Scientific EffectPhysical containment: Physical Containment

Data Source

PatentEP2877516B1Method for preparing a polyamide by reactive extrusion, and extruder adapted for the implementation of such a method
Publication Date: 2018.04.04 SETUP PERFORMANCE
  • EP2877516B1 patent drawingFigure 1~3
  • EP2877516B1 patent drawingFigure 4~8
  • EP2877516B1 patent drawing

AI summary

The invention concerns a method for preparing a polyamide from one or a plurality of monomers suitable for the preparation of a polyamide characterised in that the selected monomer or monomers are introduced, without any prior reaction and without any prior preparation of the corresponding salt, into an extruder comprising at least two feed screws rotating in a co-rotating manner and in that all of the steps of reaction and polycondensation, starting initially with the selected monomer or monomers, and making it possible to achieve the desired polyamide, are carried out in an extruder comprising at least two feed screws rotating in a co-rotating manner, and the polycondensation is carried out by conducting at least two operations of evacuating the by-product or by-products formed by the polycondensation reaction.