Two-Stage Membrane Biogas Purification for Methane Liquefaction

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Solution Overview

Problem

Existing biogas purification methods for producing high-purity methane are energy-inefficient, use harmful chemicals, require high operating costs, and do not integrate well with liquefaction processes, while traditional CO2 management is inefficient and discontinuous.

Innovation Solution

A two-stage purification process using membrane separation units to achieve methane purity of less than 5% CO2 in the first stage and less than 400 ppm CO2 in the second stage, combined with efficient heat exchange systems and optional distillation, to produce high-purity methane suitable for liquefaction, with CO2 valorization.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If traditional purification methods (amine scrubbing, adsorption) are used to achieve high methane purity, then CO2 removal efficiency is improved, but energy consumption increases and harmful chemicals are used

Engineering Contradiction:
Improvemethane purityVSAvoidenergy consumption
Core Design Contradiction:
Manufacturing precisionVSUse of energy by moving object

Solution Approach 1:

The purification process is divided into two distinct stages: a first purification stage using membrane separation to remove the bulk of CO2, and a second polishing stage using adsorption to achieve high purity. This segmentation allows each stage to be optimized for its specific function, reducing overall energy consumption compared to using a single high-performance method throughout.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

A membrane separation unit is introduced as an intermediary component between the raw biogas and the final polishing stage. The membrane unit performs preliminary CO2 removal, reducing the burden on the subsequent adsorption system and thereby lowering total energy consumption while avoiding the need for high-energy amine scrubbing processes.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Manufacturing precision

If amine scrubbing is used for CO2 removal, then purification efficiency is improved, but harmful chemicals are introduced and operating costs increase

Engineering Contradiction:
ImproveCO2 removal efficiencyVSAvoidharmful chemicals
Core Design Contradiction:
Manufacturing precisionVSObject-generated harmful factors

Solution Approach 1:

The harmful amine chemicals are completely extracted from the purification process and replaced with a membrane separation unit that uses physical selective permeation. This extraction of the harmful substance eliminates the associated environmental and safety issues while maintaining effective CO2 removal capability.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The chemical absorption mechanism of amine scrubbing is replaced with a physical membrane separation process. The membrane unit uses selective permeability based on gas properties rather than chemical reactions, eliminating harmful chemicals from the system while achieving comparable or superior CO2 removal efficiency.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Manufacturing precision

If adsorption units (PTSA, PSA, TSA) are used for fine polishing, then methane purity is improved, but process complexity and operating costs increase

Engineering Contradiction:
Improvemethane purityVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

Instead of using complex multi-component adsorption systems (PTSA, PSA, TSA) for the entire purification process, the invention applies adsorption only partially in the second polishing stage after preliminary CO2 removal by membrane separation. This partial application reduces process complexity while achieving the required high purity level.

Inventive Principle:
Principle #16Partial or excessive action

4Manufacturing precision

If traditional purification stages are implemented, then CO2 content is reduced, but energy efficiency deteriorates and CO2 management is discontinuous

Engineering Contradiction:
ImproveCO2 contentVSAvoidenergy efficiency
Core Design Contradiction:
Manufacturing precisionVSLoss of energy

Solution Approach 1:

The membrane separation unit operates continuously to remove CO2 from the biogas stream, providing continuous CO2 management rather than discontinuous batch processing. This continuous operation improves energy efficiency by eliminating idle times and maintaining steady-state conditions throughout the purification process.

Inventive Principle:
Principle #20Continuity of useful action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process achieves energy-efficient, continuous production of high-purity methane for liquefaction, reduces operating costs, and effectively manages CO2, optimizing methane recovery and utilization.

Implementation Method 1

a second purification unit (7) comprising a membrane separation unit configured to produce the second gas stream enriched in methane with less than 400 ppm of carbon dioxide

Methodology Applied
Scientific EffectPermeation: Permeation

Implementation Method 2

the first heat exchange system being configured to exchange heat between the cold source and the first methane-enriched gas stream in order to cool the first methane-enriched gas stream

Methodology Applied
Scientific EffectHeat exchange: Heat Exchanger

Data Source

PatentEP4640299A1System and method for treating biogas
Publication Date: 2025.10.29 LAIR LIQUIDE SA POUR LETUDE & LEXPLOITATION DES PROCEDES GEORGES CLAUDE
  • EP4640299A1 patent drawingFigure 1~2
  • EP4640299A1 patent drawingFigure 3
  • EP4640299A1 patent drawing

AI summary

Installation (1) for the treatment of a gas stream (10), in particular biogas, comprising methane and carbon dioxide, the installation (1) comprising a first cold source (6) and a gas circuit for the gas stream (10), the gas circuit comprising, arranged in series and fluidly connected by a set of pipes, a first compressor (2), a first purification unit (3) configured to produce a first gas stream enriched in methane (11) with less than 5% carbon dioxide, and a gas stream enriched in carbon dioxide (12), a first heat exchange system (4, 5), and a second purification unit (7) configured to produce a second gas stream enriched in methane (13) with less than 400 ppm of carbon dioxide, and a gas stream depleted in methane (14).