Upflow Alkylene Glycol Reactor with Ion Exchange Resin

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Solution Overview

Problem

Current processes for producing monoalkylene glycol from alkylene oxides using liquid phase hydrolysis are inefficient due to the need for large amounts of water, which increases production costs and requires energy-intensive water removal, and existing catalytic processes face challenges with catalyst swelling and selectivity issues.

Innovation Solution

A catalytic hydrolysis process using an ion exchange resin catalyst in an upflow reactor direction, allowing for fluidization of the catalyst bed, which extends catalyst lifetime, facilitates catalyst replacement, and improves selectivity by maintaining a higher void space and preventing particle trapping, thus reducing pressure drop and mechanical damage.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If a large excess of water is added to increase selectivity towards monoalkylene glycol, then the selectivity is improved, but the energy consumption and production costs increase due to water removal requirements

Engineering Contradiction:
Improveselectivity to monoalkylene glycolVSAvoidenergy consumption for water removal
Core Design Contradiction:
Manufacturing precisionVSUse of energy by moving object

Solution Approach 1:

The invention extracts and removes the harmful factor (excess water) from the system by using a heterogeneous catalyst that enables high selectivity with reduced water requirements, eliminating the need for energy-intensive water removal processes while maintaining high monoalkylene glycol selectivity

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention changes the reaction parameters by introducing a heterogeneous catalyst (ion exchange resin) that alters the reaction mechanism, allowing the process to achieve high selectivity with lower water-to-oxide ratios, thereby reducing the energy burden of water removal

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If a heterogeneous catalyst based on ion exchange resin is used to increase selectivity, then the selectivity to monoalkylene glycol is improved, but the catalyst swells and requires periodic replacement which disrupts production

Engineering Contradiction:
Improveselectivity to monoalkylene glycolVSAvoidproduction continuity
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The invention makes the catalyst bed dynamic by implementing fluidization technology, allowing the catalyst particles to move freely within the reactor. This dynamic state enables continuous operation even during catalyst replacement, as spent catalyst can be removed and fresh catalyst added without shutting down the reactor, thus maintaining production continuity while using swellable ion exchange resin catalysts

Inventive Principle:
Principle #15Dynamics

Solution Approach 2:

The invention implements a system where spent catalyst is continuously discarded and replaced with fresh catalyst through the fluidized bed mechanism. The catalyst circulation system allows for periodic regeneration or replacement of catalyst particles without interrupting the overall production process, ensuring continuous monoalkylene glycol synthesis

Inventive Principle:
Principle #34Discarding and recovering

3Stability of the object's composition

If downflow operation is used in the reactor, then the catalyst bed stability is maintained, but the catalyst lifetime is reduced and selectivity decreases over time

Engineering Contradiction:
Improvecatalyst bed stabilityVSAvoidcatalyst lifetime
Core Design Contradiction:
Stability of the object's compositionVSDuration of action of stationary object

Solution Approach 1:

The invention inverts the conventional downflow operation by implementing upflow operation where the fluid flows upward through the catalyst bed. This inversion reduces mechanical stress and channeling effects on the catalyst particles, minimizing catalyst degradation and maintaining both bed stability and high selectivity over extended operational periods, thereby extending catalyst lifetime

Inventive Principle:
Principle #13The other way round (Inversion)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The upflow process enhances catalyst lifetime by up to twice that of downflow operations, allows for on-stream catalyst replacement, and maintains selectivity over a longer period, reducing energy costs and operational disruptions.

Implementation Method 1

reacting water and ethylene oxide in the presence of a catalyst to form monoethylene glycol

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 2

said reactor is operating in an upflow direction at an upward velocity sufficient to fluidize the catalyst bed

Methodology Applied
Scientific EffectFluidization: Fluidisation

Implementation Method 3

The prior art hydrolysis reaction is a nucleophilic substitution reaction, in which ring opening of the alkylene oxide occurs and water serves as the nucleophile

Methodology Applied
Scientific EffectNucleophilic substitution:

Implementation Method 4

Alkylene glycols are typically prepared from their corresponding alkylene oxide utilizing a liquid phase hydrolysis process

Methodology Applied
Scientific EffectHydrolysis: Hydrolysis

Data Source

PatentEP2162417B1Process for preparing an alkylene glycol
Publication Date: 2019.03.06 SD LIZENZVERWERTUNGSGESELLSCHAFT MBH & CO KG
  • EP2162417B1 patent drawingFigure 1~2
  • EP2162417B1 patent drawingFigure 3

AI summary

A catalytic process for preparing a monoalkylene glycol from a corresponding alkylene oxide utilizing an ion exchange resin and a reactor in which an upflow process is used is provided. In particular, the process includes reacting water and an alkylene oxide in at least one reactor under conditions to form an alkylene glycol, wherein the at least one reactor includes an ion exchange resin and the reactor is operating in an upflow direction.