USY Zeolite Hydrorefining Catalyst Isomerization

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Solution Overview

Problem

Current hydrorefining methods fail to simultaneously isomerize normal paraffins and reduce oxygen-containing compounds in fuel stocks while maintaining fuel stock yields, as existing catalysts either decompose the fuel or do not effectively convert oxygen-containing compounds.

Innovation Solution

A hydrorefining method involving a catalyst with USY zeolite and specific solid acids, combined with metals from Group VIb and VIII, is used to contact fuel stocks containing normal paraffins and oxygen-containing compounds in the presence of hydrogen, allowing for effective conversion of oxygen-containing compounds to paraffins and isomerization of normal paraffins while preventing fuel stock lightening.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If hydrorefining is performed to convert normal paraffins to isoparaffins, then octane numbers and cold flow properties are improved, but fuel stock yields decrease due to decomposition

Engineering Contradiction:
Improvefuel quality (octane number and cold flow properties)VSAvoidfuel stock yields
Core Design Contradiction:
ReliabilityVSLoss of substance

Solution Approach 1:

The invention changes the chemical parameters of the catalyst system by combining specific metal components (Mo, Co, Ni, Pt, Pd) with USY zeolite support, creating a bifunctional catalyst that operates at lower temperatures to achieve isomerization without decomposition, thus improving fuel quality while maintaining yields

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention uses a composite catalyst material consisting of metal sulfides or metal oxides supported on USY zeolite, combining the hydrodesulfurization activity of metals with the isomerization activity of zeolite, enabling simultaneous conversion of normal paraffins to isoparaffins while preventing fuel stock decomposition

Inventive Principle:
Principle #40Composite materials

2Quantity of substance

If existing catalysts are used for hydrorefining, then normal paraffin conversion is achieved, but oxygen-containing compounds are not effectively reduced

Engineering Contradiction:
Improvenormal paraffin conversion rateVSAvoidoxidation stability (oxygen-containing compound reduction)
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

The invention creates a universal catalyst system that performs multiple functions simultaneously: hydrodesulfurization, isomerization of normal paraffins, and removal/conversion of oxygen-containing compounds, thereby improving both conversion rate and oxidation stability

Inventive Principle:
Principle #6Universality (Multi-functionality)

Solution Approach 2:

The USY zeolite support acts as an intermediary that facilitates the interaction between metal catalyst components and various fuel constituents, enabling effective conversion of oxygen-containing compounds through acid-catalyzed reactions while maintaining metal-catalyzed hydrodesulfurization activity

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method achieves simultaneous isomerization of normal paraffins and reduction of oxygen-containing compounds in fuel stocks, maintaining fuel stock yields and preventing lightening, thereby improving the octane numbers and cold flow properties of the fuel.

Implementation Method 1

contacting, in the presence of hydrogen, a fuel stock comprising normal paraffins and oxygen-containing compounds, with a hydrorefining catalyst comprising a support containing USY zeolite and at least one solid acid selected from among silica-alumina, alumina-boria, silica-zirconia, silica-magnesia and silica-titania, and at least one metal selected from among metals of Group VIb and metals of Group VIII of the Periodic Table supported on the support

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 2

effective conversion of the oxygen-containing compounds such as alcohols in the fuel stock to paraffins

Methodology Applied
Scientific EffectHydrogenation: Hydrogenation

Implementation Method 3

effective conversion (isomerization) of the normal paraffins derived from the oxygen-containing compounds and the normal paraffins originally present in the fuel stock

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 4

sufficiently inhibit lightening of the fuel stock that occurs with conversion of the oxygen-containing compounds to paraffins and isomerization to normal paraffins

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentUS8852428B2Hydrorefining method
Publication Date: 2014.10.07 NIPPON OIL CORP

AI summary

The hydrorefining method of the invention is characterized by contacting, in the presence of hydrogen, a fuel stock comprising normal paraffins and oxygen-containing compounds, with a hydrorefining catalyst comprising a support containing USY zeolite and at least one solid acid selected from among silica-alumina, alumina-boria, silica-zirconia, silica-magnesia and silica-titania, and at least one metal selected from among metals of Group VIb and metals of Group VIII of the Periodic Table supported on the support.