VAM Purification With Two-Stage Distillation for Ethyl Acetate Removal

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Solution Overview

Problem

Current VAM production processes face challenges in efficiently and cost-effectively reducing the amount of ethyl acetate in the finished vinyl acetate monomer product due to similar boiling behaviors, leading to high energy consumption and impurity retention.

Innovation Solution

A two-stage distillation process is implemented, where the side draw from the azeotropic distillation tower is positioned to maintain a constant water content in the bottom product, enhancing the ETAC-enriched vapor stream, which is then processed in a secondary distillation tower to separate and recover valuable components for recycling.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If azeotropic distillation is used to purify VAM, then VAM can be separated from acetic acid and water, but ethyl acetate cannot be effectively removed due to similar boiling behavior

Engineering Contradiction:
ImproveVAM purification qualityVSAvoidethyl acetate content in product
Core Design Contradiction:
Manufacturing precisionVSQuantity of substance

Solution Approach 1:

The distillation process is divided into two separate stages: first azeotropic distillation to separate VAM from acetic acid and water, then a second distillation column specifically dedicated to removing ethyl acetate. This segmentation allows each column to be optimized for its specific separation task, with the second column receiving a feed stream that is already enriched in ethyl acetate relative to other components.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

A side stream is extracted from the azeotropic distillation column that is enriched in ethyl acetate. This side stream is then fed to a second distillation column where ethyl acetate is selectively removed. By extracting and treating the ethyl acetate-rich stream separately, the main VAM product stream is protected from contamination while ethyl acetate removal is addressed in a dedicated unit.

Inventive Principle:
Principle #2Taking out (Extraction)

2Quantity of substance

If secondary distillation is implemented to remove ethyl acetate, then ethyl acetate content in VAM product is reduced, but energy consumption increases

Engineering Contradiction:
Improveethyl acetate content in productVSAvoiddistillation energy consumption
Core Design Contradiction:
Quantity of substanceVSUse of energy by moving object

Solution Approach 1:

The second distillation column is designed with localized optimization for ethyl acetate removal. The column configuration, including tray arrangement and reflux ratio, is specifically tailored to achieve efficient ethyl acetate separation while minimizing energy consumption. The side stream feed location is strategically positioned to maximize ethyl acetate recovery efficiency.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The process recovers ethyl acetate from the side stream of the azeotropic distillation column and concentrates it in the second distillation column. The ethyl acetate-rich bottom product from the second column can be discarded as waste or recovered for potential reuse, while the overhead product returns to the main VAM product stream with reduced ethyl acetate content.

Inventive Principle:
Principle #34Discarding and recovering

3Manufacturing precision

If side draw position is optimized to maintain constant water content, then bottom product quality is improved, but process complexity increases

Engineering Contradiction:
Improvebottom product water content controlVSAvoiddistillation tower configuration
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The side draw position in the azeotropic distillation column is determined based on feedback from the desired bottom product water content specification. By positioning the side draw at the appropriate tray location, the column automatically maintains the target water content in the bottom product through the natural concentration gradients established during distillation operation.

Inventive Principle:
Principle #23Feedback

Solution Approach 2:

The azeotropic distillation column is designed with a predetermined side draw position that is calculated based on mass balance and equilibrium considerations. This preliminary design ensures that the bottom product will have the desired water content without requiring complex real-time control adjustments during operation.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach reduces ethyl acetate content in the VAM product, decreases energy and water consumption, and improves overall production efficiency by allowing for the recovery and recycling of valuable materials.

Implementation Method 1

This crude stream can be purified by an azeotropic distillation, between VAM and water, in the purification section of the VAM plant

Methodology Applied
Scientific EffectAzeotropic distillation: Distillation

Implementation Method 2

The overhead product is condensed and further separated into an organic phase containing VAM, a water phase

Methodology Applied
Scientific EffectCondensation: Condensation

Implementation Method 3

an ethyl acetate enriched liquid stream is obtained as a side stream... separation of the ethyl acetate requires a high energy consumption

Methodology Applied
Scientific EffectDistillation: Distillation

Data Source

PatentEP4010310B1Ethyl acetate removal during VAM production
Publication Date: 2025.10.22 LYONDELLBASELL ACETYLS LLC
  • EP4010310B1 patent drawingFigure 1
  • EP4010310B1 patent drawingFigure 2

AI summary

Purification methods and systems for working up a crude vinyl acetate stream containing vinyl acetate monomer, acetic acid, water, ethyl acetate, and other impurities. Crude vinyl acetate streams are purified with an azeotropic distillation tower using a side draw to remove ethyl acetate and water, and a bottom stream to remove acetic acid from the crude vinyl acetate. The methods and systems move the side draw to a location on the azeotropic distillation tower that maintains a constant water concentration in the bottom product of about 4 to about 15 wt. % and forms a vapor side product. A second distillation tower is used to further purify the vapor side product to obtain water, VAM, ethyl acetate and AA. The system provides easier disposal of ethyl acetate, and cleaner water that can be recycled in the reactor or purification sections of a VAM plant and full recovery of AA.