VDF Fluoropolymer Binder Composition for Dry Electrode Metal Adhesion

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Solution Overview

Problem

Current dry electrode processes for batteries face challenges with adhesion of fluoropolymer binders to metal current collectors, particularly PTFE, which lacks sufficient adhesion while maintaining stability in electrolyte solvents and high temperatures.

Innovation Solution

Development of VDF-based copolymers with specific melting points and semi-crystalline properties that exhibit improved adhesion to metals, enabling their use as binders in dry electrode processes and extrusion at low temperatures, forming self-supporting films without the need for solvents or primers.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If PTFE binder is used in dry electrode processes, then good cohesion with electrode active material and stability in electrolyte solvents at high temperatures is achieved, but adhesion to current collector deteriorates

Engineering Contradiction:
Improvestability in electrolyte solventVSAvoidadhesion to current collector
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The patent modifies the chemical composition parameters of the fluoropolymer binder by incorporating specific comonomers (VDF, HFP, TFE) in controlled ratios to achieve optimal balance between adhesion and stability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite fluoropolymer system combining multiple monomer units (VDF, HFP, TFE) to achieve synergistic properties that neither monomer alone can provide, specifically improving both adhesion and solvent resistance

Inventive Principle:
Principle #40Composite materials

2Ease of manufacture

If PTFE binder is used to form free-standing films, then good processability is achieved, but adhesion to current collector deteriorates

Engineering Contradiction:
ImproveprocessabilityVSAvoidadhesion to current collector
Core Design Contradiction:
Ease of manufactureVSStrength

Solution Approach 1:

The patent adjusts the molecular composition parameters of the fluoropolymer to enable both film formation and adhesion, using specific VDF/HFP/TFE ratios that provide appropriate melt behavior and surface properties

Inventive Principle:
Principle #35Parameter changes

3Strength

If wet process is used for electrode manufacturing, then good adhesion to current collector is achieved, but drying time and cost increase

Engineering Contradiction:
Improveadhesion to current collectorVSAvoiddrying time
Core Design Contradiction:
StrengthVSLoss of time

Solution Approach 1:

The patent extracts and eliminates the drying step from the electrode manufacturing process by using a dry process approach with fluoropolymer binders that provide sufficient adhesion without requiring solvent evaporation

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent replaces the thermal drying process with a mechanical compaction process, using pressure and cold isostatic pressing to form electrodes without thermal treatment

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The VDF-based copolymers demonstrate enhanced adhesion to metal current collectors, facilitating efficient electrode production with improved processability and maintaining excellent electrical properties, suitable for use in secondary batteries and other electrochemical devices.

Implementation Method 1

polymer (A) has at least two melting points, one melting point lower than 220°C. and one melting point higher than 250°C.

Methodology Applied
Scientific EffectMelting: Melting

Data Source

PatentUS20250023053A1TFE-based fluoropolymers with outstanding metal-adhesion properties
Publication Date: 2025.01.16 SOLVAY SPECIALTY POLYMERS ITALY SPA

AI summary

The present invention relates to VDF-based fluoropolymers with outstanding metal-adhesion properties for use as a binding agent for electrodes for batteries.