Mixed Waste Plastic Joule Heating for Graphene and Hydrogen

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Solution Overview

Problem

Current plastic waste recycling technologies face challenges such as time- and energy-consuming sorting and purification requirements, low economic feasibility, high greenhouse gas emissions, and low selectivity for desirable products, leading to limited practical applications and environmental issues.

Innovation Solution

A method and device utilizing Joule heat to convert waste plastics into graphene and hydrogen gas, employing an airtight reaction chamber, gas collecting system, and power control system to rapidly transform mixed plastics into high-purity graphene and hydrogen gas with minimal energy consumption and simplified sorting.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If mechanical recycling is used, then the process is simple and widely used, but it cannot handle temperature-sensitive plastics, composites, thermosets and requires complex pre-sorting process

Engineering Contradiction:
Improveprocess simplicityVSAvoidplastic type handling capability
Core Design Contradiction:
Ease of manufactureVSAdaptability or versatility

Solution Approach 1:

The patent changes the fundamental processing parameter from mechanical action to thermal action (heating to 700-900°C). This temperature parameter change enables the processing of previously incompatible materials like thermosets and composites, while the high temperature also vaporizes contaminants, eliminating the need for complex pre-sorting

Inventive Principle:
Principle #35Parameter changes

2Adaptability or versatility

If plastic cracking technology is used, then it can process various plastics, but the process is complex, energy-consuming and has poor selectivity for desirable products

Engineering Contradiction:
Improveplastic type processing capabilityVSAvoidprocess complexity
Core Design Contradiction:
Adaptability or versatilityVSDevice complexity

Solution Approach 1:

The patent extracts and isolates the desired products (hydrogen gas and carbon materials) through a simplified thermal process. By heating to high temperatures, the plastic decomposes and hydrogen gas is released and collected, while carbon remains as solid residue. This extraction approach eliminates complex purification steps while maintaining high product selectivity

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent replaces complex mechanical cracking systems with a thermal system. Instead of using mechanical force, catalysts, and multiple processing stages, the invention uses controlled heating to achieve decomposition and product separation, significantly simplifying the overall process

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Ease of operation

If incineration is used, then it does not require complicated pretreatment process and can generate electricity, but monomers derived from fossil fuels are only partially recovered in the form of heat energy and lose their recycling value

Engineering Contradiction:
Improvepretreatment requirementVSAvoidrecycling value loss
Core Design Contradiction:
Ease of operationVSLoss of substance

Solution Approach 1:

The patent changes the temperature parameter and heating rate to achieve selective decomposition rather than complete combustion. By controlling the thermal parameters (heating to 700-900°C without oxygen), the process recovers hydrogen gas and carbon materials in concentrated forms, preserving their recycling value while still requiring minimal pretreatment

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method achieves high-value conversion of mixed plastics into high-purity graphene and hydrogen gas with low energy consumption, eliminating the need for further purification and reducing environmental impact, thereby improving resource efficiency and economic benefits.

Implementation Method 1

converting waste plastics with Joule heat

Methodology Applied
Scientific EffectJoule heating: Joule Heating

Data Source

PatentUS12398041B2Method and device for preparing graphene and hydrogen gas by converting waste plastics with joule heat
Publication Date: 2025.08.26 TONGJI UNIV
  • US12398041B2 patent drawing

AI summary

A method and a device for preparing graphene and hydrogen gas by converting waste plastics with Joule heat are provided according to the present application. The method uses the Joule heat generated when a strong current passes through the mixed plastic material mixed with conductive additive, as the reaction driving energy. By Joule heating, carbon-carbon bonds and carbon-hydrogen bonds are broken, amorphous carbon is converted into sp2 hybridized high-purity graphene, and hydrogen atoms are converted into hydrogen gas. The reaction device used by the method is mainly composed of three parts: an airtight reaction chamber, a gas collecting system and a power control system.