Water Selective Separators for Flue Gas Heat Recovery

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

The high water vapor content in flue gas from syngas combustors in IGCC plants prevents the recovery of heat for power generation due to the need to maintain temperatures above the dew point, leading to energy inefficiency and potential corrosion issues.

Innovation Solution

Implementing a power plant with a combustor and downstream water selective separators to remove water from the flue gas, allowing for heat recovery and reusing the separated water in the syngas production process to increase hydrogen content without increasing water consumption, using membranes like hydrophilic stainless steel or ceramic filters to achieve high water recovery efficiency.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Loss of energy

If water selective separators are used to remove water from flue gas, then heat recovery efficiency is improved, but device complexity increases

Engineering Contradiction:
Improveheat recovery efficiencyVSAvoiddevice complexity
Core Design Contradiction:
Loss of energyVSDevice complexity

Solution Approach 1:

The patent extracts water vapor from the flue gas stream using water selective separators (membranes) positioned downstream of the combustor. By removing water before the heat exchanger, the flue gas temperature can be reduced more effectively without condensing water, enabling更高效 heat recovery while preventing corrosion.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The water selective separator acts as an intermediary component between the combustor and heat exchanger. It selectively removes water vapor from the flue gas, allowing the system to achieve lower temperatures in the heat exchanger without water condensation, thus enabling more efficient heat recovery while protecting against corrosion.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Reliability

If flue gas temperature is maintained above dew point to prevent corrosion, then equipment reliability is improved, but heat recovery efficiency deteriorates

Engineering Contradiction:
Improveequipment reliabilityVSAvoidheat recovery efficiency
Core Design Contradiction:
ReliabilityVSLoss of energy

Solution Approach 1:

The patent extracts water vapor from the flue gas using water selective separators before the gas enters the heat exchanger. This removal of water allows the flue gas temperature to be reduced below the original dew point without causing water condensation and corrosion, thereby improving heat recovery efficiency while maintaining equipment reliability.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent changes the composition parameter of the flue gas by removing water vapor. This parameter change effectively lowers the dew point temperature of the flue gas, allowing the system to operate at lower temperatures in the heat exchanger without water condensation, thus improving heat recovery while preventing corrosion.

Inventive Principle:
Principle #35Parameter changes

3Loss of energy

If hydrogen content in syngas is increased through water-gas shift reaction, then energy yield is improved, but water consumption increases

Engineering Contradiction:
Improveenergy yieldVSAvoidwater consumption
Core Design Contradiction:
Loss of energyVSQuantity of substance

Solution Approach 1:

The patent recovers water vapor that would otherwise be discarded in the flue gas by using water selective separators to extract it. The recovered water is then fed back to the gasifier and/or CO shift cell, reducing the need for fresh water input while maintaining the water-gas shift reaction for hydrogen production, thus improving energy yield without increasing net water consumption.

Inventive Principle:
Principle #34Discarding and recovering

Solution Approach 2:

The patent implements a feedback loop where water vapor separated from the flue gas is returned to the gasifier and CO shift cell. This feedback mechanism ensures that water consumed in the water-gas shift reaction for hydrogen production is replenished by recovered water, maintaining sustainable operation with reduced net water consumption.

Inventive Principle:
Principle #23Feedback

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach allows for the recovery of about 70% of the flue gas water, which can be reused, reducing energy consumption and improving overall power generation efficiency by enabling more heat recovery and reducing the need for fresh make-up water preparation, while maintaining equipment integrity.

Implementation Method 1

downstream of the flue gas outlet water selective separators are provided to separate water from the flue gas

Methodology Applied
Scientific EffectSelective permeation: Permeation

Implementation Method 2

using membranes like hydrophilic stainless steel or ceramic filters to achieve high water recovery efficiency

Methodology Applied
Scientific EffectHydrophilic absorption: Hydrophile

Implementation Method 3

The hydrogen content in the syngas can be increased by the water-gas shift reaction. With this reaction carbon monoxide reacts with water to form carbon dioxide and hydrogen: CO(g) + H2O(l) → CO2(g) + H2(g)

Methodology Applied
Scientific EffectWater-gas shift reaction: Chemical Transport Reactions

Implementation Method 4

Heat can be extracted from the flue gas discharged from the combustor to be used for generating power, typically via a steam cycle

Methodology Applied
Scientific EffectHeat conduction: Conduction (thermal)

Implementation Method 5

Heat can be extracted from the flue gas discharged from the combustor to be used for generating power

Methodology Applied
Scientific EffectConvection: Convection

Data Source

PatentEP2965006B1Power plant
Publication Date: 2019.07.24 SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ BV
  • EP2965006B1 patent drawingFigure 1

AI summary

A process and a power plant (1) comprising a combustor (7) with a flue gas outlet (8) and one or more water selective separators (9) downstream the flue gas outlet to separate water from the flue gas. Optionally, a water return line (11) returns separated water from the water selective separator (9) to a water inlet of a CO shift cell (5) with an outlet feeding H2 enriched syngas to the combustor.