Water Solvent Crystallization for Organic Acid Purification

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Solution Overview

Problem

Existing methods for purifying organic acids and salts from fermentation broths are complex, costly, and environmentally inefficient, often requiring additional substances that can contaminate the product and consume significant energy.

Innovation Solution

A method utilizing nanofiltration and water solvent crystallization to produce crystalline forms of organic acids and salts, such as mevalonolactone monohydrate, without the use of organic solvents, followed by cation exchange to convert salts into lactones, achieving high purity products suitable for the personal care industry.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If organic solvent extraction or solid phase absorption is used to purify organic acids from fermentation broth, then purification effectiveness is improved, but process complexity and cost increase

Engineering Contradiction:
Improvepurification effectivenessVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The invention changes the fundamental parameter of the purification approach by using water solvent crystallization instead of organic solvent extraction or solid phase absorption. This involves controlling temperature, pH, and concentration parameters to achieve crystallization of the target organic acid from the fermentation broth, thereby simplifying the process while maintaining high purification effectiveness.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention exploits the phase transition of the target organic acid from dissolved state in aqueous solution to crystalline solid state through controlled cooling and concentration. This phase transition enables efficient separation of the purified product from the fermentation broth without requiring complex extraction or adsorption equipment.

Inventive Principle:
Principle #36Phase transitions

2Productivity

If additional substances are supplied to enhance crystallization, then crystallization efficiency is improved, but product purity deteriorates due to contamination

Engineering Contradiction:
Improvecrystallization efficiencyVSAvoidproduct purity
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The invention employs self-service crystallization where the target organic acid crystallizes from the fermentation broth through controlled temperature reduction and concentration without requiring additional crystallization promoters or additives. The process utilizes the inherent properties of the organic acid and its aqueous solution to achieve both high efficiency and high purity.

Inventive Principle:
Principle #25Self-service

3Quantity of substance

If conventional purification methods are used, then organic acid recovery is achieved, but energy consumption increases

Engineering Contradiction:
Improveorganic acid recoveryVSAvoidenergy consumption
Core Design Contradiction:
Quantity of substanceVSUse of energy by moving object

Solution Approach 1:

The invention employs periodic action through controlled temperature cycling - initially concentrating the fermentation broth through evaporation or membrane filtration, then cooling the concentrated solution to induce crystallization. This periodic temperature control enables efficient organic acid recovery with lower energy consumption compared to continuous heating or solvent regeneration processes.

Inventive Principle:
Principle #19Periodic action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method achieves high-purity organic acid products with minimal color formation, suitable for large-scale manufacturing, reducing environmental impact and operational costs while maintaining product quality.

Implementation Method 1

subjecting the aqueous solution comprising said organic acid or salt or lactone thereof to a nanofiltration to produce a permeate

Methodology Applied
Scientific EffectNanofiltration: Semipermeable Membrane

Implementation Method 2

crystallizing said organic acid or salt or lactone thereof from said permeate by water solvent crystallization

Methodology Applied
Scientific EffectCrystallization: Crystallisation

Implementation Method 3

The water solvent crystallization comprises evaporating the permeate to obtain a syrup

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP4706822A2Methods for recovering organic acids or salts or lactones thereof from aqueous solutions using water solvent crystallization and compositions thereof
Publication Date: 2026.03.11 DANISCO US INC
  • EP4706822A2 patent drawingFigure 1A
  • EP4706822A2 patent drawingFigure 1B
  • EP4706822A2 patent drawingFigure 2

AI summary

Compositions and methods are provided for producing crystalline forms of organic acids or salts or lactones thereof from an aqueous solution. More specifically, methods are provided for producing a crystalline form of a salt of mevalonic acid (also referred to as X-MVA) from an aqueous solution, comprising subjecting the aqueous solution comprising said X-MVA to a purification step to produce a purified solution and crystallizing said X-MVA from said purified solution by water solvent crystallization. Methods are also provided for producing mevalonolactone from an aqueous solution comprising X-MVA, comprising subjecting the aqueous solution comprising said X-MVA to cation exchange thereby converting said aqueous solution comprising X-MVA to an aqueous solution comprising mevalonolactone (MVL). Methods are also provided for producing mevalonolactone monohydrate crystals.