Wavelength Converting Element Refractive Index Matching

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Solution Overview

Problem

Existing lighting devices with wavelength converting elements using phosphors with metal-ion activators excited via partially forbidden transitions suffer from high scattering losses due to refractive index mismatches between the phosphor and the encapsulant, leading to inefficient light conversion and increased thickness requirements.

Innovation Solution

A lighting device with a wavelength converting element comprising a Mn(IV)-activated fluoride compound compounded with a polymer, where the refractive index difference between the phosphor and the polymer is minimized to less than 0.1, preferably less than 0.05, to reduce scattering losses and enhance light conversion efficiency, using materials like K2SiF6:Mn(IV) and Na3Li3Al2F12:Mn(IV) with a fluorine-containing polymer, such as a co-polymer of tetrafluoroethylene, hexafluoropropylene, and vinylidene fluoride.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Use of energy by moving object

If phosphors with metal-ion activators excited via partially forbidden transitions are used, then light conversion can be achieved, but scattering losses increase due to refractive index mismatch

Engineering Contradiction:
Improvelight conversion efficiencyVSAvoidscattering losses
Core Design Contradiction:
Use of energy by moving objectVSLoss of energy

Solution Approach 1:

The patent changes the refractive index parameter of the encapsulant material to match that of the phosphor. By selecting an encapsulant with a refractive index between 1.33-1.47, the patent optimizes the optical parameter to minimize scattering losses while maintaining efficient light conversion through the phosphor's partially forbidden transition characteristics.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs a composite encapsulant composition comprising a polymer matrix combined with specific additives or compounds that adjust the overall refractive index to match the phosphor. This composite approach allows precise tuning of the encapsulant's optical properties to reduce scattering while maintaining structural integrity and other required functions.

Inventive Principle:
Principle #40Composite materials

2Use of energy by moving object

If long interaction paths are used to achieve sufficient light conversion, then conversion efficiency improves, but scattering losses increase

Engineering Contradiction:
Improvelight conversion efficiencyVSAvoidinteraction path length
Core Design Contradiction:
Use of energy by moving objectVSLength of stationary object

Solution Approach 1:

By optimizing the refractive index parameter of the encapsulant to match the phosphor, the patent reduces scattering losses per unit length. This allows the use of thinner encapsulant layers with shorter interaction paths while maintaining sufficient light conversion efficiency, thereby resolving the contradiction between conversion efficiency and path length.

Inventive Principle:
Principle #35Parameter changes

3Ease of manufacture

If refractive index mismatch between phosphor and encapsulant is large, then manufacturing is easier, but scattering losses increase

Engineering Contradiction:
Improveencapsulant selectionVSAvoidscattering losses
Core Design Contradiction:
Ease of manufactureVSLoss of energy

Solution Approach 1:

The patent establishes a specific refractive index range (1.33-1.47) for the encapsulant that balances manufacturability with optical performance. This parameter optimization allows selection from a practical range of materials while ensuring minimal scattering losses through refractive index matching with the phosphor.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution significantly reduces scattering losses and achieves efficient light conversion with a compact design, suitable for use in various lighting devices, including LEDs, by matching the refractive indices of the phosphor and polymer, resulting in a cost-effective and efficient wavelength converting element with low scattering.

Implementation Method 1

a phosphor with a metal-ion activator which is excitable via a partially forbidden electronic transition

Methodology Applied
Scientific EffectPartially forbidden electronic transition: Fluorescence

Implementation Method 2

a wavelength converting element arranged to convert at least part of the light with the primary wavelength into light with a secondary wavelength

Methodology Applied
Scientific EffectWavelength conversion: Photoluminescence

Data Source

PatentEP2513246B1Lighting device with light source and wavelength converting element
Publication Date: 2014.02.26 PHILIPS INTPROP & STANDARDS GMBH
  • EP2513246B1 patent drawingFigure 1~2

AI summary

The invention relates to a lighting (1) device comprising a light source (2) and a wavelength converting element (7), which comprises a phosphor compounded with a polymer. The phosphor contains a metal- ion activator which is excitable via a partially forbidden electronic transition. The phosphor and the polymer being chosen such that the difference in their refractive index is smaller than 0.1. Due to this choice, scattering in the wavelength converting element (7) remains at minimum. Interesting wavelength converting elements (7) are obtained when using phosphors comprising specific Mn(IV)-activated fluoride compounds and specific fluorine-containing polymers.