WC-W Super-Hard Sintered Material Without W2C Formation

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Solution Overview

Problem

Sintered materials containing tungsten (W) and tungsten carbide (WC) face challenges with the generation of low-strength WC (W2C) at high temperatures, leading to reduced hardness and strength, especially when used in severe conditions or high-temperature applications.

Innovation Solution

A super-hard sintered material is developed using nano-sized W and WC powders with adjusted grain sizes and sintering conditions at 1450°C or less to prevent W2C formation, employing a hydrogen reduction method and hot press or spark plasma sintering techniques to achieve high hardness and strength without generating W2C.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Temperature

If sintering is performed at high temperature (1750-1900°C) to obtain cemented carbide with W binder phase, then the material can be formed with WC and W, but W transforms into W2C which has low hardness and low strength

Engineering Contradiction:
Improvesintering temperatureVSAvoidhardness and strength
Core Design Contradiction:
TemperatureVSStrength

Solution Approach 1:

The patent changes the sintering temperature parameter from conventional high temperature (1750-1900°C) to a lower range (1400-1650°C), which prevents W transformation into W2C while still achieving complete sintering. This parameter change resolves the contradiction by finding an optimal temperature window that maintains both formability and mechanical properties.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent performs preliminary classification of WC particles to create a specific particle size distribution before sintering. This preliminary action ensures proper packing and sintering behavior at the lower temperature, preventing W2C formation while achieving dense microstructure and high strength.

Inventive Principle:
Principle #10Preliminary action

2Stability of the object's composition

If sintering temperature is increased to improve densification, then compactness improves, but W transforms into W2C which reduces hardness

Engineering Contradiction:
ImprovecompactnessVSAvoidhardness
Core Design Contradiction:
Stability of the object's compositionVSStrength

Solution Approach 1:

The patent identifies and applies an optimal sintering temperature range (1400-1650°C) that achieves complete densification and compactness without causing W transformation into W2C. This parameter optimization resolves the contradiction by finding the temperature window where both compactness and hardness are maximized.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting material exhibits excellent high hardness, strength, compactness, and corrosion resistance, suitable for cutting tools and high-temperature applications, with no detectable W2C by X-ray diffraction, extending tool life and maintaining hardness across varying temperatures.

Implementation Method 1

a sintered material in which WC (tungsten carbide) particles known as a high hardness, high strength and high melting point ceramic are set as a hard phase, and tungsten metal (W) having high affinity with WC and high strength and high melting point like WC is set as a binder phase

Methodology Applied
Scientific EffectSintering: Sintering

Implementation Method 2

employing a hydrogen reduction method and hot press or spark plasma sintering techniques

Methodology Applied
Scientific EffectHydrogen reduction: Reduction

Data Source

PatentEP3480328B1Super hard sintered body
Publication Date: 2022.05.11 MITSUBISHI MATERIALS CORP
  • EP3480328B1 patent drawingFigure 1
  • EP3480328B1 patent drawingFigure 2~3

AI summary

Provided is a super-hard sintered material which contains 5 to 55 mass% of W and a WC balance containing inevitable impurities and is excellent in high hardness and high strength.