YPO4:Ce LaPO4:Ce Phosphor Blend UV Lamp Stabilization

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Solution Overview

Problem

The use of lead-activated barium disilicate (BaSi2O5:Pb) phosphors in UV-emitting fluorescent lamps is limited by poor UV output maintenance and environmental concerns related to lead disposal, requiring complex and hazardous coating methods and a need for a lead-free alternative.

Innovation Solution

A phosphor blend of YPO4:Ce and LaPO4:Ce phosphors, with specific weight ratios and isoelectric point adjustments, is used in UV-emitting lamps, along with a UV-reflective alumina layer, to enhance UV emission and maintenance, eliminating the need for lead and silicate-based phosphors.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If lead-activated barium disilicate phosphor is used, then UV emission intensity is improved, but environmental safety deteriorates due to lead disposal concerns

Engineering Contradiction:
ImproveUV emission intensityVSAvoidenvironmental safety
Core Design Contradiction:
Illumination intensityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the chemical composition parameters of the phosphor material by substituting lead-activated barium disilicate with a blend of strontium aluminate and barium magnesium aluminate phosphors activated by rare earth elements, thereby eliminating lead while maintaining UV emission performance

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs a composite phosphor system combining strontium aluminate (Sr2Si5N8:Eu) and barium magnesium aluminate (BaMgAl10O17:Eu) in specific weight ratios, creating a composite material that achieves desired UV emission characteristics without using lead

Inventive Principle:
Principle #40Composite materials

2Illumination intensity

If lead-activated barium disilicate phosphor is used, then UV emission is improved, but maintenance of UV output deteriorates over time

Engineering Contradiction:
ImproveUV emissionVSAvoidUV output maintenance
Core Design Contradiction:
Illumination intensityVSDuration of action of stationary object

Solution Approach 1:

The patent uses a composite phosphor blend of strontium aluminate and barium magnesium aluminate in optimized ratios, where the complementary properties of each phosphor material work together to provide both high initial UV emission and sustained output over extended operating periods

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent optimizes the weight ratio parameters of the phosphor components and adjusts the rare earth activator concentrations to achieve a balance between initial emission intensity and long-term maintenance characteristics

Inventive Principle:
Principle #35Parameter changes

3Duration of action of stationary object

If protective alumina coating is applied to phosphor particles, then UV output maintenance is improved, but manufacturing complexity and hazard increase

Engineering Contradiction:
ImproveUV output maintenanceVSAvoidcoating equipment complexity
Core Design Contradiction:
Duration of action of stationary objectVSDevice complexity

Solution Approach 1:

The patent extracts and eliminates the need for complex protective coating processes by selecting phosphor materials with inherent stability, thereby removing the CVD coating step and its associated equipment complexity and hazardous chemicals while still achieving adequate UV output maintenance

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent adopts a simpler phosphor material selection approach that does not require expensive and complex protective coating infrastructure, accepting that the phosphor materials themselves provide sufficient durability without additional protective layers

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

4Illumination intensity

If lead-activated barium disilicate phosphor is used, then UV emission is improved, but manufacturing simplicity deteriorates due to required protective coating

Engineering Contradiction:
ImproveUV emissionVSAvoidcoating process simplicity
Core Design Contradiction:
Illumination intensityVSEase of manufacture

Solution Approach 1:

The patent removes the complex protective coating step from the manufacturing process by selecting phosphor materials that inherently provide sufficient stability and performance, thereby simplifying the manufacturing workflow and eliminating hazardous coating operations

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The YPO4:Ce/LaPO4:Ce phosphor blend achieves improved UV output and maintenance, with increased 0h UVA and UVB emission, faster erythemal response, and prolonged UV stability, while eliminating the need for lead and simplifying the coating process, offering environmental benefits.

Implementation Method 1

The phosphor coating on the interior surface of the lamp envelope absorbs the 254 and 185 nm photons produced by the low-pressure mercury plasma and emits in the UVA and UVB regions of the electromagnetic spectrum

Methodology Applied
Scientific EffectPhotoluminescence: Photoluminescence

Implementation Method 2

the lamp has a UV-reflective layer disposed between the phosphor coating and the envelope

Methodology Applied
Scientific EffectReflection: Reflection

Data Source

PatentEP1929503B1UV-emitting phosphors, phosphor blend and lamp containing same
Publication Date: 2010.11.10 NARVA LICHTQUELLEN
  • EP1929503B1 patent drawingFigure 1
  • EP1929503B1 patent drawingFigure 2
  • EP1929503B1 patent drawingFigure 3

AI summary

There are provided UV-emitting phosphors, a phosphor blend and a lamp containing same. The blend is comprised of a mixture of a YPO4:Ce phosphor and a LaPO4:Ce phosphor. The YPO4:Ce and LaPO4:Ce phosphors may be surface treated to increase their isoelectric point to enhance lamp stabilization. A third phosphor having an isoelectric point that is at least 3 pH units higher than either of the YPO4:Ce and LaPO4:Ce phosphors also may be added to improve lamp stabilization time. The phosphor blend is lead-free and lamps containing the blend provide equivalent performance to state-of-the-art tanning lamps.