Zeolite Catalyst Extrusion with Inorganic Binder

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Solution Overview

Problem

Zeolite-based catalysts face challenges in extrusion due to their specific properties and morphology, requiring higher binder proportions for mechanical stability, which reduces catalytic activity per unit volume.

Innovation Solution

A process involving diatomaceous earth particles with mesoporosity, treated through hydrothermal crystallization and ion-exchange to form a zeolite-based catalyst composition with a high proportion of ion-exchanged zeolite as a binder, enhancing mechanical stability and catalytic activity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If higher proportions of binder are used to achieve sufficient mechanical stability of zeolite-based catalysts, then mechanical stability is improved, but the proportion of catalytically active component decreases, reducing specific catalytic activity per unit volume

Engineering Contradiction:
Improvemechanical stabilityVSAvoidproportion of catalytically active component
Core Design Contradiction:
StrengthVSQuantity of substance

Solution Approach 1:

The patent changes the chemical composition parameters of the binder from conventional organic binders to inorganic binder components (such as water glass, alumina, or silica) that can serve dual functions: providing mechanical stability and contributing to catalytic activity. This parameter change allows the binder to replace part of the catalytically active zeolite material while maintaining or enhancing mechanical strength.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The inorganic binder components are designed to perform multiple functions simultaneously: they provide mechanical stability as a binder, contribute to the structural integrity of the extruded catalyst body, and when catalytically activated through hydrothermal treatment, they also provide catalytic activity for SCR reactions. This multi-functionality reduces the need for separate catalytically active materials.

Inventive Principle:
Principle #6Universality (Multi-functionality)

2Quantity of substance

If zeolites are used as catalytically active component, then catalytic activity is improved, but extrusion becomes more difficult and mechanical stability is reduced

Engineering Contradiction:
Improvecatalytic activityVSAvoidextrusion difficulty
Core Design Contradiction:
Quantity of substanceVSEase of manufacture

Solution Approach 1:

The patent creates a composite material system where inorganic binder components (water glass, alumina, silica) are combined with catalytically active zeolite materials. The inorganic binders provide the necessary mechanical strength and extrudability, while the zeolite components provide catalytic activity. The composite structure allows both properties to coexist without compromising either.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent modifies the rheological and mechanical parameters of the catalyst composition by introducing inorganic binder components that improve extrudability and green strength. These binders adjust the flow characteristics of the extrusion mass and provide sufficient mechanical strength during the extrusion process, making manufacturing easier while maintaining high catalytic activity.

Inventive Principle:
Principle #35Parameter changes

3Quantity of substance

If inorganic binder components are catalytically activated through hydrothermal treatment, then catalytic activity is improved, but additional processing steps and time are required

Engineering Contradiction:
Improvecatalytic activityVSAvoidprocessing time
Core Design Contradiction:
Quantity of substanceVSLoss of time

Solution Approach 1:

The patent merges the binder activation process with the catalyst formation process. The inorganic binder components are catalytically activated through hydrothermal treatment at temperatures of 80-200°C over periods of 1-10 days, which simultaneously activates the catalytic activity of the binder and completes the formation of the extruded catalyst body. This combined approach eliminates separate activation steps.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The inorganic binder components are prepared and positioned in the extruded catalyst body before final catalytic activation. The binders are already in place providing mechanical strength during extrusion and drying, and then the catalytic activation is performed as a preliminary treatment before the catalyst enters service. This preliminary action allows the catalyst to be structurally ready before catalytic functionality is fully developed.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process enables the production of an extrudable catalyst with high stability and catalytic activity, ensuring efficient nitrogen oxide reduction in exhaust gases while optimizing the use of zeolitic material.

Implementation Method 1

hydrothermal crystallisation at a temperature of 80 to 200°C, autogenous pressurisation over a reaction time of one to ten days to form crystalline material

Methodology Applied
Scientific EffectHydrothermal crystallization: Crystallisation

Implementation Method 2

ion-exchanging the zeolite with iron or copper to form an ion-exchanged zeolite

Methodology Applied
Scientific EffectIon-exchange: Ion Exchange

Implementation Method 3

extruding a catalyst composition to produce a catalyst body

Methodology Applied
Scientific EffectExtrusion: Extrusion

Implementation Method 4

calcining the crystalline material to form a zeolite, wherein the crystalline material is calcined at a temperature of 400 to 800°C

Methodology Applied
Scientific EffectCalcination: Heat Treatment

Data Source

PatentEP3122457B1Process for producing a catalyst
Publication Date: 2021.11.03 JOHNSON MATTHEY PLC
  • EP3122457B1 patent drawingFigure 1
  • EP3122457B1 patent drawingFigure 2~4

AI summary

To be able to produce an SCR catalyst (2), in particular one having a zeolite fraction (Z) as catalytically active fraction, in a reliable process and at the same time achieve good catalytic activity of the catalyst (2), an inorganic binder fraction (B) which is catalytically inactive in the starting state and has been treated to develop catalytic activity is mixed into a catalyst composition (4). The inorganic binder component for the binder fraction (B) is, in the starting state, preferably porous particles (10), in particular diatomaceous earth, which display mesoporosity. To effect catalytic activation, the individual particles (10) are either coated with a catalytically active layer (12) or transformed into a catalytically active zeolite (14) with maintenance of the mesoporosity.