Surfactant Removal from Mesoporous Zeolites via Composite Extraction

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Solution Overview

Problem

Surfactants, particularly cationic surfactants, strongly adhere to polar solid surfaces and are difficult to remove, necessitating improved methods for effective extraction from polar solids like mesoporous zeolites.

Innovation Solution

A method involving contact with an extraction agent comprising water, salt, and a polar organic compound under specific conditions to solubilize and separate surfactants from the polar solid, reducing surfactant content to a weight ratio of 0.9:1 or less within the solid's pores.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If conventional extraction methods are used to remove surfactants from polar solids, then some surfactant removal is achieved, but the removal efficiency is insufficient due to strong adhesion

Engineering Contradiction:
Improvesurfactant removal amountVSAvoidsurfactant removal efficiency
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

The patent changes the chemical parameters of the extraction agent by combining water, salt, and polar organic compound to create a synergistic extraction system. This parameter change enables effective surfactant removal from polar solids by overcoming the strong adhesion forces through optimized chemical composition and interaction mechanisms.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The extraction agent is formulated as a composite system comprising water, salt, and polar organic compound. This composite approach leverages the complementary properties of each component: water as the base solvent, salt to modulate ionic strength and surfactant-surfactant interactions, and polar organic compound to enhance solubilization of cationic surfactants, achieving superior removal efficiency compared to single-component systems.

Inventive Principle:
Principle #40Composite materials

2Quantity of substance

If strong extraction agents are used to remove surfactants, then surfactant removal improves, but structural damage to the polar solid increases

Engineering Contradiction:
Improvesurfactant removal amountVSAvoidstructural integrity of polar solid
Core Design Contradiction:
Quantity of substanceVSStrength

Solution Approach 1:

The patent optimizes extraction parameters including temperature, contact time, and extraction agent composition to achieve effective surfactant removal while maintaining the structural integrity of the polar solid. By carefully controlling these parameters, the method balances extraction efficiency with preservation of the solid's porous structure and mechanical strength.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The salt component acts as an intermediary that facilitates surfactant removal through ionic interactions without requiring harsh chemicals or extreme conditions. The polar organic compound serves as a mediator that enhances surfactant solubilization through mild solvation effects, thereby achieving effective extraction while protecting the polar solid structure from damage.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Reliability

If multiple extraction steps are used to increase removal efficiency, then surfactant removal improves, but processing time and complexity increase

Engineering Contradiction:
Improvesurfactant removal efficiencyVSAvoidextraction processing time
Core Design Contradiction:
ReliabilityVSLoss of time

Solution Approach 1:

The patent merges multiple extraction functions into a single integrated extraction agent system comprising water, salt, and polar organic compound. This combination achieves the cumulative effect of multiple sequential extraction steps in one operation, significantly reducing processing time while maintaining high surfactant removal efficiency through synergistic interactions among the components.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The optimized composition and parameters of the extraction agent enable a single extraction step to achieve removal efficiency comparable to or exceeding multiple conventional steps. By adjusting the ratios and types of salt and polar organic compound, the method maximizes surfactant extraction kinetics and equilibrium, reducing the number of required processing steps.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Effectively removes a significant portion of surfactants from polar solids, such as mesoporous zeolites, with minimal structural damage and porosity change, allowing for repeated extraction and surfactant recovery.

Implementation Method 1

contacting a surfactant-containing mesoporous zeolite with an initial extraction agent under conditions sufficient to remove at least a portion of a cationic surfactant from the pores of the surfactant-containing mesoporous zeolite wherein the initial extraction agent comprises water, a salt, and a polar organic compound and is capable of at least partially solubilizing the cationic surfactant

Methodology Applied
Scientific EffectSolvation: Solvation

Data Source

PatentUS8765660B1Separation of surfactants from polar solids
Publication Date: 2014.07.01 WR GRACE & CO CONN

AI summary

Methods for removing surfactants from polar solids are described herein. In particular, various embodiments described herein relate to the removal of surfactants from polar solids that involves contacting a surfactant-containing porous polar solid with an extraction agent comprising water, a salt, and, optionally, a polar organic compound. In certain embodiments described herein, the extraction agents are used to remove surfactants from a mesoporous zeolite.