Zinc Oxysulphide CVD Coating Preventing Apparatus Blockage

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Solution Overview

Problem

Existing methods for depositing zinc oxysulphide coatings using dialkyl zinc precursors face challenges with pre-reaction issues, leading to blockage of CVD apparatus and exhaust systems, especially at high substrate temperatures, making it difficult to operate in float glass manufacturing environments.

Innovation Solution

A method involving Atmospheric Pressure Chemical Vapour Deposition using a mixture of dimethyl zinc or diethyl zinc as the zinc source, an episulphide or sulphoxide as the sulphur source, and nitrous oxide or carboxylic esters as the oxygen source, allowing for pre-mixing of precursors without pre-reaction, and controlling the oxygen/sulphur content in the coatings.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If dialkyl zinc precursors are used for depositing zinc oxysulphide coatings, then coating deposition is achieved, but pre-reaction occurs leading to blockage of CVD apparatus and exhaust systems

Engineering Contradiction:
Improvecoating deposition qualityVSAvoidapparatus operational reliability
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The precursor delivery system is segmented into separate channels: one for dialkyl zinc and another for sulphur-containing precursor. This physical separation prevents pre-reaction in the mixing zone while allowing controlled reaction at the substrate surface, resolving the contradiction between achieving coating deposition and preventing apparatus blockage

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

A carrier gas (nitrogen or argon) acts as an intermediary medium to transport the dialkyl zinc and sulphur precursors separately through the CVD chamber. The carrier gas enables precursor delivery without direct contact between precursors until they reach the heated substrate, preventing premature reaction while ensuring coating formation

Inventive Principle:
Principle #24Intermediary (Mediator)

2Reliability

If complex delivery systems with separate precursor lines are used, then pre-reaction is prevented, but device complexity increases

Engineering Contradiction:
Improvepre-reaction preventionVSAvoidprecursor delivery system complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

Multiple precursor delivery functions are merged into a single CVD chamber environment where separate precursor inlets feed into a common reaction zone. The chamber's heated atmosphere and flow dynamics naturally separate and control the precursors until they reach the substrate, reducing external complexity while maintaining pre-reaction prevention

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The CVD chamber serves multiple functions: it acts as the reaction vessel, the heating zone, the precursor mixing chamber (with controlled separation), and the deposition surface. This multi-functionality eliminates the need for separate dedicated delivery systems for each precursor, simplifying the overall apparatus while preventing pre-reaction

Inventive Principle:
Principle #6Universality (Multi-functionality)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables the production of stable and efficient zinc oxysulphide coatings on glass substrates, reducing the need for complex delivery systems and preventing apparatus blockage, while maintaining coating quality and substrate integrity.

Implementation Method 1

The invention relates to a method of forming a coating comprising ZnO (1-x) S x by Atmospheric Pressure Chemical Vapour Deposition

Methodology Applied
Scientific EffectChemical Vapour Deposition: Chemical Vapour Deposition

Implementation Method 2

The glass substrate is heated to a temperature sufficient to cause the reaction

Methodology Applied
Scientific EffectThermal heating: Heating

Data Source

PatentEP3146088B1Deposition of zinc oxysulphide by CVD
Publication Date: 2018.07.25 PILKINGTON GRP LTD
  • EP3146088B1 patent drawingFigure 1
  • EP3146088B1 patent drawingFigure 2
  • EP3146088B1 patent drawing

AI summary

A method of coating a substrate with zinc oxysulphate (ZnO(1-x)Sx, where 0 ≤ x ≤ 1) by atmospheric pressure chemical vapour deposition is disclosed. Various precursors offering sources of zinc, oxygen and sulphur are provided.