Zinc Stannate Layer for Low-E Coating Thermal Stability

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Solution Overview

Problem

Existing low-emissivity (low-E) coatings in window applications face challenges with thermal stability during heat treatment, leading to unpredictable color changes and performance degradation, making it difficult to match heat-treated and non-heat-treated products in terms of color and performance.

Innovation Solution

Incorporating a zinc stannate based layer between silver-based infrared reflecting layers, along with silicon nitride and nickel-chromium oxide layers, to enhance thermal stability and maintain color consistency during heat treatment.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If high temperature heat treatment (at least 580°C, preferably 600-620°C) is applied to low-E coatings, then thermal stability and strength are improved, but coating breakdown and unpredictable color changes occur

Engineering Contradiction:
Improvethermal stabilityVSAvoidcoating integrity
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

A zinc stannate based layer is introduced as an intermediary between the silver-based infrared reflecting layer and the silicon nitride based layer. This intermediate layer acts as a protective buffer that prevents direct harmful interactions between the silver layer and the silicon nitride layer during high temperature heat treatment, thereby maintaining coating integrity while allowing thermal stability to be achieved

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent employs a composite multi-layer structure combining zinc stannate, silicon nitride, and silver-based materials. This composite approach creates a synergistic system where each material contributes specific properties: zinc stannate provides thermal stability and protective characteristics, silicon nitride offers structural support and barrier properties, and silver provides infrared reflection. The composite structure enables the coating to withstand heat treatment temperatures of at least 580°C without breakdown

Inventive Principle:
Principle #40Composite materials

2Strength

If heat treatment is applied to coated glass articles, then tempered glass strength is improved, but color match between heat-treated and non-heat-treated products deteriorates (high ΔE* value)

Engineering Contradiction:
Improveglass strengthVSAvoidcolor matching
Core Design Contradiction:
StrengthVSEase of manufacture

Solution Approach 1:

The zinc stannate based layer serves as a mediator that stabilizes the optical properties of the coating during heat treatment. It prevents excessive color changes by acting as a buffer between the heat treatment process and the silver-based infrared reflecting layer, ensuring that the ΔE* value remains at or below 5.0, and preferably at or below 4.0

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent utilizes controlled parameter changes during heat treatment, specifically maintaining heat treatment temperatures of at least 580°C (preferably 600-620°C) for controlled durations. The zinc stannate layer enables these parameter changes to occur without causing unacceptable color shifts, allowing the coating to achieve thermal stability while maintaining color consistency

Inventive Principle:
Principle #35Parameter changes

3Reliability

If zinc stannate based layer is added between silver layers, then thermal stability upon heat treatment is improved, but device complexity increases

Engineering Contradiction:
Improvethermal stabilityVSAvoidcoating structure
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The zinc stannate based layer performs multiple functions simultaneously: it provides thermal stability during heat treatment, prevents coating breakdown, reduces color changes (keeping ΔE* ≤ 5.0), and maintains the structural integrity of the multi-layer coating. This multi-functionality justifies the added layer by delivering several benefits from a single component

Inventive Principle:
Principle #6Universality (Multi-functionality)

Solution Approach 2:

The zinc stannate layer is strategically positioned in specific locations within the coating structure - between the silicon nitride based layer and the silver-based infrared reflecting layer, and in some embodiments between two silver-based layers. This localized placement optimizes thermal stability where it is most needed while minimizing the overall complexity of the coating structure

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The zinc stannate based layer improves thermal stability, ensuring a low ΔE* value of no greater than 5.0, maintaining color consistency and performance across various heat treatment times, and allowing for the production of heat-treated products that match non-heat-treated versions in terms of color and performance.

Implementation Method 1

a zinc stannate based layer provided over a silver-based infrared (IR) reflecting layer

Methodology Applied
Scientific EffectInfrared reflection: Reflection

Implementation Method 2

the provision of the zinc stannate based layer results in a coated article having improved thermal stability upon heat treatment (HT)

Methodology Applied
Scientific EffectThermal stability: Heat Treatment

Data Source

PatentEP3071530B1Heat treatable coated article with low-e coating having zinc stannate based layer between IR reflecting layers and corresponding method
Publication Date: 2023.07.19 GUARDIAN EURO S A R L
  • EP3071530B1 patent drawingFigure 1
  • EP3071530B1 patent drawingFigure 2
  • EP3071530B1 patent drawingFigure 3

AI summary

A coated article is provided which may be heat treated (e.g., thermally tempered) in certain example instances. In certain example embodiments, the coated article includes a low-emissivity (low-E) coating having a zinc stannate based layer provided over a silver-based infrared (IR) reflecting layer, where the zinc stannate based layer is preferably located between first and second silver based IR reflecting layers. The zinc stannate based layer may be provided between and contacting (i) an upper contact layer of or including Ni and/or Cr (or Ti, or TiOx), and (ii) a layer of or including silicon nitride.