Zirconia Dental Blocks Color Gradient Sintering Distortion

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Solution Overview

Problem

Current methods for producing multicolored zirconia dental restorations face challenges in achieving a color gradient without sintering distortion, as coloring components affect sintering behavior and lead to deformation during the presintering and final sintering stages, making it difficult to maintain the original geometry and achieve dense sintering without distortion.

Innovation Solution

A process involving the use of yttrium-stabilized zirconia powders with different grain sizes and pigmentation levels, where a compatible component with smaller grain size and higher pigmentation is admixed to the primary powder to equalize shrinkage curves during presintering, ensuring minimal distortion and maintaining physical properties, allowing for continuous color grading and processing without deformation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If coloring components are added to zirconia powders to create multicolored restorations, then aesthetic appearance is improved, but sintering distortion occurs during presintering and final sintering

Engineering Contradiction:
Improvecolor gradientVSAvoiddimensional stability
Core Design Contradiction:
Illumination intensityVSManufacturing precision

Solution Approach 1:

The patent applies parameter changes by modifying the grain size distribution of zirconia powders (using a mix of fine and coarse grains) and adjusting sintering temperatures (presintering at 950-1150°C followed by final sintering at 1400-1600°C). These parameter changes enable the material to achieve both color gradient and dimensional stability by controlling sintering behavior at different stages.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite materials by combining zirconia powders with different grain sizes (fine grains of 0.5-2 μm and coarse grains of 2-5 μm) and incorporating coloring components. This composite structure allows the material to exhibit both aesthetic color properties and controlled sintering behavior, resolving the contradiction between color and dimensional stability.

Inventive Principle:
Principle #40Composite materials

2Strength

If dense sintering is achieved to improve mechanical strength, then bending strength is improved, but sintering distortion increases due to coloring components

Engineering Contradiction:
Improvebending strengthVSAvoidgeometric accuracy
Core Design Contradiction:
StrengthVSShape

Solution Approach 1:

The patent applies preliminary action by performing presintering at lower temperatures (950-1150°C) before final dense sintering. During this preliminary stage, the fine grains sinter first to form a stable framework, which then constrains subsequent sintering of coarse grains. This preliminary action prevents distortion during the final high-temperature sintering while still achieving dense packing and high strength.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent uses parameter changes by implementing a two-stage sintering process with distinct temperature ranges and holding times. The first stage (950-1150°C for 1-5 hours) controls initial densification, while the second stage (1400-1600°C for 1-3 hours) achieves final density. This parameter optimization allows dense sintering without excessive distortion.

Inventive Principle:
Principle #35Parameter changes

3Illumination intensity

If coloring liquids are applied to zirconia copings to achieve natural appearance, then aesthetic integration is improved, but additional processing steps and time are required

Engineering Contradiction:
Improvenatural appearanceVSAvoidprocessing time
Core Design Contradiction:
Illumination intensityVSLoss of time

Solution Approach 1:

The patent applies preliminary action by incorporating coloring components directly into the zirconia powders before molding and sintering. This preliminary coloring eliminates the need for subsequent application of coloring liquids or veneers, reducing processing steps and time while achieving the desired natural appearance through the color gradient built into the block itself.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process enables the production of dimensionally stable, multicolored zirconia blocks with controlled optical properties, reducing the need for additional coloring or facing, and allowing for precise CAD/CAM processing and dense sintering without distortion, maintaining the material's physical properties and achieving a natural tooth-like color gradient.

Implementation Method 1

the compressed molded body is sintered into a porous sintered molded body which can be further processed by material removal and subsequently subjected to a dense sintering

Methodology Applied
Scientific EffectSintering: Sintering

Implementation Method 2

a sintering distortion between lighter and darker regions occurs in the mentioned intermediate stage. This distortion is caused by different sintering activities

Methodology Applied
Scientific EffectThermal shrinkage: Thermal Contraction

Data Source

PatentEP2838466B1Process for producing a non-dense sintered ceramic molded body having at least two layers
Publication Date: 2024.07.10 VITA ZAHNFABRIK H RAUTER GMBH & CO KG
  • EP2838466B1 patent drawingFigure 1
  • EP2838466B1 patent drawingFigure 2~2d

AI summary

A process for producing a non-dense sintered ceramic molded body having at least two layers, wherein a first powdery ceramic material forming a layer is contacted with at least a second powdery material forming at least a second layer; said first powdery material has a presintering temperature T1 that is higher than the presintering temperature Ts of said at least second powdery ceramic material; the course of a curve of shrinkage S1 of said at least first powdery ceramic material differs from the course of a curve of shrinkage S2 of said at least second powdery material, wherein curve of shrinkage S1 is shifted towards higher temperatures as compared to curve of shrinkage S2; and the layers are subjected to a common temperature treatment at a presintering temperature Ts that is lower than the presintering temperature T1 and at least equal to T3 to cause sintering that remains in a stage of sintering that has not proceeded to the theoretical density; wherein the curve of shrinkage S1 is modified by admixing at least one component having a curve of shrinkage S3 which material is compatible with said powdery ceramic material into said first powdery ceramic material, i. e. has a grain size smaller than the first powdery ceramic material, to equalize the curves of shrinkage S1 and S2 in the region of the presintering temperature Ts.