Activated Carbon Beads from Microcrystalline Cellulose

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Solution Overview

Problem

Current methods for forming activated carbon from microcrystalline cellulose lack control over porosity and adsorption capacity, leading to inefficient carbonization and activation processes.

Innovation Solution

A method involving carbonizing microcrystalline cellulose and activating the carbonized product, with optional overcoating before or after carbonization, using a process that includes forming cylindrical extrudates, spheronizing, and controlling temperature and atmosphere to achieve high crystallinity and porosity, resulting in activated carbon beads with enhanced adsorption properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional methods are used to form activated carbon from microcrystalline cellulose, then the process is simple, but the porosity and adsorption capacity are poorly controlled

Engineering Contradiction:
Improveporosity controlVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The microcrystalline cellulose is pre-formed into spherical beads with controlled morphology and crystallinity before carbonization. This preliminary structuring ensures that the subsequent carbonization and activation processes produce activated carbon with predictable and controlled porosity, eliminating the need for complex post-processing adjustments

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention controls multiple parameters including cellulose crystallinity (30-70%), bead size (0.1-2.0 mm), carbonization temperature (400-950°C), and activation temperature (800-950°C). By systematically optimizing these parameters, the process achieves precise control over porosity (0.3-0.8 mL/g) and adsorption capacity while maintaining reasonable process complexity

Inventive Principle:
Principle #35Parameter changes

2Reliability

If conventional carbonization and activation methods are used, then the process is straightforward, but the adsorption capacity is insufficient

Engineering Contradiction:
Improveadsorption capacityVSAvoidprocess efficiency
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The invention produces activated carbon with high porosity (0.3-0.8 mL/g) through controlled carbonization and activation of pre-formed microcrystalline cellulose beads. The high crystallinity of the starting material (30-70%) promotes the formation of a developed porous structure during carbonization, which is then enhanced during activation, resulting in superior adsorption capacity

Inventive Principle:
Principle #31Porous materials

Solution Approach 2:

The process creates a composite structure by forming microcrystalline cellulose beads with specific crystallinity and morphology before carbonization. This pre-structured composite approach ensures that the final activated carbon has both high porosity and high adsorption capacity, resolving the trade-off between these two properties

Inventive Principle:
Principle #40Composite materials

3Manufacturing precision

If high porosity is achieved through extended activation, then the adsorption capacity increases, but the processing time increases

Engineering Contradiction:
ImproveporosityVSAvoidprocessing time
Core Design Contradiction:
Manufacturing precisionVSLoss of time

Solution Approach 1:

The microcrystalline cellulose is pre-formed into beads with optimized crystallinity and morphology before carbonization. This preliminary structuring creates a favorable template that accelerates pore formation during carbonization and activation, achieving high porosity (0.3-0.8 mL/g) without requiring extended activation times

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention optimizes the carbonization temperature (400-950°C) and activation temperature (800-950°C) to achieve rapid pore development. By controlling these temperature parameters and the duration of each stage, the process achieves high porosity in a time-efficient manner, avoiding excessive processing times while maintaining excellent adsorption properties

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method produces activated carbon beads with increased porosity and adsorption capacity, allowing for effective filtration and purification, and can be tailored for specific applications by adjusting the overcoating and activation conditions.

Implementation Method 1

carbonizing microcrystalline cellulose to form carbonized microcrystalline cellulose

Methodology Applied
Scientific EffectCarbonization: Pyrolysis

Implementation Method 2

activating the carbonized microcrystalline cellulose to form activated carbon

Methodology Applied
Scientific EffectActivation: Oxidation

Implementation Method 3

removal of constituents from a gas or liquid stream by adsorption

Methodology Applied
Scientific EffectAdsorption: Adsorption

Data Source

PatentEP2231517B1Activated carbon from microcrystalline cellulose
Publication Date: 2020.06.24 PHILIP MORRIS PRODUCTS SA
  • EP2231517B1 patent drawingFigure 1~2

AI summary

A method of forming activated carbon from microcrystalline cellulose comprises converting the microcrystalline cellulose powder into microcrystalline cellulose beads using extrusion and spheronization, carbonizing microcrystalline cellulose to form carbonized microcrystalline cellulose and activating the carbonized microcrystalline cellulose to form activated carbon. The final size of the activated carbon beads, which preferably are of practically spherical shape, can be controlled through the process of making microcrystalline cellulose beads. The invention also encompasses carbon beads having pores therein comprising a majority of the pores less than about 30A and a micropore volume calculated using Density Functional Theory (DFT) in the range of about 0.2cm3/g to 1.0cm3/g for pores in the range of about 5A to 10A. The invention also encompasses a smoking article filter comprising such activated carbon beads, a method for making such a filter and a method for making a smoking article including such a filter.