Arbitrary Waveform Laser Electron Microscope for Nanosecond Imaging

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Solution Overview

Problem

Conventional transmission electron microscopes lack the temporal resolution to capture fast dynamic processes in materials, often missing critical details of nanoscale events due to their low frame rates and inability to capture unique, complex processes in real-time.

Innovation Solution

A high-speed multi-frame dynamic transmission electron microscope image acquisition system with arbitrary timing, utilizing an arbitrary-waveform generation laser and a high-speed deflector subsystem to produce programmable and flexible electron pulses, enabling nanosecond to microsecond-scale image acquisition before, during, and after a sample drive event, allowing for detailed observation of complex material processes.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If conventional TEM uses standard video frame rates for image acquisition, then the system is simple and operates at standard speeds, but the temporal resolution is insufficient to capture fast dynamic processes occurring at nanosecond to microsecond scales

Engineering Contradiction:
Improvetemporal resolutionVSAvoidframe rate
Core Design Contradiction:
Measurement precisionVSProductivity

Solution Approach 1:

The patent employs periodic pulsed electron beams instead of continuous beams, synchronizing electron pulses with the dynamic process being studied. This allows multiple images to be captured at different time points within a single process evolution, achieving nanosecond to microsecond temporal resolution while maintaining system simplicity

Inventive Principle:
Principle #19Periodic action

Solution Approach 2:

The system dynamically adjusts the timing and duration of electron pulses to match the specific temporal characteristics of the material process being studied. By making the electron beam parameters variable and controllable on nanosecond scales, the system achieves high temporal resolution without requiring complete system redesign

Inventive Principle:
Principle #15Dynamics

2Measurement precision

If conventional TEM uses continuous electron beams with small apertures to achieve desired beam parameters, then spatial resolution is maintained, but the frame rate remains limited to standard video rates

Engineering Contradiction:
Improvespatial resolutionVSAvoidacquisition time
Core Design Contradiction:
Measurement precisionVSLoss of time

Solution Approach 1:

Instead of using continuous electron beams, the system employs periodic pulsed electron beams where electrons are emitted in synchronized bursts. This allows the beam to be concentrated into short pulses that can capture rapid temporal changes while maintaining spatial coherence through controlled pulse duration and synchronization with the imaging process

Inventive Principle:
Principle #19Periodic action

Solution Approach 2:

The system changes the temporal parameters of the electron beam by introducing pulsed operation with variable pulse widths from nanoseconds to microseconds. This parameter change enables the beam to resolve fast dynamic processes while maintaining spatial resolution through controlled pulse characteristics and synchronization

Inventive Principle:
Principle #35Parameter changes

3Measurement precision

If conventional TEM starts and stops processes to capture dynamic behavior, then some temporal information can be obtained, but the process cannot be observed in real-time and precision is poor

Engineering Contradiction:
Improvetemporal precisionVSAvoidprocess control
Core Design Contradiction:
Measurement precisionVSEase of operation

Solution Approach 1:

The system uses periodic pulsed electron beams that are synchronized with the material process evolution, allowing real-time observation without interrupting the process. The pulsed timing can be adjusted to capture specific moments in the process evolution, providing both temporal precision and ease of operation

Inventive Principle:
Principle #19Periodic action

Solution Approach 2:

The system prepares the electron beam pulsing sequence in advance to match the expected process timeline, allowing precise capture of dynamic events without needing to interrupt or control the material process itself. This preliminary timing setup provides both temporal precision and operational simplicity

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Enables the capture of high-resolution images of fast, complex material processes and events, such as phase transformations and chemical reactions, with improved spatial and temporal resolution, allowing for more detailed analysis and understanding of material properties and behavior.

Implementation Method 1

The high current is typically achieved through photoemission, driven by a pulsed laser (e.g. ultraviolet laser) directed upon a metal cathode

Methodology Applied
Scientific EffectPhotoemission: Photoelectric Effect

Implementation Method 2

Electrons emitted by a source, usually at the top of the microscope, are typically focused by magnetic lenses into a narrow beam

Methodology Applied
Scientific EffectMagnetic lens focusing: Electromagnet

Implementation Method 3

a high-speed deflector subsystem arranged for synchronous operation with the laser system and capable of bidirectional, two-dimensional image shifting on the nanosecond scale

Methodology Applied
Scientific EffectElectrostatic deflection: Electrostatic Induction

Data Source

PatentEP2997591B1High-speed multi-frame dynamic transmission electron microscope image acquisition system with arbitrary timing
Publication Date: 2019.12.11 LAWRENCE LIVERMORE NAT SECURITY LLC
  • EP2997591B1 patent drawingFigure 1
  • EP2997591B1 patent drawingFigure 2~3
  • EP2997591B1 patent drawingFigure 4A

AI summary

An electron microscope is disclosed which has a laser-driven photocathode and an arbitrary waveform generator (AWG) laser system ("laser"). The laser produces a train of temporally-shaped laser pulses each being of a programmable pulse duration, and directs the laser pulses to the laser-driven photocathode to produce a train of electron pulses. An image sensor is used along with a deflector subsystem. The deflector subsystem is arranged downstream of the target but upstream of the image sensor, and has a plurality of plates. A control system having a digital sequencer controls the laser and a plurality of switching components, synchronized with the laser, to independently control excitation of each one of the deflector plates. This allows each electron pulse to be directed to a different portion of the image sensor, as well as to enable programmable pulse durations and programmable inter-pulse spacings.