Autoclave Metal Powder Dissolution for High-Purity Sulfate Solutions

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Solution Overview

Problem

Existing methods for producing metal sulphates such as nickel sulphate are impractically slow, unsafe, and inefficient, often requiring aggressive oxidizing agents, oxygen or nitrogen gases, and are not scalable for commercial operations.

Innovation Solution

A process involving the reaction of an aqueous slurry of metal powder with sulphuric acid in an autoclave reactor at controlled temperatures (100°C to 250°C) with a molar ratio below 1.0, followed by separation of the metal sulphate solution from residual powder, operates under reducing conditions without oxygen, and allows for continuous or batch processing.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If elemental nickel is dissolved in sulfuric acid at room temperature, then the process is safe, but the reaction rate is impractically slow

Engineering Contradiction:
Improveprocess safetyVSAvoidreaction rate
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent applies parameter changes by increasing the temperature from room temperature to 100-250°C and adjusting the molar ratio of sulfuric acid to metal to below 1.0, thereby achieving both rapid dissolution and process safety through controlled parameter optimization

Inventive Principle:
Principle #35Parameter changes

2Productivity

If the pH is lowered to increase reaction rate, then the dissolution speed improves, but the final product pH becomes too low for battery applications

Engineering Contradiction:
Improvedissolution speedVSAvoidproduct pH control
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent applies preliminary action by conducting the dissolution at elevated temperature (100-250°C) with controlled acid-to-metal ratio below 1.0, which pre-optimizes the reaction conditions to achieve both high dissolution rate and appropriate final pH (3.5-5.0) suitable for battery applications without requiring additional pH adjustment steps

Inventive Principle:
Principle #10Preliminary action

3Productivity

If oxidizing agents are added to accelerate dissolution, then the reaction rate increases, but the process complexity and safety requirements increase

Engineering Contradiction:
Improvereaction rateVSAvoidprocess complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent applies the taking out principle by removing oxidizing agents from the process entirely, achieving rapid dissolution through thermal energy input (100-250°C) and optimized acid-to-metal ratio instead, thereby simplifying the process and eliminating safety concerns associated with oxidizing agents

Inventive Principle:
Principle #2Taking out (Extraction)

4Device complexity

If atmospheric pressure is used for dissolution, then the equipment complexity is reduced, but hydrogen gas accumulation creates safety hazards

Engineering Contradiction:
Improveequipment complexityVSAvoidhydrogen gas hazard
Core Design Contradiction:
Device complexityVSObject-affected harmful factors

Solution Approach 1:

The patent applies parameter changes by operating at elevated temperatures (100-250°C) which increase the solubility of hydrogen gas in the aqueous solution and accelerate its evolution, allowing safe hydrogen management through temperature control rather than complex pressure management systems

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process ensures safe, efficient, and scalable production of high-purity metal sulphate solutions with minimal reagent use, high circuit utilization, and flexibility in operation modes, promoting rapid dissolution and high nickel sulphate concentrations.

Implementation Method 1

reacting an aqueous slurry of metal powder with sulfuric acid in an autoclave reactor at a temperature between 100°C and 250°C

Methodology Applied
Scientific EffectHeating: Heating

Implementation Method 2

reacting an aqueous slurry of metal powder with sulfuric acid in an autoclave reactor at a temperature between 100°C and 250°C

Methodology Applied
Scientific EffectPressurisation: Pressurisation

Implementation Method 3

reacting an aqueous slurry of metal powder with sulfuric acid... thereby forming a metal sulphate solution

Methodology Applied
Scientific EffectChemical reaction: Chemical Bonding

Data Source

PatentEP4711338A1Controlled autoclave dissolution of metal powders for producing high-purity metal sulfate solutions
Publication Date: 2026.03.18 UMICORE(BE)
  • EP4711338A1 patent drawingFigure 1~3
  • EP4711338A1 patent drawingFigure 4
  • EP4711338A1 patent drawingFigure 5

AI summary

The present invention provides a controlled autoclave dissolution of metal powders for producing high-purity metal sulphate solutions, comprising the steps of: a. reacting an aqueous slurry comprising a metal powder with sulphuric acid in an autoclave section comprising one or more autoclave reactors at a temperature between 100°C and 250°C, thereby forming a metal sulphate solution having a residual amount of metal powder, whereby the molar ratio of sulphuric acid and metal in said autoclave section is lower than 1.0; and b. separating said metal sulphate solution from said residual metal powder.