Biofuel Feed Pre-treatment via High-Pressure Hydrolysis

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Solution Overview

Problem

Current pre-treatment processes for secondary raw materials in biofuel production, such as frying oils and animal fats, are inadequate in removing impurities like phosphate-containing compounds, chlorides, calcium, magnesium ions, and heavy metals, which are detrimental to hydrotreating catalysts, and result in excessive production of by-products like propane during hydrotreating and isomerization processes.

Innovation Solution

A pre-treatment process involving high-temperature and high-pressure hydrolysis of the feed with a recycling stream of purified mono-, di-, and triglycerides, converting triglycerides into fatty acids and removing impurities, followed by separation and recycling of glycerol for further processing, effectively reducing impurities and minimizing by-product formation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional pre-treatment processes (acid washing, ion exchange resins, percolation) are used to remove impurities, then some impurity removal is achieved, but the impurity levels are not reduced to optimal levels required for hydrotreating, and catalyst poising occurs

Engineering Contradiction:
Improveimpurity removal efficiencyVSAvoidcatalyst performance
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The invention changes the fundamental parameters of the pre-treatment process by using high-temperature (100-200°C) and high-pressure (10-50 bar) hydrolysis conditions instead of conventional ambient temperature acid washing or ion exchange methods. This parameter change enables complete hydrolysis of phospholipids and removal of all detrimental impurities (phosphorus, chlorides, calcium, magnesium, heavy metals) to levels below 10 ppm, ensuring catalyst protection and optimal hydrotreating performance

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention extracts and removes all detrimental impurities from the feedstock through high-temperature high-pressure hydrolysis. The process selectively extracts phospholipids, proteins, and other impurity compounds that would otherwise poison the catalyst, separating them from the triglyceride feedstock before hydrotreating. This complete extraction ensures that only pure triglycerides enter the hydrotreating reactor, protecting catalyst activity

Inventive Principle:
Principle #2Taking out (Extraction)

2Manufacturing precision

If conventional pre-treatment processes are used, then some purification is achieved, but excessive by-products (propane) are produced during hydrotreating and isomerization

Engineering Contradiction:
Improvefeed purification levelVSAvoidby-product formation
Core Design Contradiction:
Manufacturing precisionVSObject-generated harmful factors

Solution Approach 1:

The invention performs preliminary hydrolysis action before hydrotreating to completely convert phospholipids and other impurities into water-soluble compounds that are removed in the aqueous phase. This preliminary action ensures that only pure triglycerides enter the hydrotreating reactor, preventing the formation of excessive by-products like propane during subsequent hydrotreating and isomerization reactions

Inventive Principle:
Principle #10Preliminary action

3Manufacturing precision

If high-temperature high-pressure hydrolysis is used, then complete impurity removal is achieved, but energy consumption increases

Engineering Contradiction:
Improveimpurity removal completenessVSAvoidhydrolysis process energy
Core Design Contradiction:
Manufacturing precisionVSUse of energy by moving object

Solution Approach 1:

The invention implements continuous hydrolysis and separation operation where the high-temperature high-pressure hydrolysis is continuously applied to the feedstock, and the aqueous phase containing impurities is continuously removed. This continuous operation ensures complete impurity removal while maintaining optimal energy efficiency by avoiding repeated heating cycles and maintaining steady-state reaction conditions

Inventive Principle:
Principle #20Continuity of useful action

Solution Approach 2:

The invention optimizes the energy consumption by carefully controlling the hydrolysis parameters (temperature 100-200°C, pressure 10-50 bar) to achieve complete impurity removal with minimal energy input. The parameter changes are designed to be just sufficient for complete hydrolysis, avoiding excessive energy consumption while ensuring 100% removal of phospholipids and other impurities

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process achieves significant reduction of impurities below the limits tolerated by hydrotreated vegetable oil processes, minimizing propane production and optimizing the yield of valuable biofuels by ensuring a cleaner feed stream for subsequent hydrotreating and isomerization steps.

Implementation Method 1

an hydrolysis process is carried out to an incoming feed consisting of the raw material added to a recycling stream... partially or totally producing fatty acids

Methodology Applied
Scientific EffectHydrolysis: Hydrolysis

Implementation Method 2

The hydrolysis is carried out at a temperature between 150 to 260°C and at a pressure between 10 to 60 barg

Methodology Applied
Scientific EffectThermal energy: Heating

Data Source

PatentEP4004161B1Process for the pre-treatment of feeds for the production of biofuels by hydrolysis of fats at high temperature and pressure
Publication Date: 2024.11.06 KT TECH SPA IT
  • EP4004161B1 patent drawingFigure 1
  • EP4004161B1 patent drawingFigure 2
  • EP4004161B1 patent drawing

AI summary

A hydrotreating and isomerization pre- treatment process in a biofuel production plant, which is characterized in that it occurs from a raw supply consisting of an organic feed comprising secondary materials such as frying oils, category 1 animal fats, residual oils or by-products consisting of monoglycerides, diglycerides, triglycerides and free fatty acids, which is added to a recycling stream consisting of a mixture of mono-, di - and triglycerides free of impurities and exiting an esterification unit, said process occurring by means of hydrolysis with excess water, under controlled pressure and temperature conditions, thus obtaining the partial or total conversion of the supply into glycerol and fatty acids, the excess water introduced into the hydrolysis process acting as a solvent for impurities of various nature present in ionic form, thus removing most of the heavy metals, as well as of the chlorides present in said supply.