Boron Phosphate Matrix Layer for Fuel Cells

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Solution Overview

Problem

Phosphoric acid fuel cells face performance degradation due to reactions between the electrolyte and matrix materials, and previous matrix layers like silicon carbide suffer from oxide dissolution, leading to acid loss and blockages.

Innovation Solution

A porous matrix layer comprising at least 90% boron phosphate is used between the electrodes, with phosphoric acid as the electrolyte, providing chemical stability and preventing reactant mixing, while allowing for a thin layer to minimize IR losses and enhance fuel cell efficiency.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If phenolic resin matrix layer is used, then the matrix provides structural support, but the organic material reacts with phosphoric acid at elevated temperatures producing catalyst-poisoning molecules

Engineering Contradiction:
Improvestructural supportVSAvoidcatalyst poisoning
Core Design Contradiction:
StrengthVSObject-generated harmful factors

Solution Approach 1:

The patent changes the chemical composition parameter of the matrix layer from organic phenolic resin to inorganic boron phosphate, which does not react with phosphoric acid to produce harmful substances, thereby eliminating catalyst poisoning while maintaining structural support

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses a composite structure combining boron phosphate particles with a binder material, creating a composite matrix layer that provides both structural integrity and chemical stability against phosphoric acid

Inventive Principle:
Principle #40Composite materials

2Stability of the object's composition

If silicon carbide matrix layer is used, then the matrix provides chemical stability, but the oxide on silicon carbide dissolves slowly during operation converting to insoluble silicon phosphate

Engineering Contradiction:
Improvechemical stabilityVSAvoidphosphoric acid electrolyte loss
Core Design Contradiction:
Stability of the object's compositionVSLoss of substance

Solution Approach 1:

The patent changes the matrix material from silicon carbide to boron phosphate, which has superior chemical stability and does not undergo dissolution or conversion reactions with phosphoric acid, thereby preventing electrolyte loss

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent selects boron phosphate as a more stable material that prevents the short-term dissolution issues experienced with silicon carbide, effectively creating a long-lasting matrix layer

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Strength

If silicon carbide matrix layer is used, then the matrix provides structural integrity, but insoluble silicon phosphate blocks fuel or oxidant gas delivery to electrodes

Engineering Contradiction:
Improvestructural integrityVSAvoidgas delivery blockage
Core Design Contradiction:
StrengthVSObject-generated harmful factors

Solution Approach 1:

The patent changes the matrix material composition to boron phosphate, which does not form insoluble phosphate deposits, thereby preventing blockage of gas delivery channels while maintaining structural integrity

Inventive Principle:
Principle #35Parameter changes

4Reliability

If thicker matrix layer is used, then electrolyte retention is improved, but IR losses increase reducing fuel cell efficiency

Engineering Contradiction:
Improveelectrolyte retentionVSAvoidIR losses
Core Design Contradiction:
ReliabilityVSLoss of energy

Solution Approach 1:

The patent uses a porous structure of boron phosphate particles that provides high electrolyte retention through capillary action while maintaining thin layer thickness, thereby minimizing IR losses

Inventive Principle:
Principle #31Porous materials

Solution Approach 2:

The composite structure of boron phosphate particles with appropriate pore distribution enables both good electrolyte retention and low resistance by optimizing the balance between density and porosity

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The boron phosphate matrix layer maintains electrolyte retention, reduces IR losses, and increases fuel cell efficiency and lifetime, while lowering platinum loadings and costs.

Implementation Method 1

The porous matrix layer comprises pores and solids. The solids of the matrix layer comprise at least 90% by mass boron phosphate. A phosphoric acid electrolyte is within the pores of the matrix layer

Methodology Applied
Scientific EffectCapillary action: Capillary Action

Implementation Method 2

providing chemical stability and preventing reactant mixing

Methodology Applied
Scientific EffectPhysical separation: Physical Containment

Data Source

PatentEP3504745B1Boron phosphate matrix layer
Publication Date: 2021.12.01 DOOSAN FUEL CELL AMERICA INC
  • EP3504745B1 patent drawingFigure 1~2

AI summary

An illustrative example embodiment of a fuel cell includes a cathode electrode, an anode electrode, and a porous matrix layer between the electrodes. The porous matrix layer includes pores and solids. The solids comprises at least 90% boron phosphate. A phosphoric acid electrolyte is within the pores of the matrix layer.