Carboxyl-Functionalized Adsorbent for Amine Isolation

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Solution Overview

Problem

Current methods for purifying amines from aqueous solutions, particularly from diluted solutions, are inefficient and require high energy, multiple solvents, and additional purification steps.

Innovation Solution

A method involving the use of an adsorbent functionalized with carboxyl groups to adsorb amines from aqueous solutions, followed by water removal and thermal desorption to obtain the amine in pure form.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If distillation methods are used to purify amines from aqueous solutions, then purification can be achieved, but high energy demand and complex additional purification steps are required

Engineering Contradiction:
Improvepurity of amineVSAvoidenergy demand
Core Design Contradiction:
Manufacturing precisionVSUse of energy by moving object

Solution Approach 1:

An adsorbent material functionalized with carboxyl groups serves as an intermediary substance that selectively binds amines from aqueous solutions. The adsorbent captures amines through acid-base interactions, allowing separation without energy-intensive distillation. After adsorption, the adsorbent can be regenerated by simple heating to release concentrated amine, eliminating the need for complex purification steps while reducing energy consumption.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The invention changes the separation parameter from thermal-based (distillation requiring high energy) to chemical-based (adsorption through carboxyl group interactions). By modifying the adsorbent with carboxyl functional groups, the system exploits chemical affinity differences to achieve selective amine capture at lower temperatures, then releases amines through controlled thermal desorption, significantly reducing overall energy demand while maintaining high purity.

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If multiple solvents and additional purification steps are used, then high purity amine can be obtained, but the process complexity and solvent usage increase

Engineering Contradiction:
Improvepurity of amineVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The carboxyl-functionalized adsorbent acts as a selective intermediary that captures amines from aqueous solutions through specific acid-base interactions. This single-step adsorption process replaces multiple purification steps and solvent systems. The adsorbent can be easily regenerated by heating, providing a simple two-step process (adsorption followed by thermal desorption) that achieves high purity without complex equipment or multiple solvents.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The invention extracts amines from aqueous solutions using a solid adsorbent phase, separating the amine component directly from the aqueous matrix. This extraction approach using carboxyl-functionalized materials selectively removes amines in one step, eliminating the need for multiple liquid-liquid extraction steps or complex chromatographic purifications, thereby simplifying the overall process while maintaining high purity.

Inventive Principle:
Principle #2Taking out (Extraction)

3Quantity of substance

If conventional purification methods are used for diluted amine solutions, then amine can be recovered, but the economic efficiency decreases due to high energy and solvent costs

Engineering Contradiction:
Improveyield of amineVSAvoideconomic efficiency
Core Design Contradiction:
Quantity of substanceVSEase of manufacture

Solution Approach 1:

The carboxyl-functionalized adsorbent serves as an economical intermediary that efficiently captures amines from diluted solutions. The adsorbent can be regenerated and reused multiple times through simple heating, reducing both solvent consumption and energy costs compared to conventional methods. This reusable adsorption-desorption cycle provides high amine recovery yields while significantly improving economic efficiency by eliminating the need for expensive solvents and energy-intensive continuous purification.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The invention changes the recovery parameter from thermal separation (distillation requiring high energy input proportional to solution volume) to chemical adsorption (which is effective even for diluted solutions). The carboxyl groups provide selective binding that works efficiently at low amine concentrations, enabling economical recovery from diluted streams without the prohibitive energy costs of conventional thermal methods, thereby improving both yield and economic efficiency.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method provides economical access to high-purity amines with lower energy demand, reduced solvent usage, and higher yield, while eliminating the need for additional solvent separation steps.

Implementation Method 1

contacting the aqueous solution of the amine with an adsorbent functionalized with carboxyl groups

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 2

removing water from the adsorbent

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 3

thermally desorbing the amine

Methodology Applied
Scientific EffectThermal desorption: Desorption

Data Source

PatentEP4326705B1Process for the isolation of amines
Publication Date: 2025.05.28 GIVAUDAN SA
  • EP4326705B1 patent drawingFigure 1a~1b
  • EP4326705B1 patent drawingFigure 2
  • EP4326705B1 patent drawing

AI summary

There is provided a method for the isolation of an amine from an aqueous solution thereof, comprising the steps of: a) contacting the aqueous solution of the amine with an adsorbent functionalized with carboxyl groups; b) removing water from the adsorbent; and c) thermally desorbing the amine. The method is particularly suitable for the isolation of ethanolamine.