Microbial Carbonate Precipitation Using ChaA Bacteria for CO2 Sequestration

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Solution Overview

Problem

Current CO2 sequestration methods, such as microbial induced carbonate precipitation using ureolysis, face challenges like malodor issues, limited distribution of ureolytic species, and viability under extreme conditions, while other methods like burial require high-quality CO2 and high temperatures/pressures, making them inefficient for large-scale CO2 storage.

Innovation Solution

A method involving a liquid calcification medium with yeast extract, specific carbon sources like calcium carboxylic acids, and bacteria expressing the chaA gene to induce microbial carbonate precipitation, allowing CO2 sequestration through microbial induced carbonate precipitation (MICP) without relying on urea, thereby overcoming previous limitations.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If ureolysis is used for microbial induced carbonate precipitation, then CO2 sequestration can be achieved, but malodor issues and limited distribution of ureolytic species occur

Engineering Contradiction:
ImproveCO2 sequestrationVSAvoidmalodor
Core Design Contradiction:
Quantity of substanceVSObject-generated harmful factors

Solution Approach 1:

The invention changes the chemical parameters of the system by replacing urea with alternative carbon sources (acetate, propionate, butyrate) and nitrogen sources (ammonium salts, nitrate, nitrite). This parameter change eliminates the malodor associated with urea decomposition while maintaining the ability to drive carbonate precipitation through pH elevation via ammonia production from the alternative nitrogen sources.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention uses readily available, inexpensive materials such as table salt (NaCl) as a nitrogen source and common organic acids (acetate, propionate, butyrate) as carbon sources. These replace the need for specialized ureolytic bacteria and urea, making the system more accessible and eliminating odor problems while achieving the same CO2 sequestration goal.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

2Ease of manufacture

If burial method is used for CO2 sequestration, then simplicity and cost are improved, but CO2 escape risk and inefficient CO2 conversion occur

Engineering Contradiction:
Improvesimplicity and costVSAvoidCO2 escape risk
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The invention replaces the mechanical burial approach with a bio-chemical system where microorganisms actively convert CO2 into solid carbonate minerals through metabolic processes. This substitution transforms CO2 from a gas that could escape into stable solid carbonates, eliminating the leakage risk while maintaining simplicity and low cost through the use of natural biological processes.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The invention utilizes phase transition by converting gaseous CO2 into solid calcium carbonate minerals through microbially induced carbonate precipitation. This phase change from gas to solid ensures permanent sequestration without the risk of escape that plagues burial methods, while the process remains simple and cost-effective.

Inventive Principle:
Principle #36Phase transitions

3Ease of operation

If burial method is used for CO2 sequestration, then simplicity is improved, but inefficient CO2 conversion to stable carbonates occurs

Engineering Contradiction:
ImprovesimplicityVSAvoidCO2 conversion efficiency
Core Design Contradiction:
Ease of operationVSProductivity

Solution Approach 1:

The invention employs self-service by utilizing the natural metabolic capabilities of microorganisms to convert CO2 into stable carbonates. The system requires minimal external intervention beyond providing the appropriate chemical environment (pH, nutrients), allowing the biological system to perform the conversion automatically. This maintains simplicity while dramatically improving conversion efficiency compared to passive burial methods.

Inventive Principle:
Principle #25Self-service

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method effectively sequesters CO2 by forming precipitated calcium carbonates, which can be recovered and used industrially, offering a scalable and environmentally friendly alternative with net-negative CO2 release, addressing the inefficiencies of existing methods.

Implementation Method 1

allowing microbial induced carbonate precipitation of calcium carbonate, thereby sequestering at least some of the CO2 introduced in said step of introducing

Methodology Applied
Scientific EffectMicrobial induced carbonate precipitation:

Implementation Method 2

creation of precipitated calcium carbonates through a microbially induced carbonate precipitation

Methodology Applied
Scientific EffectPrecipitation: Precipitation

Data Source

PatentUS12043858B2CO<sub>2 </sub>sequestration and creation of calcium carbonates through microbial induced carbonate precipitation
Publication Date: 2024.07.23 THE UNIVERSITY OF AKRON

AI summary

A method for sequestering CO2 and creating precipitated calcium carbonates includes: (a) providing a liquid calcification medium including: a nutrient broth including water and a yeast extract, a carbon source selected from calcium carboxylic acids and calcium dicarboxylic acids and mixtures thereof, and bacteria that naturally express the chaA gene; (b) introducing CO2 to the liquid calcification medium; and (c) allowing microbial induced carbonate precipitation of calcium carbonate, thereby sequestering at least some of the CO2 introduced in the step of introducing.