Chromium Silica Catalyst Calcination via Fluidized Gas Flow

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Solution Overview

Problem

Current methods for producing polymerization catalysts face challenges in enhancing catalyst performance, leading to increased production costs and inefficient process economics.

Innovation Solution

A method involving calcining a catalyst precursor comprising chromium and silica at temperatures between 95°C to 400°C, with controlled gas flow rates and space velocities, to produce high melt index (MI) catalysts (HMCs) with optimized silica-support characteristics and titanium and chromium compositions.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional catalyst preparation methods are used, then production costs are reduced, but catalyst performance and melt index potential are limited

Engineering Contradiction:
Improvecatalyst performanceVSAvoidproduction cost
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The patent applies parameter changes by precisely controlling calcination temperature (95-400°C range) and gas flow rates (2.5-30 times settled volume per minute) to optimize catalyst performance. These parameter optimizations enable improved melt index potential and polymerization efficiency while maintaining cost-effective production through controlled atmospheric conditions during calcination

Inventive Principle:
Principle #35Parameter changes

2Reliability

If calcination is performed at higher temperatures to improve catalyst activation, then catalyst activity increases, but energy consumption and production costs increase

Engineering Contradiction:
Improvecatalyst activityVSAvoidenergy consumption
Core Design Contradiction:
ReliabilityVSUse of energy by moving object

Solution Approach 1:

The patent resolves this contradiction by changing the temperature parameter to a lower range (95-400°C) combined with optimized gas flow rates (2.5-30 times settled volume per minute). This parameter combination achieves sufficient catalyst activation and activity while significantly reducing energy consumption compared to conventional high-temperature calcination methods

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs pneumatic principles by using controlled gas flow through the catalyst bed during calcination. The gas flow rate (2.5-30 times settled volume per minute) creates fluidization and enhances heat and mass transfer, allowing effective catalyst activation at lower temperatures and reducing overall energy requirements

Inventive Principle:
Principle #29Pneumatics and hydraulics

3Manufacturing precision

If gas flow rate is increased to improve heat and mass transfer during calcination, then catalyst uniformity improves, but equipment complexity and operational difficulty increase

Engineering Contradiction:
Improvecatalyst uniformityVSAvoidequipment complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent achieves catalyst uniformity by optimizing the gas flow rate parameter to 2.5-30 times the settled volume per minute. This parameter range creates effective fluidization and uniform heat distribution throughout the catalyst bed, ensuring consistent catalyst properties without requiring complex equipment modifications or control systems

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach results in catalysts with improved high melt index potential, enhancing polymerization efficiency and reducing production costs by optimizing catalyst performance.

Implementation Method 1

calcining a catalyst precursor comprising chromium and a silica support material at a temperature in the range of from about 95° C. to about 400° C. in a bed fluidized by a gas flowing at a volumetric flow rate from about 2.5 to about 30 times the settled volume of the bed per minute

Methodology Applied
Scientific EffectFluidization: Fluidisation

Implementation Method 2

calcining a catalyst precursor comprising chromium and silica at temperatures between 95°C to 400°C

Methodology Applied
Scientific EffectHeating: Heating

Data Source

PatentUS10287369B2Methods of preparing a catalyst
Publication Date: 2019.05.14 CHEVRON PHILLIPS CHEMICAL COMPANY LP

AI summary

A method comprising calcining a catalyst precursor comprising chromium and a silica support material at a temperature in the range of from about 95° C. to about 400° C. in a bed fluidized by a gas flowing at a volumetric flow rate of from about 2.5 to about 30 times the settled volume of the bed per minute to form a calcined catalyst precursor. A method comprising calcining a catalyst precursor comprising chromium and silica at a temperature in the range of from about 95° C. to about 400° C. with a gas flowing through the bed at a gas hourly space velocity of from about 15 to about 200 per hour. A method comprising calcining a catalyst precursor comprising chromium and silica at a temperature in the range of from about 95° C. to about 400° C. with a gas flowing through the bed at a weight hourly space velocity of from about 1.9 to about 240 per hour.