Copper Silicide Fluidization Additive for Agglomeration

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Solution Overview

Problem

Copper silicide particles exhibit cohesive behavior at high temperatures, leading to nonuniform fluidized bed conditions and agglomeration in fluidized bed reactors, which hinders the efficient production of halosilanes.

Innovation Solution

A method involving heating a mixture of greater than 80% copper silicide particles and up to 20% fluidization additive particles, such as silica or silicon carbide, at temperatures of at least 400°C, while feeding a fluid at a sufficient velocity to maintain uniform fluidization, preventing agglomeration and ensuring a bubbling bed state.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If copper silicide particles are heated to high temperatures (at least 400°C) in a fluidized bed reactor, then the production efficiency of halosilanes is improved, but the particles exhibit cohesive behavior leading to agglomeration and nonuniform fluidization

Engineering Contradiction:
Improveproduction efficiency of halosilanesVSAvoiduniformity of fluidized bed
Core Design Contradiction:
ProductivityVSStability of the object's composition

Solution Approach 1:

An intermediary substance (fluidization additive such as silica, silicon carbide, or fumed silica) is introduced to mediate between the copper silicide particles. This additive prevents direct cohesive interactions between copper silicide particles at high temperatures, maintaining fluidization uniformity while allowing high-temperature operation for efficient halosilane production.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The physical and chemical parameters of the particle mixture are changed by adding fluidization additives with specific properties (particle size, surface area, thermal stability). These parameter changes modify the overall behavior of the particle bed, preventing agglomeration and maintaining uniform fluidization at elevated temperatures required for high productivity.

Inventive Principle:
Principle #35Parameter changes

2Quantity of substance

If copper silicide particles are fluidized at high temperatures, then the contact between particles and fluidization gas is enhanced, but agglomeration occurs leading to channeling and nonuniform fluidization

Engineering Contradiction:
Improvecontact between particles and fluidization gasVSAvoidagglomeration and channeling
Core Design Contradiction:
Quantity of substanceVSObject-generated harmful factors

Solution Approach 1:

The fluidization additive acts as a protective intermediary layer between copper silicide particles, preventing them from adhering to each other during high-temperature fluidization. This intermediary substance maintains particle separation, ensuring continuous contact with fluidization gas while preventing the formation of agglomerates and channels.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The harmful cohesive behavior of copper silicide particles at high temperatures is converted into a beneficial situation by introducing fluidization additives. These additives exploit their own physical properties (such as surface area and thermal stability) to prevent agglomeration, transforming the high-temperature environment from a source of harm into a condition that enables enhanced gas-solid contact for improved reaction efficiency.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method effectively maintains a uniformly fluidized bed at high temperatures, preventing agglomeration and channeling, thus ensuring consistent and efficient fluidization for halosilane production.

Implementation Method 1

A fluidized bed apparatus comprises a fluidized bed comprising solid particles and a fluidization gas or vapor. The fluidized bed is a fluid-solid heterogeneous mixture that exhibits fluid-like properties. In fluidized beds, the contact of the solid particles with the fluidization gas or vapor is greatly enhanced

Methodology Applied
Scientific EffectFluidization: Fluidisation

Implementation Method 2

heating, at a temperature of at least 400°C, a mixture of particles comprising greater than 80% to less than 100% copper silicide particles and greater than 0 to 20% fluidization additive particles

Methodology Applied
Scientific EffectHeating: Heating

Data Source

PatentEP3274296B1Method for fluidizing copper silicide and process for preparing a halosilane using the method
Publication Date: 2020.02.19 DOW SILICONES CORP

AI summary

A method is useful for maintaining a uniformly fluidized bed in a fluidized bed apparatus. The method includes the steps of charging a mixture of particles including copper silicide particles and fluidization additive particles into the fluidized bed apparatus, and uniformly fluidizing the particles at a temperature of at least 400 °C in the fluidized bed apparatus.