Covalently Linked Emulsion Material for Stable Aqueous Gels

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Solution Overview

Problem

Existing water-based gels with a three-dimensional network formed by non-covalent interactions are relatively fluid, fail to maintain shape, and disintegrate quickly in aqueous phases, limiting their applications due to high dispersed phase proportions and instability in physiological fluids.

Innovation Solution

A water-based material with a continuous aqueous phase and covalently linked droplets, comprising a phospholipid, solubilizing lipid, co-surfactant, and surfactant of specific formula (I), which maintains shape and resists dilution, ensuring stability and cohesion through covalent bonds.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of operation

If non-covalent interactions are used to form the three-dimensional network, then the gel is relatively fluid and easy to shape, but it does not maintain its form and disintegrates rapidly in aqueous phases

Engineering Contradiction:
Improveease of shapingVSAvoidstability in aqueous phase
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The patent changes the bonding parameter from non-covalent to covalent interactions between droplets, transforming the gel's fundamental structure. This covalent bonding provides stable, irreversible connections that maintain the gel's three-dimensional network and shape in aqueous environments, resolving the contradiction between ease of shaping and stability.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention creates a composite structure where droplets are covalently bonded to form a hybrid material combining liquid crystalline phases with polymeric networks. This composite approach integrates the fluidity of liquid crystals with the structural stability of covalently bonded polymers, achieving both ease of shaping and reliability in aqueous phases.

Inventive Principle:
Principle #40Composite materials

2Stability of the object's composition

If high proportions of dispersed phase are used, then the gel structure can be formed, but the applications are limited due to instability and fluidity

Engineering Contradiction:
Improvegel structure formationVSAvoidapplication stability
Core Design Contradiction:
Stability of the object's compositionVSReliability

Solution Approach 1:

The patent changes the bonding parameter from non-covalent to covalent interactions, which fundamentally alters the gel's stability profile. Covalent bonds provide irreversible, stable connections that maintain the gel structure while enabling new applications in aqueous environments where previous gels failed.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention replaces the unstable, short-lived non-covalent gel structures with stable, long-lasting covalently bonded networks. This transition creates durable materials that maintain their composition and structure over time, expanding application possibilities beyond the limited lifespan of conventional gels.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Shape

If covalent bonds are used to link droplets, then the material maintains shape and resists dilution, but the manufacturing complexity increases

Engineering Contradiction:
Improveshape maintenanceVSAvoidmanufacturing process complexity
Core Design Contradiction:
ShapeVSDevice complexity

Solution Approach 1:

The patent incorporates reactive functional groups into the surfactant molecules during the preliminary formulation stage. These pre-installed functional groups are designed to form covalent bonds under specific triggering conditions (light, heat, pH), allowing the gel structure to self-assemble with covalent crosslinking without requiring complex post-processing manufacturing steps.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention utilizes phase transition mechanisms where the covalent bonding process is triggered by external stimuli such as light irradiation or temperature changes. This allows the material to transition from a liquid precursor state to a gel state with covalently bonded droplets, simplifying manufacturing by using natural phase transitions rather than complex processing equipment.

Inventive Principle:
Principle #36Phase transitions

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The material maintains shape and stability in aqueous environments, enabling diverse applications by providing strong cohesion between droplets, thus overcoming the limitations of previous gel technologies.

Implementation Method 1

The droplets of the dispersed phase being covalently linked together by the surfactant of formula (I)

Methodology Applied
Scientific EffectCovalent bonding: Chemical Bonding

Implementation Method 2

an oil, and a surfactant of the following formula (I)

Methodology Applied
Scientific EffectSurface tension reduction: Surfactant

Data Source

PatentEP2830591B1Material, its process of preparation and utilisations thereof
Publication Date: 2023.03.22 COMMISSARIAT A LENERGIE ATOMIQUE ET AUX ENERGIES ALTERNATIVES
  • EP2830591B1 patent drawingFigure 1~2
  • EP2830591B1 patent drawingFigure 3~4
  • EP2830591B1 patent drawingFigure 5~6

AI summary

The invention relates to a material including a continuous aqueous phase and a dispersed phase in the form of droplets including an amphiphilic lipid and a surfactant having the following formula (I): (L1-X1-H1-Y1)v-G-(Y2-H2-X2-L2)w (I), where: L1 and L2 are independently lipophilic groups; X1, X2, Y1, Y2 and G are independently a linkage group; H1 and H2 are independently hydrophilic groups including a polyalkoxylated chain; and v and w are independently an integer from 1 to 8, wherein the droplets of the dispersed phase are covalently bonded by the surfactant of formula (I), the invention also relating to the method for preparing same and to the uses thereof.