Covalent Modifier Attachment on Aminoplast Microcapsule Shells

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Solution Overview

Problem

Existing methods for surface modification of microcapsules, such as adding modifiers to an aqueous slurry or entrapping them in the capsule shell, are inefficient, leading to either loss of modifiers during use or reduced functionality, and lack control over the degree of entrapment.

Innovation Solution

Covalent attachment of modifiers to the surface of aminoplast microcapsule shells using coupling molecules with epoxy groups, ensuring stable and functional surface modification.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If modifiers are added to aqueous slurry and rely on preferential adhesion, then the modification process is simple, but the modifiers can be washed off the surface reducing or removing the desired effect

Engineering Contradiction:
Improvemodification process simplicityVSAvoidmodifier retention on capsule surface
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent introduces a coupling molecule as an intermediary that contains both a shell-binding group (for binding to capsule shell) and a modifier-binding group (for binding to modifier). This mediator enables covalent attachment of modifiers to capsules while maintaining process simplicity, resolving the contradiction between ease of manufacture and reliability of modifier retention.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent changes the bonding parameter from weak physical adhesion (van der Waals forces) to strong covalent bonding through the coupling molecule. This parameter change ensures modifiers remain attached under rinsing conditions while preserving the simplicity of the modification process.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If modifiers are entrapped in the capsule shell during formation, then the modifier is secured in place, but its functionality and effectiveness may be reduced

Engineering Contradiction:
Improvemodifier retention on capsule surfaceVSAvoidreduced modifier functionality
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent applies local quality by positioning the modifier at the capsule surface through covalent attachment rather than deep entrapment in the shell matrix. The coupling molecule anchors the modifier at the interface, ensuring both retention and accessibility for functionality, thus resolving the contradiction between reliability and harmful effects.

Inventive Principle:
Principle #3Local quality

3Reliability

If high degree of entrapment of modifier is used, then the modifier is secured in place, but its functionality and effectiveness are reduced

Engineering Contradiction:
Improvemodifier retention on capsule surfaceVSAvoidmodifier effectiveness
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent applies partial action by using a coupling molecule that provides just enough attachment strength to retain modifiers during rinsing, without excessive entrapment that would reduce functionality. The covalent bonding through the coupling molecule achieves optimal retention while preserving modifier accessibility and effectiveness.

Inventive Principle:
Principle #16Partial or excessive action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The covalent grafting of modifiers enhances the capsules' ability to adhere to substrates, maintaining their functionality and performance under adverse conditions, such as rinsing, thereby increasing the retention of active core materials like fragrances in laundry products.

Implementation Method 1

covalent attachment of the modifier to the capsule shell surface by means of a coupling molecule capable of covalent bonding to both shell and modifier by means of epoxy groups on the coupling molecule

Methodology Applied
Scientific EffectCovalent bonding: Chemical Bonding

Implementation Method 2

Aminoplast polymer capsule walls contain on their surface secondary amine groups. These will readily react with epoxides.

Methodology Applied
Scientific EffectEpoxy reaction with amine groups: Chemical Bonding

Data Source

PatentEP3582888B1Process for preparing microcapsules comprising a microcapsule modifier
Publication Date: 2024.01.24 GIVAUDAN SA
  • EP3582888B1 patent drawingFigure 1a~1b
  • EP3582888B1 patent drawingFigure 2a~3b
  • EP3582888B1 patent drawing

AI summary

A method of providing a modifier on the surface of an active-containing core-shell aminoplast microcapsule, comprising the covalent attachment of the modifier to the capsule shell surface by means of a coupling compound capable of covalent bonding to both shell and modifier by means of epoxy groups on the coupling compound. The method is especially useful for enhancing the substantiveness to fabrics of fragrance microcapsules added to laundry products.