Ebullated Bed Hydroconversion of Bio-Feeds for Fuel Bases

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Solution Overview

Problem

Existing processes for producing fuel bases from vegetable and animal oils face challenges such as high costs, limited cold properties, and narrow distillation ranges, as well as catalyst contamination issues due to the formation of water and carbon oxides in fixed bed reactors during hydrotreatment and hydroconversion.

Innovation Solution

An ebullated bed process using a catalyst free of Zn, Mg, and Ca, which allows for direct treatment of crude bio-renewable feeds without prior purification, maximizing fuel base yield and minimizing catalyst contamination by employing a granular catalyst with hydrodehydrogenating metals like nickel and molybdenum on an amorphous support, and optimizing conditions for hydrotreatment and hydroconversion.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If fixed bed reactor is used for hydrotreatment and hydroconversion of vegetable oils and animal fats, then catalyst contamination occurs due to formation of water and carbon oxides, but reactor simplicity and ease of operation are maintained

Engineering Contradiction:
Improvecatalyst efficiencyVSAvoidcatalyst contamination
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the operational parameters of the reactor from fixed bed to ebullated bed mode, which fundamentally alters the hydrodynamics and mass transfer conditions. This parameter change allows the catalyst to be continuously circulated and regenerated, preventing contamination accumulation and maintaining catalyst efficiency throughout the process.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention transitions from a static fixed bed reactor to a dynamic ebullated bed reactor where the catalyst is in constant motion, suspended by gas or liquid flow. This dynamic operation enables continuous removal of contaminated catalyst and replacement with fresh catalyst, resolving the contamination issue while maintaining operational simplicity.

Inventive Principle:
Principle #15Dynamics

2Reliability

If prior purification steps are performed to remove metals and impurities from crude oils, then catalyst contamination is reduced, but process cost and complexity increase

Engineering Contradiction:
Improvecatalyst performanceVSAvoidprocess steps
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The invention extracts and removes the purification step from the overall process by using an ebullated bed reactor that can tolerate and handle crude feeds directly. The reactor design itself provides the necessary separation and protection functions, eliminating the need for separate pre-treatment units and reducing process complexity.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The ebullated bed reactor performs self-purification through continuous catalyst circulation and regeneration. The system automatically handles impurity removal and catalyst maintenance without requiring external purification facilities, allowing direct processing of crude oils while maintaining catalyst performance.

Inventive Principle:
Principle #25Self-service

3Ease of manufacture

If vegetable oil methyl esters are used as biofuels, then production cost is reduced and process simplicity is improved, but cold properties and cetane numbers remain limited

Engineering Contradiction:
Improveproduction costVSAvoidfuel properties
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The invention produces a composite fuel product by combining the benefits of esterification (cost-effectiveness) with hydroconversion (superior fuel properties). The ebullated bed reactor facilitates simultaneous or sequential esterification and hydroconversion, creating a fuel that meets both economic and performance requirements through composite chemical transformation.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process produces fuel bases with excellent combustion properties, thermal stability, and storage stability, achieving high cetane numbers and smoke points, while maintaining catalyst efficiency and reducing unwanted co-product formation.

Implementation Method 1

hydrotreatment and/or hydroconversion of said bio-renewable feed in an ebullated bed reactor in the presence of a granular catalyst comprising, on an amorphous support, at least one metal or compound of a metal having a hydrodehydrogenating function

Methodology Applied
Scientific EffectHydroconversion: Catalysis

Implementation Method 2

at least one metal or compound of a metal having a hydrodehydrogenating function, to produce a first effluent

Methodology Applied
Scientific EffectHydrodehydrogenation: Catalysis

Implementation Method 3

ebullated bed process for hydrotreatment (HDT) and/or hydroconversion (HDC) of feeds of bio-renewable origin

Methodology Applied
Scientific EffectFluidization: Fluidisation

Data Source

PatentUS8877993B2Process for ebullated bed hydroconversion of feeds of bio-renewable origin for the production of fuel bases
Publication Date: 2014.11.04 IFP ENERGIES NOUVELLES

AI summary

The invention concerns a process for hydrotreatment and/or hydroconversion of a feed of bio-renewable origin containing triglyceride and/or fatty acid structures and wherein the fatty chains contain in the range 8 to 25 carbon atoms, said process comprising the following steps:a) hydrotreatment and/or hydroconversion of said bio-renewable feed in an ebullated bed reactor in the presence of a granular catalyst comprising, on an amorphous support, at least one metal or compound of a metal having a hydrodehydrogenating function, to produce a first effluent;b) sending the effluent produced in step a) to a distillation zone from which a gaseous fraction and at least one distillate cut the end point of which is less than 400° C.