Secondary Battery Electrode Pore Analysis via Silicon EDS Mapping

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Solution Overview

Problem

Current methods fail to accurately analyze the distribution of pores within secondary battery electrodes due to the inability to distinguish between constituent materials and pores, leading to inaccurate performance prediction.

Innovation Solution

A method involving ion milling to produce a clean electrode cross-sectional sample, filling pores with a silicon-containing polymer, and using energy-dispersive X-ray spectroscopy to map and analyze the distribution of silicon, allowing clear differentiation between materials and pores.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If scanning electron microscope (SEM) is used to observe electrode cross-section, then deep focal depth allows signals from different focal planes to be detected, but this causes constituent materials inside the electrode to be expressed as pores, making it impossible to exactly analyze the distribution of pores

Engineering Contradiction:
Improvepore distribution analysis accuracyVSAvoiddistinction between constituent materials and pores
Core Design Contradiction:
Measurement precisionVSLoss of information

Solution Approach 1:

The patent introduces a staining agent as an intermediary substance that selectively binds to constituent materials in the electrode. This staining agent has different affinity for different materials, causing them to appear with different contrast levels in SEM images. This allows clear distinction between constituent materials and pores, resolving the information loss problem while maintaining the deep focal depth advantage of SEM

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent applies staining agents that cause constituent materials to exhibit different contrast levels or 'colors' in SEM images based on their chemical composition. This color/contrast differentiation enables clear visual distinction between various constituent materials and pores, allowing accurate pore distribution analysis without the information loss that would otherwise occur

Inventive Principle:
Principle #32Color changes

2Reliability

If conventional observation methods are used, then the process is simple, but it is impossible to clearly distinguish constituent materials and pores inside the electrode from each other

Engineering Contradiction:
Improvedistinguishment clarity between materials and poresVSAvoidmeasurement process complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent applies staining agents to the electrode cross-section before SEM observation. This preliminary staining action modifies the constituent materials to have different contrast properties, ensuring that when the SEM image is taken, the distinction between materials and pores is already established. This preliminary preparation resolves the reliability issue while keeping the overall process manageable

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Enables precise analysis of pore size, number, and distribution, improving the prediction of secondary battery performance by clearly distinguishing between electrode components.

Implementation Method 1

irradiating the electrode for a secondary battery with an ion beam of an ion milling device to produce an electrode cross-sectional sample

Methodology Applied
Scientific EffectIon beam sputtering: Ion Beam

Implementation Method 2

detecting silicon present on the electrode cross-sectional sample by using an energy-dispersive X-ray spectroscopy

Methodology Applied
Scientific EffectEnergy-dispersive X-ray spectroscopy: X-Ray

Data Source

PatentEP3633359B1Method for measuring pore distribution in electrode for secondary battery
Publication Date: 2024.06.12 LG ENERGY SOLUTION LTD
  • EP3633359B1 patent drawingFigure 1
  • EP3633359B1 patent drawingFigure 2A~2B
  • EP3633359B1 patent drawingFigure 3A~3B

AI summary

The present invention provides a method for measuring a distribution of pores in an electrode for a secondary battery, which can easily measure a distribution of pores inside the electrode for a secondary battery.