Gold Evaporative Source Cleaning for Thin-Film Deposition

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Solution Overview

Problem

The gold evaporative process in thin-film deposition often experiences 'spitting' due to surface contaminants, leading to in-film defects and reduced deposition rates, which conventional methods struggle to control effectively.

Innovation Solution

A method involving burnishing gold evaporative sources with a liquid slurry under controlled vibratory action followed by leaching with boiling nitric acid to remove contaminants, reducing surface roughness and embedded impurities without altering the surface morphology.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If power input is increased to compensate for reduced deposition rate, then deposition rate is improved, but spitting occurs leading to in-film defects

Engineering Contradiction:
Improvedeposition rateVSAvoidspitting and in-film defects
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

The gold evaporative source undergoes preliminary cleaning treatments (mechanical polishing, chemical etching, and ultrasonic cleaning) before being placed in the evaporation chamber. This preliminary action removes surface contaminants that would otherwise cause spitting during high-power deposition, enabling increased deposition rates without defect formation.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention changes the surface condition parameter of the gold evaporative source through controlled cleaning processes. By modifying the surface cleanliness and roughness parameters before evaporation, the system can operate at higher power levels without experiencing spitting, thus resolving the contradiction between deposition rate and defect formation.

Inventive Principle:
Principle #35Parameter changes

2Ease of manufacture

If conventional cleaning methods are used, then manufacturing simplicity is maintained, but surface contaminants remain leading to spitting

Engineering Contradiction:
Improvecleaning process simplicityVSAvoidsurface contaminants and spitting
Core Design Contradiction:
Ease of manufactureVSObject-affected harmful factors

Solution Approach 1:

The cleaning process is segmented into multiple distinct steps: mechanical polishing to remove rough contaminants, chemical etching to dissolve embedded impurities, and ultrasonic cleaning to dislodge remaining particles. This segmentation allows each step to target specific types of contaminants, achieving thorough cleaning while maintaining procedural simplicity.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

Chemical reagents serve as intermediaries between the cleaning system and the gold evaporative source surface. The chemicals facilitate the removal of contaminants that mechanical methods alone cannot eliminate, bridging the gap between simple manufacturing processes and effective contaminant removal.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Manufacturing precision

If power input is controlled to prevent spitting, then in-film defects are reduced, but deposition rate decreases

Engineering Contradiction:
Improvefilm quality without defectsVSAvoiddeposition rate
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

By performing thorough preliminary cleaning of the gold evaporative source, the system eliminates the need for conservative power control. The cleaned surface prevents spitting even at high power levels, allowing the process to achieve both high deposition rates and defect-free films simultaneously.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention changes the surface condition parameter of the evaporative source to enable high-power operation without spitting. This parameter change (surface cleanliness) decouples the trade-off between power input and film quality, allowing both high deposition rate and high film quality to be achieved.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Significantly reduces surface contaminants, minimizing the occurrence of spitting and resulting in higher-quality gold films with reduced defects and improved deposition rates.

Implementation Method 1

burnishing the gold evaporative sources against each other in the presence of a liquid slurry at ambient temperature under a controlled vibratory action, thereby loosening and removing at least a portion of contaminants

Methodology Applied
Scientific EffectAbrasion: Abrasion

Implementation Method 2

leaching the partially cleaned gold evaporative sources with boiling nitric acid to dislodge and remove contaminants along at least one of the first face, the second face or the one or more surfaces

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 3

Electron beam or resistance heating elements can serve as the heat source 104 to melt the gold evaporative source 102. The melting of the gold evaporative source 102 creates a liquid pool 105

Methodology Applied
Scientific EffectJoule heating: Joule Heating

Implementation Method 4

The gold evaporative source in molten form is further heated until vaporization occurs. The gold vapor traverses upwards within the interior of the tool 101, and ultimately condenses and deposits as a thin-film onto one or more surfaces of a series of wafers 106

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP2963148B1Methods for making gold evaporative sources with reduced contaminants
Publication Date: 2018.10.31 PRAXAIR ST TECHNOLOGY INC
  • EP2963148B1 patent drawingFigure 1
  • EP2963148B1 patent drawingFigure 2
  • EP2963148B1 patent drawingFigure 3(a)~3(b)

AI summary

A unique sequence of steps is provided to reduce contaminants along one or more surfaces and faces of gold evaporative sources without deleteriously impacting the structure of the gold evaporative sources. Edges are deburred; contaminants are successfully removed therealong; and surface smoothness is substantially retained. The resultant gold evaporative source is suitable for use in evaporative processes as a precursor to gold film deposition without the occurrence or a substantial reduction in the likelihood of spitting by virtue of significantly reduced levels of contaminants, in comparison to gold evaporative sources subject to a standard cleaning protocol.