Graphite Bipolar Plate Bonding With 1K Epoxy for Fast Curing

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Solution Overview

Problem

The mechanical connection of graphitic monopolar plates to form bipolar plates for fuel cells is challenging due to the need for strong, chemically resistant, and gas-tight bonding while maintaining simplicity and cost-effectiveness in process technology, with conventional adhesives often having limitations such as short pot life, long curing times, and potential thermal issues.

Innovation Solution

A method using 1K epoxy resin adapted with aromatic amines as solid hardeners, which is heated to at least 200°C for rapid curing, providing a strong and durable bond suitable for high-temperature applications, while ensuring thermal stability and long pot life, thus overcoming the limitations of conventional adhesives.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional adhesives (2K epoxy resin, cyanoacrylates, silicone polymers) are used to bond graphitic monopolar plates, then the bonding strength and chemical resistance are improved, but the production time increases due to long curing times and short pot life

Engineering Contradiction:
Improvebonding strengthVSAvoidproduction time
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent applies parameter changes by modifying the adhesive system from conventional 2K epoxy resin to a specifically formulated 1K epoxy resin with altered chemical composition and curing characteristics. This 1K resin is designed with extended pot life and reduced curing time through compositional adjustments, directly resolving the contradiction between bonding reliability and production productivity by enabling both strong bonds and faster manufacturing cycles

Inventive Principle:
Principle #35Parameter changes

2Ease of manufacture

If 1K epoxy resin is used for bonding, then the production process is simplified and pot life is extended, but the curing time increases and thermal stability may be compromised

Engineering Contradiction:
Improveprocess simplicityVSAvoidcuring time
Core Design Contradiction:
Ease of manufactureVSDuration of action of moving object

Solution Approach 1:

The patent resolves this contradiction through parameter changes by formulating a specialized 1K epoxy resin with modified chemical composition that simultaneously achieves extended pot life for ease of manufacture and reduced curing time for productivity. The specific resin formulation parameters are optimized to balance these opposing requirements, enabling both simplified processing and acceptable curing speeds

Inventive Principle:
Principle #35Parameter changes

3Strength

If high bonding strength is achieved through conventional adhesives, then mechanical connection is improved, but gas permeability may be reduced due to potential sealing of channel structures

Engineering Contradiction:
Improvemechanical connection strengthVSAvoidgas permeability
Core Design Contradiction:
StrengthVSObject-affected harmful factors

Solution Approach 1:

The patent applies local quality by carefully controlling the adhesive application to specific locations and thicknesses on the monopolar plates. The bonding process is designed to create strong mechanical connections at the bonding interfaces while maintaining controlled gas permeability in the channel structures. This selective bonding approach ensures that structural strength is achieved without compromising the fuel cell's gas flow requirements

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The 1K epoxy resin method enables rapid and efficient bonding of graphitic monopolar plates with high mechanical strength, chemical resistance, and gas-tightness, facilitating high production rates and maintaining strength at operating temperatures, thereby improving the manufacturing efficiency and performance of bipolar plates.

Implementation Method 1

The 1K epoxy resin is used in a process step (ii) of bonding the monopolar plates, wherein the 1K epoxy resin is adapted to have an activation temperature of at least 50°C by using aromatic amines as solid hardeners

Methodology Applied
Scientific EffectThermal heating: Heating

Implementation Method 2

A method using 1K epoxy resin adapted with aromatic amines as solid hardeners, which is heated to at least 200°C for rapid curing

Methodology Applied
Scientific EffectCuring:

Implementation Method 3

A 1K epoxy resin is used for bonding, which is adapted to have an activation temperature of at least 50°C by using aromatic amines as solid hardeners

Methodology Applied
Scientific EffectChemical bonding: Chemical Bonding

Data Source

PatentEP4295425B1Process for manufacturing a graphite bipolar plate by adhesively bonding monopolar plates, and bipolar plate and fuell cell or redox flow battery comprising same
Publication Date: 2024.10.16 SCHUNK KOHLENSTEOFFTECHNIK GMBH
  • EP4295425B1 patent drawingFigure 1~2
  • EP4295425B1 patent drawingFigure 3~4

AI summary

A process for manufacturing a graphite bipolar plate (1) for a fuel cell (21) or a redox flow battery is described. A pair of graphite monopolar plates (3) is provided. Said monopolar plates (3) are adhesively bonded to one another along opposing contact surfaces (7) of the monopolar plates (3). A 1K epoxy resin (9) is used for creating the adhesive bond. Properties of the 1K epoxy resin (9) and/or process parameters can be adjusted to the specific use.