Hydrocarbon Desulfurization via Oxidation and Extraction

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Solution Overview

Problem

Current methods for removing sulfur compounds from hydrocarbon streams, such as diesel fuel, are inadequate in achieving ultra-low sulfur levels required by stringent regulations, as they often result in high waste streams and hydrocarbon component losses.

Innovation Solution

A tailored oxidation process involving primary, secondary, and tertiary oxidants, along with phase transfer catalysts, to convert sulfur compounds into sulphoxides and sulphones, which are then extracted, producing low sulfur hydrocarbon streams with minimal waste and hydrocarbon loss.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional desulfurization methods are used, then sulfur removal is achieved, but high waste streams and hydrocarbon component losses occur

Engineering Contradiction:
Improvesulfur removal efficiencyVSAvoidhydrocarbon component loss
Core Design Contradiction:
Manufacturing precisionVSLoss of substance

Solution Approach 1:

The patent employs strong oxidants including ozone, hydrogen peroxide, and peracetic acid to oxidize sulfur compounds in hydrocarbon streams. This oxidation converts sulfur compounds into water-soluble forms that can be easily removed through extraction, achieving ultra-low sulfur levels while preserving hydrocarbon components without the losses associated with conventional methods

Inventive Principle:
Principle #38Strong oxidants (Accelerated oxidation)

Solution Approach 2:

The patent introduces an intermediary extraction step using water or aqueous solutions to separate oxidized sulfur compounds from the hydrocarbon stream. This intermediary medium allows for selective removal of sulfur compounds while leaving the desired hydrocarbon components intact, thereby reducing both waste streams and hydrocarbon losses

Inventive Principle:
Principle #24Intermediary (Mediator)

2Manufacturing precision

If oxidation process is used to convert sulfur compounds, then sulfur levels are reduced to ultra-low ppm, but process complexity increases

Engineering Contradiction:
Improvesulfur content reductionVSAvoidprocess steps
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent segments the desulfurization process into distinct sequential steps: oxidation of sulfur compounds followed by extraction. This segmentation allows each step to be optimized independently and facilitates easier control and monitoring, reducing overall process complexity while achieving ultra-low sulfur levels

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent utilizes parameter changes in the oxidation process, specifically adjusting oxidant concentration, contact time, and temperature, to optimize sulfur removal efficiency. By controlling these parameters, the process achieves consistent ultra-low sulfur levels without requiring overly complex process equipment or procedures

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process effectively reduces sulfur levels in hydrocarbons to ultra-low ppm, minimizing waste and hydrocarbon loss, while allowing for recycling of low sulfur streams and the production of valuable low sulfur aromatic hydrocarbons.

Implementation Method 1

A tailored oxidation process involving primary, secondary, and tertiary oxidants, along with phase transfer catalysts, to convert sulfur compounds into sulphoxides and sulphones

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 2

which are then extracted, producing a low sulfur hydrocarbon stream

Methodology Applied
Scientific EffectLiquid-liquid extraction: Liquid-Liquid Extraction

Data Source

PatentEP2970795B1Process for removing sulphur compounds from hydrocarbons
Publication Date: 2020.05.27 ULTRACLEAN FUEL LTD
  • EP2970795B1 patent drawingFigure 1
  • EP2970795B1 patent drawingFigure 2
  • EP2970795B1 patent drawingFigure 3

AI summary

The present disclosure relates to a process for reducing the sulphur content of hydrocarbon feedstocks such as Natural Gas Condensate, Kerosene, Jet Fuel, Diesel, Vacuum Gas Oil and Fuel Oil. The process uses a tailored oxidation process comprising one or two oxidation steps to produce sulphoxides and/or sulphones. These sulphoxides and sulphones, whilst being still present in the liquid hydrocarbon streams, are subsequently extracted thereby producing a low sulphur hydrocarbon stream and optionally following further treatment of the sulphoxides and/or sulphones, produce a low sulphur aromatic hydrocarbon stream and an aqueous stream of sodium sulphite or sulphuric acid. The low sulphur hydrocarbon stream and low sulphur aromatic hydrocarbon stream may be individually recycled or combined for recycling.