Hydrogel-Ceramic Separator for Low-Resistance Gas Barrier

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Solution Overview

Problem

Existing electrochemical devices, such as water electrolysers and fuel cells, face challenges with separators that compromise between safety and efficiency due to limitations in thickness, porosity, and chemical stability, particularly in alkaline conditions, leading to high ionic resistance and potential gas crossover.

Innovation Solution

A porous carrier with a hydrogel made of a metal oxide and an aqueous medium is used, which provides low gas permeability, high ionic conductivity, and chemical stability, allowing for efficient ion transport while preventing gas crossover, by creating a membrane-like function within a ceramic-type hydrogel supported by a porous carrier.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If a diaphragm separator is used, then gas barrier properties are improved, but ionic resistance increases and thickness must be increased

Engineering Contradiction:
Improvegas crossoverVSAvoidionic resistance
Core Design Contradiction:
Object-affected harmful factorsVSReliability

Solution Approach 1:

The separator combines a porous ceramic support structure with a hydrogel coating layer, creating a composite material that integrates the gas barrier properties of the ceramic substrate with the high ionic conductivity of the hydrogel layer, thereby achieving low ionic resistance while maintaining gas barrier performance

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The separator utilizes a porous ceramic substrate with controlled pore structure that provides both mechanical support and gas barrier functionality, while the porosity allows for hydrogel infiltration to enhance ionic conductivity without compromising the gas blocking capability

Inventive Principle:
Principle #31Porous materials

2Reliability

If separator thickness is reduced to lower ionic resistance, then ionic conductivity is improved, but mechanical robustness and gas barrier properties deteriorate

Engineering Contradiction:
Improveionic resistanceVSAvoidmechanical robustness
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The composite structure of a rigid porous ceramic substrate combined with a hydrogel coating enables the separator to achieve thin dimensions with low ionic resistance while the ceramic substrate provides the necessary mechanical strength and gas barrier properties that would be impossible to achieve with hydrogel alone

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The separator employs different materials with specialized functions at different locations: the porous ceramic substrate provides mechanical support and gas barrier properties, while the hydrogel coating layer specifically enhances ionic conductivity at the separator surfaces and pores

Inventive Principle:
Principle #3Local quality

3Reliability

If a membrane separator is used, then ionic conductivity is improved, but chemical stability in alkaline conditions deteriorates

Engineering Contradiction:
Improveionic conductivityVSAvoidchemical stability
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

The separator combines a chemically stable porous ceramic substrate (such as alumina or titania) with a hydrogel coating that provides high ionic conductivity, creating a composite where the ceramic component ensures chemical stability in alkaline environments while the hydrogel maintains excellent ion transport properties

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution results in a separator with low ionic resistance and enhanced mechanical robustness, enabling efficient operation in alkaline conditions while maintaining safety by effectively preventing gas crossover and ensuring stable performance.

Implementation Method 1

a hydrogel, made of a first metal oxide and an aqueous medium, present within the first of both largest sides and in at least part of the thickness

Methodology Applied
Scientific EffectIonic conduction: Conduction (electrical)

Implementation Method 2

a porous carrier having two, respectively a first and a second, largest parallel sides separated by a thickness

Methodology Applied
Scientific EffectDiffusion: Diffusion

Implementation Method 3

the separator may have a low gas permeability, i.e., may act as a good gas barrier

Methodology Applied
Scientific EffectPermeation barrier: Permeation

Data Source

PatentEP4407071A1Separator for electrochemical devices
Publication Date: 2024.07.31 THE HYVE BV
  • EP4407071A1 patent drawingFigure 1~5
  • EP4407071A1 patent drawingFigure 6~7
  • EP4407071A1 patent drawingFigure 8~9

AI summary

A separator (3) for an electrochemical device (9), comprising: a. A porous carrier (1) having two, respectively a first and a second, largest parallel sides (15, 16) separated by a thickness, and b. A hydrogel (10), made of a first metal oxide (12) and an aqueous medium, present within the first of both largest sides (15) and in at least part of the thickness.