Inductively Heated Packed Bed Reactor for Lithium Recovery

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Solution Overview

Problem

Current methods are inadequate for efficiently recovering lithium and phosphorus from lithium-ion battery residues in a versatile manner, regardless of the chemical structure or composition of the raw material, as they often result in impurities and reduced yield.

Innovation Solution

An inductively heated, packed bed reactor system with a refractory reactor body and varying susceptor material particle sizes is used to transfer lithium and phosphorus compounds into a gaseous phase, allowing for separation and recovery, while minimizing thermal and chemical stress on the reactor materials.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional thermal treatment methods are used to recover lithium and phosphorus from lithium-ion battery residues, then the recovery process can be performed, but the recovery yield is reduced and impurities remain in the recovered materials

Engineering Contradiction:
Improvepurity of recovered lithium and phosphorusVSAvoidrecovery yield of lithium and phosphorus
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The invention utilizes phase transitions by vaporizing lithium and phosphorus compounds at high temperatures (1000-2000°C) to transfer them into the gas phase, then condensing them in a condenser to obtain purified recovered materials. This phase transition approach enables simultaneous high purity and high recovery yield by separating the target materials from impurities through vaporization and selective condensation.

Inventive Principle:
Principle #36Phase transitions

2Productivity

If high temperatures are applied to vaporize lithium and phosphorus compounds, then recovery efficiency improves, but thermal stress on the reactor materials increases

Engineering Contradiction:
Improverecovery efficiency of lithium and phosphorusVSAvoidthermal stress on reactor materials
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

The invention introduces a susceptor material as an intermediary substance that absorbs electromagnetic radiation and converts it to heat, indirectly heating the lithium-ion battery residues. This mediator approach enables high-temperature treatment (1000-2000°C) required for efficient vaporization while protecting the reactor structure from direct thermal exposure, thus maintaining high recovery efficiency without excessive thermal stress on reactor materials.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The invention replaces conventional direct thermal heating with electromagnetic induction heating using a susceptor material. This substitution allows precise control of heating zones and temperatures, enabling efficient vaporization of lithium and phosphorus compounds at 1000-2000°C while minimizing unwanted thermal stress on reactor materials through localized and controlled energy input.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Stability of the object's composition

If the reactor body is made of refractory material to withstand high temperatures, then thermal stability improves, but the device complexity increases

Engineering Contradiction:
Improvethermal stability of reactor bodyVSAvoidcomplexity of reactor construction
Core Design Contradiction:
Stability of the object's compositionVSDevice complexity

Solution Approach 1:

The susceptor material serves as a thermal intermediary that absorbs electromagnetic energy and transfers heat to the processing materials. This mediator function allows the use of refractory materials for the reactor body to withstand high temperatures (1000-2000°C) while the actual heating occurs through electromagnetic induction in the susceptor, reducing direct thermal exposure and simplifying the overall thermal management complexity of the reactor construction.

Inventive Principle:
Principle #24Intermediary (Mediator)

4Stability of the object's composition

If varying particle sizes of susceptor material are used to optimize heat distribution, then thermal treatment uniformity improves, but the device complexity increases

Engineering Contradiction:
Improveuniformity of thermal treatmentVSAvoidcomplexity of susceptor arrangement
Core Design Contradiction:
Stability of the object's compositionVSDevice complexity

Solution Approach 1:

The invention applies local quality by using susceptor material particles with varying sizes (0.1-10 mm) distributed throughout the reactor bed. Different particle sizes create varied heat absorption and distribution characteristics in different regions, improving thermal treatment uniformity across the entire charge material volume. This natural size distribution approach achieves uniform heating without requiring complex external heating zones or adjustable mechanisms, thus improving thermal uniformity while maintaining relatively simple device structure.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables the high-purity recovery of lithium and phosphorus, along with other metals, by effectively separating gaseous and molten phases, reducing impurities, and optimizing thermal treatment conditions.

Implementation Method 1

an induction coil (114) surrounding the reactor body (112) and configured for inductively heating the susceptor material (116)

Methodology Applied
Scientific EffectElectromagnetic induction: Electromagnetic Induction

Implementation Method 2

the reactor body (112) being surrounded by at least one induction coil (114), the induction coil (114) being configured for inductively heating the susceptor material (116)

Methodology Applied
Scientific EffectInductive heating: Induction Heating

Implementation Method 3

the reactor body (112) being at least partially filled with a susceptor material (116), the induction coil (114) being configured for inductively heating the susceptor material (116)

Methodology Applied
Scientific EffectElectromagnetic energy absorption and conversion to heat: Dielectric Heating

Implementation Method 4

thermally treating the raw material in the inductively heated packed bed reactor, such that at least part of the raw material including lithium compounds and/or phosphorus compounds is transferred into a gaseous phase

Methodology Applied
Scientific EffectVaporization: Evaporation

Implementation Method 5

a condenser (150) in fluidic connection with the one or more gas outlets (118) and configured for depositing lithium species from a gaseous phase discharged from the packed bed reactor

Methodology Applied
Scientific EffectCondensation: Condensation

Data Source

PatentEP4114997B1Apparatus and process for thermal treatment of raw material containing lithium compounds and phosphorus compounds, method of recovering lithium and/or phosphorus from residue material of lithium-ion batteries
Publication Date: 2024.04.03 MONTANUNIV LEOBEN
  • EP4114997B1 patent drawingFigure 1
  • EP4114997B1 patent drawingFigure 2

AI summary

The present invention relates to an apparatus (100) for thermal treatment of a raw material containing lithium compounds and phosphorus compounds, a process for thermal treatment of a raw material containing lithium compounds and phosphorus compounds and a method of recovering lithium and/or phosphorus from residue material of lithium-ion batteries. The apparatus (100) for thermal treatment of a raw material containing lithium compounds and phosphorus compounds comprises an inductively heated, packed bed reactor (110) comprising a reactor body (112) at least partially made of refractory material, the reactor body (112) being surrounded by at least one induction coil (114), the reactor body (112) being at least partially filled/packed with a susceptor material (116), the inductively heated packed bed reactor (110) being configured for transferring at least part of the raw material including lithium compounds and/or phosphorus compounds into a gaseous phase and configured for forming a molten phase from another part of the raw material, the inductively heated packed bed reactor (110) comprising one or more gas outlets (118) and a molten phase outlet (119), and a condenser (150) in fluidic connection with the one or more gas outlets (118) and configured for depositing lithium species from a gaseous phase discharged from the packed bed reactor (110) via the one or more gas outlets (118) and configured for separating the deposited lithium species from an exhaust gas substantially free from lithium species.