Integrated Ammonia–Nitric Acid Process With Ammonia Buffering

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Solution Overview

Problem

The production of ammonia and nitric acid is challenged by the inflexibility of processes powered by renewable energy sources, leading to fluctuations in hydrogen production, which affects the entire process efficiency and profitability, and requires costly energy storage solutions.

Innovation Solution

A method for controlling an integrated ammonia-nitric acid process that switches between modes of operation based on available power, storing excess ammonia during high availability and using it during low availability, with thermal and electric power transfer between processes to maintain consistent output.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If the process is powered by renewable energy sources, then the carbon footprint is reduced, but the process flexibility deteriorates due to fluctuations in energy availability

Engineering Contradiction:
Improvecarbon footprintVSAvoidprocess flexibility
Core Design Contradiction:
Object-affected harmful factorsVSAdaptability or versatility

Solution Approach 1:

The patent applies preliminary action by producing and storing ammonia during periods of high renewable energy availability before the fluctuations occur. The ammonia storage unit accumulates excess ammonia when energy is abundant, allowing the process to continue operating during periods of low energy availability without external intervention, thus resolving the flexibility issue while maintaining low carbon footprint

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent changes the operational parameters by switching between different production modes (first mode with high ammonia production and storage, second mode with adjusted production) based on renewable energy availability. This dynamic parameter adjustment allows the process to adapt to fluctuating energy inputs while maintaining consistent output, resolving the contradiction between renewable energy usage and process flexibility

Inventive Principle:
Principle #35Parameter changes

2Productivity

If hydrogen production is increased to meet demand, then ammonia production increases, but the process efficiency deteriorates due to fluctuations in renewable energy availability

Engineering Contradiction:
Improveammonia productionVSAvoidprocess efficiency
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent implements feedback control by monitoring renewable energy availability and adjusting hydrogen production rates accordingly. The system receives feedback on energy input and modulates the water electrolysis rate to match actual availability, preventing inefficiency from producing more hydrogen than can be processed while ensuring continuous ammonia production, thus maintaining both productivity and efficiency

Inventive Principle:
Principle #23Feedback

Solution Approach 2:

The system performs preliminary action by storing excess ammonia during high-energy periods before efficiency deteriorates can occur. This advance storage ensures that when energy availability drops and production must be reduced, the system can maintain stable output by drawing from stored ammonia, thereby preserving process efficiency while meeting demand

Inventive Principle:
Principle #10Preliminary action

3Stability of the object's composition

If energy storage solutions are installed to buffer fluctuations, then process stability improves, but the capital cost increases

Engineering Contradiction:
Improveprocess stabilityVSAvoidcapital cost
Core Design Contradiction:
Stability of the object's compositionVSDevice complexity

Solution Approach 1:

The patent uses ammonia as an intermediary energy storage medium rather than installing complex electrical energy storage systems. The ammonia storage unit acts as a mediator that converts electrical energy fluctuations into chemical energy storage, providing process stability without requiring expensive batteries or other electrical storage infrastructure, thus achieving stability while minimizing capital cost

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The system applies self-service by using the process itself (ammonia production) to provide the storage function. The ammonia produced during high-energy periods serves as the storage medium, eliminating the need for separate energy storage systems. This self-service approach provides process stability while avoiding the capital costs of external storage infrastructure

Inventive Principle:
Principle #25Self-service

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enhances process flexibility, reduces capital costs for hydrogen and energy storage, and maintains consistent production of ammonia, nitric acid, and optionally ammonium nitrate, even with fluctuating renewable energy sources.

Implementation Method 1

hydrogen is produced from electrolysis of water

Methodology Applied
Scientific EffectElectrolysis: Electrolysis

Implementation Method 2

conversion to ammonia in a suitable catalytic converter

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 3

Heat is normally recovered from the process, e.g. from the hot reforming effluent and from the ammonia converter, in the form of steam

Methodology Applied
Scientific EffectHeat exchange: Heat Exchanger

Implementation Method 4

Steam at a sufficient pressure may be expanded in a steam turbine to produce energy

Methodology Applied
Scientific EffectThermal expansion: Thermal Expansion

Implementation Method 5

The stored ammonia is combusted when the amount of renewable energy is low. Thereby heat is produced which is converted into electricity.

Methodology Applied
Scientific EffectCombustion: Combustion

Data Source

PatentEP4377261B1Integrated process for the synthesis of ammonia and nitric acid
Publication Date: 2025.09.03 CASALE SA
  • EP4377261B1 patent drawingFigure 1
  • EP4377261B1 patent drawingFigure 2
  • EP4377261B1 patent drawingFigure 3

AI summary

An integrated process for the synthesis of ammonia and nitric acid, including the production of hydrogen from electrolysis of water, is controlled by a selective switching between a first mode of operation and a second mode of operation, wherein in the first mode of operation ammonia is produced in excess and is stored in a suitable ammonia storage; in the second mode of operation the ammonia from said ammonia storage is used to provide an additional input of ammonia to the production of nitric acid; the switching between said first mode and second mode is based on the amount of power which is transferred to the electrolysis of water.