Isotope-Enriched Polymer Contrast Agent for MRI Signal Sensitivity

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Solution Overview

Problem

Current contrast agents for nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) face challenges in achieving high selectivity and sensitivity due to background noise from natural isotopes, and existing solutions have limitations in signal intensity and stability.

Innovation Solution

A polymer with multiple 1H-13C-15N, 1H-15N-13C, or 1H-13C-13C sequences in its side chains, utilizing stable isotopes to enhance detectability and sensitivity in NMR and MRI applications.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If conventional contrast agents are used for NMR/MRI, then the imaging method is mildly invasive with high spatial resolution, but background noise from natural isotopes reduces selectivity and sensitivity

Engineering Contradiction:
Improveselectivity and sensitivityVSAvoidbackground noise from natural isotopes
Core Design Contradiction:
Measurement precisionVSObject-affected harmful factors

Solution Approach 1:

The patent changes the isotopic composition parameter by incorporating stable isotopes (13C, 15N, 1H) into the polymer structure. This parameter change transforms the contrast agent from using natural isotope abundance to using enriched stable isotopes, thereby reducing background noise and enhancing selectivity and sensitivity in NMR/MRI detection

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite contrast agent by combining polymer chains with multiple stable isotope sequences (1H-13C-15N, 1H-15N-13C, or 1H-13C-13C). This composite structure with multiple isotopic sequences working together provides synergistic enhancement of detectability while maintaining the mildly invasive nature of MRI

Inventive Principle:
Principle #40Composite materials

2Reliability

If existing contrast agents are used, then imaging can be performed, but signal intensity and stability are limited

Engineering Contradiction:
Improvesignal intensity and stabilityVSAvoidcomplexity of polymer synthesis
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent segments the polymer structure into repeating units, each containing specific stable isotope sequences. This segmentation allows systematic construction of the polymer with controlled isotopic composition, improving signal intensity through cumulative effect while managing synthesis complexity through modular design

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent changes the molecular composition parameter by incorporating stable isotopes with different spin properties (13C with spin 1/2, 15N with spin 1/2) into the polymer backbone and side chains. This parameter change enhances signal stability and intensity while the modular polymer design keeps manufacturing feasible

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The polymer increases the abundance of detectable sequences, leading to higher selectivity and sensitivity in NMR and MRI, while avoiding the limitations of natural isotope abundance and improving signal intensity and stability.

Implementation Method 1

Magnetic resonance imaging (hereinafter sometimes abbreviated as MRI), that is, an imaging method based on the principle of nuclear magnetic resonance (NMR)

Methodology Applied
Scientific EffectNuclear magnetic resonance:

Data Source

PatentEP2833925B1Polymer, contrast agent for nuclear magnetic resonance analysis or magnetic resonance imaging using the polymer, compound and method of nuclear magnetic resonance analysis and method of magnetic resonance imaging using the polymer
Publication Date: 2024.02.28 CANON KK
  • EP2833925B1 patent drawingFigure 1~2
  • EP2833925B1 patent drawingFigure 3~4
  • EP2833925B1 patent drawingFigure 5

AI summary

As a substance used as a contrast agent for a method of nuclear magnetic resonance analysis or a method of magnetic resonance imaging, a substance with high selectivity and high sensitivity was demanded. According to the present invention, when a polymer having, in a side chain thereof, a sequence of a 1H-13C-15N, 1H-15N-13C or 1H-13C-13C bond, that is, a structure labeled with stable isotopes of 13C and 15N, is used, the abundance of such a sequence in one molecule can be increased, and hence, high selectivity and higher sensitivity can be attained when used as a contrast agent.