Lithium Iron Phosphate Precursor Recovery With Low-Impurity Precipitation

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Solution Overview

Problem

Existing methods for reclaiming lithium iron phosphate batteries are inefficient, resulting in high impurity content, high reclamation costs, and significant environmental pollution.

Innovation Solution

A method is developed to produce a lithium iron phosphate precursor using a retired lithium iron phosphate battery as a raw material, involving steps such as soaking the battery cell in acid, performing electrolysis to reclaim copper, oxidizing ferrous iron, precipitating iron phosphate, and precipitating lithium carbonate, thereby achieving low impurity content and reduced reclamation costs.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If physical methods (screening, flotation, wind separation, eddy-current separation) are used to remove copper and aluminum impurities, then separation capability is improved, but device complexity and maintenance costs increase significantly

Engineering Contradiction:
Improveimpurity removal capabilityVSAvoidequipment complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent replaces complex mechanical separation systems (screening, flotation, wind separation, eddy-current separation) with a simple chemical precipitation system. Instead of using multiple sophisticated physical separation devices, the invention uses chemical reagents to transform impurities into precipitates that can be removed through simple filtration, thereby reducing device complexity while maintaining impurity removal capability.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The patent changes the chemical state of impurities from dissolved ions to solid precipitates by adjusting solution parameters (adding precipitating agents). This parameter change allows impurities to be removed through simple filtration rather than complex physical separation processes, reducing equipment requirements while maintaining separation effectiveness.

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If chemical precipitation methods are used to remove copper and aluminum impurities, then impurity removal capability is improved, but material costs and process complexity increase

Engineering Contradiction:
Improveimpurity removal capabilityVSAvoidprocess simplicity
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The patent extracts and removes only the necessary precipitating agents (sodium hydroxide and sodium carbonate) from the complex chemical process system. By selectively removing impurities through targeted precipitation reactions rather than using multiple chemical treatments, the process is simplified while maintaining effective impurity removal capability.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent discards the need for complex chemical processing steps by using a two-stage precipitation method that naturally separates impurities from the product. The first stage removes copper and aluminum as hydroxide precipitates, and the second stage removes lithium as carbonate precipitate, with the iron phosphate product being recovered in between, simplifying the overall manufacturing process.

Inventive Principle:
Principle #34Discarding and recovering

3Manufacturing precision

If multi-stage filtering and many operation steps are used to remove impurities, then impurity removal capability is improved, but operation complexity and time consumption increase

Engineering Contradiction:
Improveimpurity removal capabilityVSAvoidprocess time
Core Design Contradiction:
Manufacturing precisionVSLoss of time

Solution Approach 1:

The patent merges multiple impurity removal operations into a unified two-stage precipitation process. Instead of performing separate screening, flotation, wind separation, and eddy-current separation operations followed by multiple filtrations, the invention combines all impurity removal into two chemical precipitation steps followed by a single filtration operation, significantly reducing process time and operational complexity.

Inventive Principle:
Principle #5Merging (Combining)

4Manufacturing precision

If produced copper(II) sulfide, copper hydroxide, and aluminum hydroxide require further smelting, then impurity removal capability is improved, but process complexity and material consumption increase

Engineering Contradiction:
Improveimpurity removal capabilityVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent converts the harmful dissolved copper and aluminum ions into beneficial solid precipitates that can be easily filtered and discarded. By using chemical precipitation to transform impurities from a problematic dissolved state into easily removable solid form, the process eliminates the need for complex smelting operations while maintaining effective impurity removal.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method achieves a lithium iron phosphate precursor with low impurity content, reducing reclamation costs and environmental impact, and enables the production of lithium iron phosphate materials with high capacity and good cycle performance for use in lithium battery systems.

Implementation Method 1

soaking the battery cell in acid, and performing filtering

Methodology Applied
Scientific EffectChemical dissolution: Hydrolysis

Implementation Method 2

performing electrolysis to reclaim copper: adding a copper cathode and a carbon anode into filtered solution, and performing electrolysis

Methodology Applied
Scientific EffectElectrolysis: Electrolysis

Implementation Method 3

oxidizing ferrous iron: adding oxidant into the electrolyzed solution, and performing oxidation reaction

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 4

precipitating iron phosphate: gradually adjusting pH of the solution resulting from the oxidation reaction to greater than 14 to obtain an iron phosphate precipitate

Methodology Applied
Scientific EffectPrecipitation: Precipitation

Implementation Method 5

precipitating lithium carbonate: keeping adding carbonate solution into the post-reaction solution until a white precipitate no longer increases

Methodology Applied
Scientific EffectPrecipitation: Precipitation

Data Source

PatentUS12304826B2Method for producing lithium iron phosphate precursor by using retired lithium iron phosphate battery as raw material
Publication Date: 2025.05.20 CONTEMPORARY AMPEREX TECHNOLOGY (HONG KONG) LIMITED

AI summary

A method for producing a lithium iron phosphate precursor by using a retired lithium iron phosphate battery as a raw material is provided, which includes steps of: soaking a battery cell in acid, performing electrolysis to reclaim copper, oxidizing ferrous iron, precipitating iron phosphate, and precipitating lithium carbonate. After precipitation is completed, performing one-step reclaim to obtain the lithium iron phosphate precursor.