MTJ Diffusion Barrier for Coercivity Retention at 400°C

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Solution Overview

Problem

Current magnetic tunnel junction (MTJ) stacks face challenges in maintaining coercivity (Hc) and thermal stability at elevated temperatures, particularly during high-temperature semiconductor processes up to 400°C, due to diffusion of hard mask materials and reduced perpendicular magnetic anisotropy (PMA), which degrades the performance of magnetic memory devices.

Innovation Solution

Incorporating a diffusion barrier between the metal oxide cap layer and the hard mask in the MTJ stack to prevent non-magnetic metal diffusion and maintain PMA, using non-magnetic metals or alloys like Mo, Zr, Nb, or TaN to block metal migration, and employing a metal oxide layer to enhance perpendicular anisotropy, thereby maintaining coercivity and thermal stability during high-temperature processing.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Temperature

If high temperature annealing (400°C) is applied to improve semiconductor process compatibility, then thermal stability and oxidation resistance are improved, but coercivity and perpendicular magnetic anisotropy deteriorate due to metal diffusion

Engineering Contradiction:
Improveannealing temperatureVSAvoidcoercivity
Core Design Contradiction:
TemperatureVSReliability

Solution Approach 1:

A diffusion barrier layer comprising TaN, Mo, Zr, or Nb is introduced between the metal oxide cap layer and the hard mask layer. This intermediary layer prevents non-magnetic metal diffusion into the free layer during high temperature annealing, thereby maintaining coercivity and perpendicular magnetic anisotropy while allowing the system to withstand 400°C processing temperatures.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Stability of the object's composition

If metal oxide cap layer is used to enhance perpendicular anisotropy, then PMA is improved, but metal diffusion occurs at high temperature causing coercivity loss

Engineering Contradiction:
Improveperpendicular magnetic anisotropyVSAvoidmetal diffusion
Core Design Contradiction:
Stability of the object's compositionVSObject-generated harmful factors

Solution Approach 1:

The diffusion barrier layer is positioned between the metal oxide cap layer and the hard mask layer to block the diffusion path of non-magnetic metals. This allows the metal oxide cap layer to maintain its function of enhancing perpendicular magnetic anisotropy at the free layer interface while preventing harmful metal diffusion during high temperature processing.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent employs a composite structure consisting of multiple layers with distinct functions: the metal oxide cap layer provides perpendicular magnetic anisotropy enhancement, while the diffusion barrier layer (TaN, Mo, Zr, or Nb) provides diffusion protection. This composite approach allows simultaneous achievement of high PMA and coercivity retention after 400°C annealing.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The diffusion barrier effectively prevents metal diffusion, maintaining high coercivity and thermal stability of the free layer, ensuring optimal magnetic memory performance even after annealing at 400°C, thus enhancing the retention time and scalability of MTJ-based memory devices.

Implementation Method 1

Incorporating a diffusion barrier between the metal oxide cap layer and the hard mask in the MTJ stack to prevent non-magnetic metal diffusion

Methodology Applied
Scientific EffectDiffusion barrier: Diffusion Barrier

Implementation Method 2

The tunnel barrier is typically about 10 Angstroms (1 Angstrom = 0.1 nm) thick so that a current through the tunnel barrier can be established by a quantum mechanical tunneling of conduction electrons

Methodology Applied
Scientific EffectQuantum mechanical tunneling:

Implementation Method 3

Magnetoresistive Random Access Memory (MRAM) has a read function based on a tunneling magnetoresistive (TMR) effect in a MTJ stack

Methodology Applied
Scientific EffectTunneling magnetoresistive effect: Magnetoresistance

Implementation Method 4

MTJ elements wherein one or both of the free layer and reference layer have perpendicular magnetic anisotropy (PMA)

Methodology Applied
Scientific EffectPerpendicular magnetic anisotropy: Anisotropy

Data Source

PatentEP3347927B1Magnetic element with perpendicular magnetic anisotropy for high coercivity after high temperature annealing
Publication Date: 2019.11.06 TAIWAN SEMICONDUCTOR MANUFACTURING CO LTD
  • EP3347927B1 patent drawingFigure 1~4
  • EP3347927B1 patent drawingFigure 5~8
  • EP3347927B1 patent drawingFigure 9~11

AI summary

A magnetic tunnel junction (MTJ) is disclosed wherein a free layer has an interface with a tunnel barrier and a second interface with a metal oxide layer to promote perpendicular magnetic anisotropy (PMA) therein. A diffusion barrier is formed on a side of the metal oxide layer opposite the second interface to prevent non-magnetic metals in a hard mask or electrode from migrating to the second interface and degrading free layer PMA. A second diffusion barrier may be formed between a second electrode and a reference layer. The diffusion barrier may be a single layer of SiN, TiN, TaN, Mo, or CoFeX where X is Zr, P, B, or Ta, or is a multilayer such as CoFeX/Mo wherein CoFeX contacts the metal oxide layer and Mo adjoins a hard mask. As a result, coercivity is maintained or increased in the MTJ after annealing at 400°C for 30 minutes.