Organic Light-Emitting Device Hole Transport Layer Stability

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Solution Overview

Problem

Current organic light emitting devices face challenges in achieving high efficiency, long lifespan, and thermal stability due to limitations in materials used for hole transport and electron transport layers, particularly with NPB and PEDOT:PSS, which have low glass transition temperatures and inappropriate energy levels, leading to issues with charge mobility and stability.

Innovation Solution

Incorporating an alkali metal complex docked to heteroatoms, phosphine oxide, thioxophosphine, or selenoxophosphine groups in heteroaryl-based compounds within the organic material layers to enhance energy levels, stability, and charge mobility, thereby improving the device's lifespan and efficiency.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If NPB is used as hole transport layer material, then the device can be manufactured with conventional materials, but the glass transition temperature is low (100°C or lower) making it difficult to apply to high current devices

Engineering Contradiction:
ImprovemanufacturabilityVSAvoidglass transition temperature
Core Design Contradiction:
Ease of manufactureVSTemperature

Solution Approach 1:

The patent modifies the molecular structure of hole transport materials by introducing specific chemical groups and substituents to increase the glass transition temperature while maintaining charge transport properties. This allows the material to withstand higher temperatures generated by high current operation.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent develops composite organic materials combining multiple functional groups and substituents to achieve both high glass transition temperature and effective hole transport capability, resolving the contradiction between thermal stability and charge transport efficiency.

Inventive Principle:
Principle #40Composite materials

2Ease of manufacture

If PEDOT:PSS is used as hole transport material, then the device can be manufactured by solution coating method, but the LUMO energy level is lower than light emitting layer material making it difficult to achieve high efficiency and long lifespan

Engineering Contradiction:
Improvesolution coating manufacturabilityVSAvoiddevice efficiency and lifespan
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent adjusts the HOMO and LUMO energy levels of hole transport materials through molecular design and substituent selection to ensure proper energy level alignment with the light emitting layer, enabling efficient charge injection while maintaining solution processability.

Inventive Principle:
Principle #35Parameter changes

3Device complexity

If conventional organic materials are used, then the device structure is simple, but the thermal stability is insufficient due to low glass transition temperature

Engineering Contradiction:
Improvematerial structure complexityVSAvoidthermal stability
Core Design Contradiction:
Device complexityVSTemperature

Solution Approach 1:

The patent systematically modifies molecular parameters including glass transition temperature, charge mobility, and energy levels through controlled introduction of substituents and functional groups, achieving high thermal stability while maintaining device performance.

Inventive Principle:
Principle #35Parameter changes

4Productivity

If materials with appropriate energy levels are selected, then charge transport efficiency improves, but the thermal stability and electrochemical stability may be compromised

Engineering Contradiction:
Improvecharge transport efficiencyVSAvoidthermal and electrochemical stability
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent designs composite organic materials incorporating multiple functional groups that work synergistically to provide both efficient charge transport through appropriate energy levels and high thermal/electrochemical stability through robust molecular structures.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The proposed solution significantly increases the lifespan of organic light emitting devices by altering the dipole moment of the compounds in the material layers, enhancing thermal stability and charge transport, resulting in improved performance and longevity.

Implementation Method 1

one or more of the organic material layers comprises a compound where an alkali metal complex is docked to one or more of a heteroatom, O of a phosphine oxide group (-P=O), S of a thioxophosphine group (-P=S) or Se of a selenoxophosphine group (-P=Se) of one or more compounds of a heteroaryl-based compound by a London dispersion force or a dipole-induced dipole force

Methodology Applied
Scientific EffectLondon dispersion force: London Dispersion Force

Implementation Method 2

one or more of the organic material layers comprises a compound where an alkali metal complex is docked to one or more of a heteroatom, O of a phosphine oxide group (-P=O), S of a thioxophosphine group (-P=S) or Se of a selenoxophosphine group (-P=Se) of one or more compounds of a heteroaryl-based compound by a London dispersion force or a dipole-induced dipole force

Methodology Applied
Scientific EffectDipole-induced dipole force:

Implementation Method 3

An organic light emitting phenomenon is an example of a conversion of current into visible rays by an internal process of a specific organic molecule. When an organic material layer is interposed between an anode and a cathode, if voltage is applied between two electrodes, electrons and holes are injected from the cathode and the anode to the organic material layer. The electrons and the holes injected into the organic material layer are recombined to form an exciton, and the exciton is reduced to a bottom state to emit light.

Methodology Applied
Scientific EffectElectroluminescence: Electroluminescence

Data Source

PatentEP2750214B1Organic light-emitting device and method for manufacturing same
Publication Date: 2020.06.17 LG CHEM LTD
  • EP2750214B1 patent drawingFigure 1~2
  • EP2750214B1 patent drawingFigure 3~4
  • EP2750214B1 patent drawingFigure 5

AI summary

The present invention provides an organic light emitting device comprising a first electrode, a second electrode, and one or more organic material layers disposed between the first electrode and the second electrode, and having an excellent life-span property by changing a dipole moment of a compound comprised in the organic material layers.