Polymer Resist Composition for High-Resolution Lithography

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Solution Overview

Problem

Current positive resist compositions face challenges in achieving high sensitivity, resolution, and minimal edge roughness for microelectronic device manufacturing, particularly as feature sizes decrease, due to issues with acid diffusion and film thickness loss during exposure processes.

Innovation Solution

A polymer comprising recurring units of butyrolactone (meth)acrylate, carboxyl or phenolic groups with acid labile substitutions, and hydroxy-aromatic groups or 2,2,2-trifluoro-1-hydroxyethyl groups is developed, which improves dissolution contrast, suppresses acid diffusion, and maintains film thickness, forming a resist composition suitable for high-resolution patterning.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If the accelerating voltage of the electron gun is increased to enable further size reduction, then the resolution and dimensional control are improved, but the sensitivity of the resist film decreases

Engineering Contradiction:
ImproveresolutionVSAvoidsensitivity
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The patent changes the chemical composition parameters of the resist film by incorporating specific polymer structures (poly-4-hydroxystyrene with controlled molecular weight and composition) to optimize the balance between sensitivity and resolution at high accelerating voltages

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite resist formulations combining poly-4-hydroxystyrene base polymer with specific additives and modifiers to achieve both high sensitivity and high resolution performance simultaneously

Inventive Principle:
Principle #40Composite materials

2Manufacturing precision

If acid diffusion is suppressed to improve resolution for fine patterns, then the resolution is improved, but the sensitivity decreases

Engineering Contradiction:
ImproveresolutionVSAvoidsensitivity
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The patent introduces local quality control by incorporating specific functional groups at controlled positions within the polymer structure to create localized acid generation zones that limit diffusion while maintaining overall sensitivity

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent optimizes the molecular weight and composition parameters of the poly-4-hydroxystyrene to control acid diffusion distance while preserving sensitivity through careful parameter selection

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If the exposure dose is increased to reduce edge roughness, then the edge roughness is reduced, but the sensitivity decreases

Engineering Contradiction:
Improveedge roughnessVSAvoidsensitivity
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The patent changes the chemical structure parameters of the resist polymer to intrinsically reduce edge roughness through controlled molecular architecture, eliminating the need for high exposure doses

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The polymer-based resist composition achieves high resolution and minimal edge roughness, preventing pattern collapse and film thickness loss, making it suitable for advanced lithography processes such as ArF, KrF, EUV, and EB lithography for microfabrication of VLSI and photomasks.

Implementation Method 1

the exposure system for mask manufacturing made a transition from the laser beam exposure system to the EB exposure system

Methodology Applied
Scientific EffectElectron beam irradiation: Electron Beam

Implementation Method 2

image blurs due to acid diffusion become a problem

Methodology Applied
Scientific EffectAcid diffusion: Diffusion

Implementation Method 3

chemically amplified resist compositions are contemplated

Methodology Applied
Scientific EffectChemically amplified:

Data Source

PatentUS9250517B2Polymer, positive resist composition and patterning process
Publication Date: 2016.02.02 SHIN ETSU CHEMICAL CO LTD

AI summary

A polymer comprising recurring units of butyrolactone (meth)acrylate, recurring units having a carboxyl or phenolic group which is substituted with an acid labile group, and recurring units having a phenol group or an adhesive group in the form of 2,2,2-trifluoro-1-hydroxyethyl is quite effective as a base resin for resist. A positive resist composition comprising the polymer is improved in such properties as a contrast of alkali dissolution rate before and after exposure, acid diffusion suppressing effect, resolution, and profile and edge roughness of a pattern after exposure.