Polyolefin Adhesive Composition for Low-Temperature Pouch Lamination

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Solution Overview

Problem

Existing adhesive compositions for lithium-ion battery packaging materials face challenges with moldability, adhesion, heat resistance, and durability, particularly when exposed to high temperatures and mechanical stress, leading to potential electrolyte leakage and delamination.

Innovation Solution

A blend of two modified polyolefins with different melting points and a styrene-based or olefin-based thermoplastic resin, along with a curing agent, is used to create an adhesive composition that exhibits excellent adhesion to polyolefin and metal substrates, providing improved followability and resistance to electrolyte solutions, even at low temperatures.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If a conventional adhesive composition is used to bond packaging materials, then adhesion between layers is achieved, but the adhesive layer cannot follow substrate extension during pouch formation, causing peeling and poor moldability

Engineering Contradiction:
ImproveadhesionVSAvoidmoldability
Core Design Contradiction:
StrengthVSEase of manufacture

Solution Approach 1:

The adhesive composition uses a composite system combining modified polyolefin (A1) with low melting point for flexibility and followability, modified polyolefin (A2) with high melting point for thermal stability, and thermoplastic resin (B) for enhanced adhesion. This composite formulation allows the adhesive to follow substrate extension during pouch formation while maintaining strong bonding strength.

Inventive Principle:
Principle #40Composite materials

2Strength

If the adhesive is processed at high temperature to improve bonding, then adhesion strength increases, but the adhesive layer breaks due to pulling force and heat resistance deteriorates

Engineering Contradiction:
Improveadhesion strengthVSAvoidheat resistance
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The invention optimizes the melting point parameters of the adhesive components. Modified polyolefin (A1) has a low melting point (50-100°C) allowing processing at lower temperatures, while modified polyolefin (A2) has a high melting point (100-160°C) providing heat resistance. The melting point difference between (A1) and (A2) is controlled at 30-50°C to balance processability and thermal stability, enabling bonding without breaking under pulling force.

Inventive Principle:
Principle #35Parameter changes

3Ease of manufacture

If the adhesive composition is simplified to improve ease of manufacture, then production becomes easier, but adhesion to both polyolefin and metal substrates deteriorates

Engineering Contradiction:
Improveease of processingVSAvoidadhesion
Core Design Contradiction:
Ease of manufactureVSStrength

Solution Approach 1:

The adhesive composition is designed with multi-functionality to bond both polyolefin resin substrates and metal substrates effectively. Modified polyolefin components provide compatibility with polyolefin substrates, while the thermoplastic resin (B) and acid value control (2-50 mgKOH/g) enable adhesion to metal substrates. This universal bonding capability is achieved within a single composition formulation that maintains ease of manufacture.

Inventive Principle:
Principle #6Universality (Multi-functionality)

4Weight of moving object

If the adhesive layer is made thinner to reduce packaging material weight, then weight reduction is achieved, but electrolyte solution penetration increases causing delamination

Engineering Contradiction:
Improvepackaging material weightVSAvoidelectrolyte solution resistance
Core Design Contradiction:
Weight of moving objectVSReliability

Solution Approach 1:

The adhesive composition uses a composite system where modified polyolefin (A1) and (A2) provide baseline electrolyte resistance, while thermoplastic resin (B) enhances barrier properties. The acid-modified components (acid value 2-50 mgKOH/g) improve chemical resistance to electrolyte solutions. This composite formulation maintains excellent electrolyte solution resistance even in thin adhesive layers, preventing delamination while reducing packaging material weight.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The adhesive composition demonstrates enhanced moldability, adhesion, electrolyte solution resistance, and heat resistance, ensuring durability and reliability of lithium-ion battery packaging materials under various environmental conditions.

Implementation Method 1

an adhesive composition comprising a modified polyolefin (A1); a modified polyolefin (A2) containing propylene in an amount of 30 mol% or more and having a melting point higher than that of the modified polyolefin (A1); and a thermoplastic resin (B)

Methodology Applied
Scientific EffectVan der Waals forces: Van der Waals Force

Implementation Method 2

the adhesion of the adhesives after curing in a high-temperature environment may be poor, or breakage may occur due to pulling force

Methodology Applied
Scientific EffectCrosslinking: Chemical Bonding

Data Source

PatentEP3778819B1Polyolefin-based adhesive composition
Publication Date: 2024.02.21 TOYOBO CO LTD

AI summary

Provided is an adhesive composition that is capable of bonding and aging at low temperature, and that has excellent adhesion, electrolyte solution resistance, heat resistance, durability, and moldability. The adhesive composition comprises a modified polyolefin (A1), a modified polyolefin (A2) having a melting point higher than that of the modified polyolefin (A1), and a thermoplastic resin (B).