Polyolefin Pyrolysis with Segmented Heating Zones

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Solution Overview

Problem

Existing methods for processing recyclable plastics into hydrocarbons face issues with high slag formation, limited flexibility in product control, and moderate purity, failing to meet current environmental standards for sulfur and chlorine levels.

Innovation Solution

A process involving pyrolytic cracking of polyolefin plastics with a specific heating and cracking reactor system, using diesel oil to improve pumpability and separate hydrocarbon fractions, and a distillation column for precise separation of hydrocarbon chains, minimizing coke formation and optimizing product purity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Loss of substance

If plastic recyclables are processed using conventional pyrolysis methods, then hydrocarbons are produced, but large amounts of slag are formed and product purity is moderate

Engineering Contradiction:
Improveslag formationVSAvoidproduct purity
Core Design Contradiction:
Loss of substanceVSManufacturing precision

Solution Approach 1:

The heating process is divided into three distinct heating zones with progressively increasing temperatures (first zone: lower temperature, second zone: medium temperature, third zone: high temperature near cracking temperature). This segmentation allows different stages of plastic decomposition to occur in separate zones, preventing premature carbonization and reducing slag formation while improving hydrocarbon yield and purity.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

Each heating zone is designed with specific temperature characteristics tailored to its function: the first zone operates at lower temperature for initial melting and decomposition, the second zone at medium temperature for further breakdown, and the third zone at high temperature for near-complete cracking. This local quality optimization ensures that plastic is converted to hydrocarbons efficiently at each stage without excessive carbon residue formation.

Inventive Principle:
Principle #3Local quality

2Adaptability or versatility

If conventional cracking processes are used, then long-chain hydrocarbons are broken down, but flexibility in product control is limited

Engineering Contradiction:
Improveproduct control flexibilityVSAvoidhydrocarbon chain length control
Core Design Contradiction:
Adaptability or versatilityVSManufacturing precision

Solution Approach 1:

The system allows dynamic adjustment of residence times in each heating zone and cracking reactor, enabling operators to control the extent of cracking. By adjusting the time plastic melt spends in the high-temperature third heating zone and cracking reactor, different proportions of short-chain vs. long-chain hydrocarbons can be produced, providing flexibility to meet different market demands for fuel specifications.

Inventive Principle:
Principle #15Dynamics

Solution Approach 2:

The process enables independent control of temperature parameters in each heating zone and the cracking reactor. By varying temperature parameters (lower in first zone, medium in second zone, high in third zone) and adjusting the degree of cracking, the product distribution can be tailored to produce specific hydrocarbon chain lengths suitable for different fuel applications.

Inventive Principle:
Principle #35Parameter changes

3Object-affected harmful factors

If conventional processing methods are applied, then plastic recyclables are converted to oil, but sulfur and chlorine levels exceed environmental requirements

Engineering Contradiction:
Improveenvironmental complianceVSAvoidimpurity removal efficiency
Core Design Contradiction:
Object-affected harmful factorsVSManufacturing precision

Solution Approach 1:

The plastic recyclables undergo preliminary treatment in the first and second heating zones before entering the cracking reactor. In the first zone, moisture and volatile components are removed. In the second zone, further decomposition occurs and some impurities are eliminated. This preliminary action prepares the material for cracking while reducing the burden of impurity removal, resulting in cleaner hydrocarbon products that meet environmental standards.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The impurities present in plastic recyclables (such as sulfur and chlorine-containing compounds) are converted during the controlled thermal processing into volatile substances that are removed as gases during heating and cracking. The thermal energy that could potentially cause harmful decomposition is instead utilized to transform impurities into removable gaseous forms, leaving cleaner liquid hydrocarbon products.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

4Manufacturing precision

If multiple heating zones are implemented, then processing precision is improved, but device complexity increases

Engineering Contradiction:
Improvetemperature control precisionVSAvoidheating system complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The heating system is segmented into three distinct heating zones with independent temperature control, allowing precise temperature management in each zone. This segmentation enables the first zone to operate at lower temperature for melting, the second zone at medium temperature for decomposition, and the third zone at high temperature for cracking, achieving superior processing precision while maintaining manageable system complexity through modular design.

Inventive Principle:
Principle #1Segmentation

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Reduces slag formation, enhances product control and purity, and meets stringent environmental standards by effectively cracking long-chain hydrocarbons into shorter chains, producing high-quality hydrocarbon products.

Implementation Method 1

steam is removed in the first heating zone or the first heat exchanger at 105 to 125°C in a first gas phase

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 2

in a second heating zone or a second heat exchanger at one temperature from 180 to 250°C a separation into a second gas phase, which consists primarily of acid gases and via a degassing dome e is removed

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 3

the molten hydrocarbons are purely thermolytically cracked at about 400°C, i.e. cracked

Methodology Applied
Scientific EffectPyrolysis: Pyrolysis

Implementation Method 4

the molten hydrocarbons are purely thermolytically cracked at about 400°C

Methodology Applied
Scientific EffectThermolysis: Thermolysis

Implementation Method 5

the gaseous hydrocarbons being fed to a partial condenser in which long-chain hydrocarbons condense

Methodology Applied
Scientific EffectCondensation: Condensation

Implementation Method 6

the gases from the partial condenser are fed to a distillation column in which they are broken down into a gaseous and a liquid fraction

Methodology Applied
Scientific EffectDistillation: Distillation

Data Source

PatentEP2876146B1Method and assembly for the treatment of recycled plastics
Publication Date: 2018.09.05 WESER GEROLD
  • EP2876146B1 patent drawingFigure 1

AI summary

A process for recovering hydrocarbons from polyolefin plastics by means of pyrolytic cracking comprises: - feeding the plastics into a mixing vessel under inert gas and mixing with diesel fuel, - removing water vapor in a first heating zone, - removing acidic gases in a second heating zone, - liquefying the unmelted plastics in a third heating zone, - cracking the plastics in a cracking reactor at approximately 400°C, - partial condensation to prevent the release of paraffins, - fractionation of the crack products. A plant for carrying out this process is also described.