Polysilicon CMP Slurry Without TMAH for High Selectivity

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Solution Overview

Problem

Commercially available polysilicon CMP slurries rely on tetramethylammonium hydroxide (TMAH), a hazardous and toxic chemical, for high removal rates, necessitating a TMAH-free alternative that maintains high polysilicon removal rates and selectivity to silicon oxide and silicon nitride layers while reducing environmental and health hazards.

Innovation Solution

A water-based chemical mechanical polishing composition containing silica abrasive particles, a nitrogen-containing polysilicon accelerator (such as amino acids or guanidine derivatives), and an alkali metal salt, with a pH range of 10 to 11, and minimal tetraalkylammonium salts, which provides high removal rates and selectivity without TMAH.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If TMAH is used as chemical accelerator, then polysilicon removal rate is improved, but environmental and health hazards increase

Engineering Contradiction:
Improvepolysilicon removal rateVSAvoidenvironmental and health hazards
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the chemical composition parameters by replacing TMAH with alternative accelerators (amino acids, guanidine derivatives) and adjusts pH to 10-11 using alkali metal salts, achieving high removal rates without hazardous materials

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses biodegradable, non-hazardous materials (amino acids, guanidine derivatives) that are environmentally friendly and can be safely disposed of, replacing persistent toxic chemicals

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

2Object-affected harmful factors

If TMAH-free composition is used, then environmental safety is improved, but polysilicon removal rate may decrease

Engineering Contradiction:
Improveenvironmental safetyVSAvoidpolysilicon removal rate
Core Design Contradiction:
Object-affected harmful factorsVSProductivity

Solution Approach 1:

The patent optimizes pH to 10-11 using alkali metal salts and selects specific accelerators (amino acids, guanidine derivatives) to achieve high polysilicon removal rates without TMAH

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces nitrogen-containing compounds (amino acids, guanidine derivatives) as intermediary substances that facilitate polysilicon removal through chemical interaction, replacing TMAH's function without its toxicity

Inventive Principle:
Principle #24Intermediary (Mediator)

3Quantity of substance

If alternative accelerator is used, then TMAH content is reduced, but selectivity to silicon oxide and silicon nitride may be affected

Engineering Contradiction:
Improvetetraalkylammonium salt contentVSAvoidselectivity to silicon oxide and silicon nitride
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

The patent carefully controls pH (10-11) and accelerator concentration to achieve high selectivity to silicon oxide and silicon nitride while maintaining low tetraalkylammonium salt content (<500 ppm)

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition achieves high polysilicon removal rates and selectivity to silicon oxide and silicon nitride, while being environmentally friendly and reducing human health hazards, as it is substantially free of tetraalkylammonium compounds.

Implementation Method 1

about 0.1 to about 3 weight percent silica abrasive particles dispersed in the liquid carrier

Methodology Applied
Scientific EffectAbrasion: Abrasion

Implementation Method 2

about 0.05 to about 1 weight percent of a polysilicon accelerator, the polysilicon accelerator selected from the group consisting of an amino acid, a guanidine derivative, and mixtures thereof

Methodology Applied
Scientific EffectChemical reaction: Chemical Bonding

Implementation Method 3

an alkali metal salt. The composition comprises less than about 500 ppm by weight tetraalkylammonium salts and has a pH in a range from about 10 to about 11

Methodology Applied
Scientific EffectBase-induced etching: Oxidation

Data Source

PatentUS12157834B2Composition and method for polysilicon CMP
Publication Date: 2024.12.03 CMC MATERIALS INC

AI summary

A chemical mechanical polishing composition for polishing a substrate having a polysilicon layer includes a water based liquid carrier, a silica abrasive, an amino acid or guanidine derivative containing polysilicon polishing accelerator, and an alkali metal salt. The composition includes less than about 500 ppm tetraalkylammonium salt and has a pH in a range from about 10 to about 11.