Quinone Flow Battery Protonation for Grid Energy Storage

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Solution Overview

Problem

Current flow batteries, such as vanadium redox flow batteries, face challenges in scalability, high costs per kWh, and limitations in dispatchability of intermittent renewable power sources due to high costs and limited cycle life, while solid electrode batteries have inadequate peak-power discharge times.

Innovation Solution

A quinone-based flow battery that stores electrical energy through the protonation of quinones to hydroquinones, allowing for a closed system with high current density, long lifetime, and reduced costs through the use of inexpensive chemicals and materials, eliminating the need for precious metals and operating at room temperature.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If vanadium redox flow batteries are used for grid-scale energy storage, then reliability and cycle life are improved, but cost per kWh increases significantly

Engineering Contradiction:
Improvecycle lifeVSAvoidcost per kWh
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent replaces expensive vanadium electrolyte with inexpensive organic quinone-based electrolytes that can be synthesized at low cost. The organic molecules serve as disposable, renewable reactants that eliminate the need for costly precious metals while maintaining acceptable cycle life through stable molecular structures.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent changes the chemical parameters by transitioning from inorganic vanadium salts to organic quinone compounds, altering the redox chemistry from V2+/V3+ and V3+/V4+ couples to quinone/hydroquinone couples. This parameter change dramatically reduces material costs while preserving the flow battery's long-duration energy storage capability.

Inventive Principle:
Principle #35Parameter changes

2Power

If solid electrode batteries are used for energy storage, then power density is improved, but duration of action (peak-power discharge time) is insufficient

Engineering Contradiction:
Improvepower densityVSAvoidpeak-power discharge time
Core Design Contradiction:
PowerVSDuration of action of moving object

Solution Approach 1:

The patent segments the battery system into separate power and energy components: the electrochemical cell stack provides high power density, while external tanks store large volumes of quinone electrolyte for extended duration. This segmentation allows independent optimization of power and energy, enabling both high power density and long discharge times.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent transitions from the conventional solid-electrode paradigm to a flow battery architecture where energy is stored in liquid electrolyte circulating through external tanks. This dimensional change separates the power-generating electrochemical reaction from the energy-storing chemical reactants, enabling scalable long-duration discharge.

Inventive Principle:
Principle #17Another dimension (Dimensionality change)

3Ease of manufacture

If flow battery architecture is used for energy storage, then scalability and cost per kWh are improved, but manufacturing complexity increases

Engineering Contradiction:
Improvecost per kWhVSAvoidsystem complexity
Core Design Contradiction:
Ease of manufactureVSDevice complexity

Solution Approach 1:

The patent employs hydraulic flow systems to circulate quinone electrolyte between external storage tanks and the electrochemical cell stack. This hydraulic architecture enables simple, scalable energy storage by decoupling the power-generating component from the energy-storing tanks, reducing manufacturing complexity compared to integrated designs.

Inventive Principle:
Principle #29Pneumatics and hydraulics

4Power

If zinc-bromine hybrid flow battery is used, then power density is improved, but reliability decreases due to dendrite formation

Engineering Contradiction:
Improvepower densityVSAvoidcycle life
Core Design Contradiction:
PowerVSReliability

Solution Approach 1:

The patent eliminates zinc metal plating and uses stable organic quinone molecules as the energy-storing medium. This replacement of reactive metals with chemically stable organic compounds eliminates dendrite formation while maintaining high power density through efficient electron transfer reactions.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The quinone-based flow battery achieves high efficiency, scalability, and cost-effectiveness, enabling the dispatchability of intermittent renewable energy sources with improved power and energy storage capabilities, reducing the overall cost per kWh and extending cycle life.

Implementation Method 1

Electrical energy is stored chemically at an electrochemical electrode by the protonation of small organic molecules called quinones to hydroquinones

Methodology Applied
Scientific EffectProtonation:

Implementation Method 2

These reactions are reversed to deliver electrical energy

Methodology Applied
Scientific EffectRedox reactions: Redox Reactions

Data Source

PatentEP3050151B1Quinone and hydroquinone based flow battery
Publication Date: 2021.12.15 PRESIDENT & FELLOWS OF HARVARD COLLEGE
  • EP3050151B1 patent drawingFigure 1
  • EP3050151B1 patent drawingFigure 2~3
  • EP3050151B1 patent drawingFigure 4a~4b

AI summary

The invention provides an electrochemical cell based on a new chemistry for a flow battery for large scale, e.g., gridscale, electrical energy storage. Electrical energy is stored chemically in quinone molecules having multiple oxidation states, e.g., three or more. During charging of the battery, the quinone molecules at one electrode are oxidized by emitting electrons and protons, and the quinone molecules at the other electrode are reduced by accepting electrons and protons. These reactions are reversed to deliver electrical energy. The invention also provides additional high and low potential quinones that are useful in rechargeable batteries.