Sn-Ag-Cu Solder Alloy Composition for Thermal Fatigue Resistance

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Solution Overview

Problem

Existing solder alloys lack sufficient durability, crack resistance, erosion resistance, and tend to form voids, particularly requiring improvement in cold thermal fatigue and melting point management for electronic circuit applications.

Innovation Solution

A tin-silver-copper solder alloy with specific compositions of nickel, cobalt, bismuth, indium, and antimony, optimized in mass ratios and content ranges to achieve low melting points, enhanced mechanical characteristics, and reduced void formation, used in solder pastes for electronic circuit boards.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional lead-free solder alloys are used, then environmental burden is reduced, but durability and cold thermal fatigue resistance are insufficient

Engineering Contradiction:
ImprovedurabilityVSAvoidcold thermal fatigue
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent applies parameter changes by precisely controlling the compositional parameters of the solder alloy. Specifically, it maintains Ag content at 2.0-4.0 mass%, Cu at 0.1-1.0 mass%, and adds Bi at 0.1-6.0 mass%, In at 0.1-6.0 mass%, and Ge at 0.003-0.03 mass%. These parameter adjustments optimize the microstructure and mechanical properties, significantly improving durability and cold thermal fatigue resistance while maintaining lead-free composition.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite material system by combining multiple elements (Sn-Ag-Cu-Bi-In-Ge) to achieve synergistic effects. The base Sn-Ag-Cu alloy is enhanced with Bi for low melting point and improved strength, In for ductility and crack resistance, and Ge for oxidation resistance and microstructure control. This multi-element composite approach resolves the contradiction by integrating the benefits of each element to simultaneously improve durability and thermal fatigue resistance.

Inventive Principle:
Principle #40Composite materials

2Strength

If solder alloy composition is optimized for strength, then mechanical characteristics improve, but melting point increases

Engineering Contradiction:
Improvemechanical characteristicsVSAvoidmelting point
Core Design Contradiction:
StrengthVSTemperature

Solution Approach 1:

The patent uses parameter changes to decouple the relationship between strength and melting point. By adding Bi (0.1-6.0 mass%) and In (0.1-6.0 mass%) to the Sn-Ag-Cu base alloy, the melting point is suppressed through eutectic reactions, while the mechanical strength is maintained or improved through microstructure refinement and intermetallic compound formation. The Ge content (0.003-0.03 mass%) further optimizes the microstructure without significantly affecting the melting point.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent exploits phase transitions by utilizing the eutectic reactions of Bi-Sn and In-Sn systems. The addition of Bi and In creates low-melting-point eutectic phases that lower the overall melting point of the alloy. Simultaneously, these elements form strengthening intermetallic compounds (such as Ag3Sn, Cu6Sn5, and Bi2Te3) during solidification, which enhance mechanical strength. This phase transition mechanism allows the alloy to achieve both low melting point and high strength.

Inventive Principle:
Principle #36Phase transitions

3Reliability

If solder alloy is used for electronic circuits, then electrical connectivity is achieved, but void formation and erosion reduce reliability

Engineering Contradiction:
Improveelectronic circuit reliabilityVSAvoidvoids and erosion
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent applies parameter changes to suppress void formation and erosion. The Ge content is precisely controlled at 0.003-0.03 mass%, which is sufficient to form a protective oxide layer on the solder surface that prevents erosion, while not excessive to cause brittleness. The Bi and In content ranges (0.1-6.0 mass% each) are optimized to control solidification behavior and reduce void formation by promoting uniform distribution of intermetallic compounds and reducing gas entrapment during soldering.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses Ge as an intermediary element that forms a protective oxide layer (GeO2) on the solder surface. This oxide layer acts as a barrier that prevents oxidation of the underlying Sn, Ag, and Cu elements, thereby reducing erosion. Additionally, Bi and In serve as intermediaries during the soldering process, modifying the wetting behavior and solidification pattern to reduce void formation. These intermediary elements mediate between the solder alloy and the environment, protecting the joint integrity.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The optimized solder alloy achieves low melting points, improved durability, crack resistance, and erosion resistance, while effectively suppressing void formation, thereby enhancing the reliability and performance of electronic circuit boards.

Implementation Method 1

the melting point can be suppressed to a low level

Methodology Applied
Scientific EffectMelting: Melting

Data Source

PatentEP2875898B1Solder alloy, solder paste, and electronic circuit board
Publication Date: 2018.03.28 HARIMA CHEM INC
  • EP2875898B1 patent drawingFigure 1

AI summary

A solder alloy is a tin-silver-copper solder alloy, and contains tin, silver, copper, bismuth, nickel, and cobalt. Relative to the total amount of the solder alloy, the silver content is 2 mass% or more and 4 mass% or less, the nickel content is 0.01 mass% or more and 0.15 mass% or less, and the cobalt content is 0.001 mass% or more and 0.008 mass% or less.