SSZ-82 Borosilicate Zeolite Synthesis Using Organic Structure-Directing Agent

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Solution Overview

Problem

There is a continuous need for new crystalline molecular sieves with desirable properties for gas separation and hydrocarbon conversions, as existing sieves may lack enhanced selectivities and novel internal pore architectures.

Innovation Solution

The development of crystalline molecular sieve SSZ-82, prepared using 1,6-bis(N-cyclohexylpyrrolidinium)hexane dication as a structure directing agent, involves a method that includes hydrothermal crystallization and post-synthesis treatments like heteroatom lattice substitution to achieve the target zeolite composition and structure.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Adaptability or versatility

If existing molecular sieves are used, then current catalytic and separation functions are provided, but enhanced selectivities and novel internal pore architectures are not achieved

Engineering Contradiction:
Improveselectivity and pore architecture noveltyVSAvoidperformance consistency
Core Design Contradiction:
Adaptability or versatilityVSReliability

Solution Approach 1:

The patent changes the chemical composition parameters by incorporating boron into the molecular sieve framework (creating borosilicate zeolite SSZ-82), which fundamentally alters the pore architecture and selectivity properties while maintaining structural stability and catalytic performance

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention creates a composite material system by combining boron and silicon in a specific ratio within the zeolite framework, achieving novel pore structures that provide enhanced selectivity while maintaining reliable catalytic and separation functions

Inventive Principle:
Principle #40Composite materials

2Adaptability or versatility

If new molecular sieve structures are developed, then enhanced selectivities and novel pore architectures are achieved, but synthesis complexity and processing steps increase

Engineering Contradiction:
Improveselectivity and pore architecture noveltyVSAvoidsynthesis process complexity
Core Design Contradiction:
Adaptability or versatilityVSDevice complexity

Solution Approach 1:

The patent employs preliminary action by using a pre-designed organic structure-directing agent (1,6-bis(N-cyclohexylpyrrolidinium)hexane dication) that guides the formation of the desired borosilicate SSZ-82 pore structure during crystallization, simplifying the synthesis of this complex novel material

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The organic dication acts as an intermediary structure-directing agent that mediates the formation of the complex borosilicate framework, enabling the creation of novel pore architectures through hydrothermal crystallization without requiring overly complex synthesis procedures

Inventive Principle:
Principle #24Intermediary (Mediator)

3Manufacturing precision

If post-synthesis treatments are applied to achieve target zeolite, then desired composition and structure are obtained, but additional processing time and steps are required

Engineering Contradiction:
Improvezeolite composition precisionVSAvoidsynthesis throughput
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The patent achieves precise boron content control (0.015-0.050 mol Q per mol YO2) through carefully controlled hydrothermal crystallization conditions, reducing the need for extensive post-synthesis treatment while maintaining manufacturing precision

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

SSZ-82 exhibits unique properties and improved selectivities in hydrocarbon conversion and gas separation processes, demonstrated by its characterization through X-ray diffraction patterns and suitability in catalysts for hydrocarbon reactions and gas separations.

Implementation Method 1

a method for preparing SSZ-82 using a 1,6-bis(N-cyclohexylpyrrolidinium)hexane dication as a structure directing agent

Methodology Applied
Scientific EffectHydrothermal crystallization: Crystallisation

Implementation Method 2

post-synthesis treatments like heteroatom lattice substitution to achieve the target zeolite composition and structure

Methodology Applied
Scientific EffectHeteroatom lattice substitution:

Implementation Method 3

characterization through X-ray diffraction patterns

Methodology Applied
Scientific EffectX-ray diffraction: X-Ray

Data Source

PatentEP2370360B1Molecular sieve SSZ-82 composition of matter and synthesis thereof
Publication Date: 2019.11.20 CHEVRON USA INC
  • EP2370360B1 patent drawingFigure 1
  • EP2370360B1 patent drawingFigure 2
  • EP2370360B1 patent drawingFigure 3

AI summary

The present invention is directed to a new crystalline molecular sieve designated SSZ-82, a method for preparing SSZ-82 using a 1,6-bis(N-cyclohexylpyrrolidinium)hexane dication as a structure directing agent, and uses for SSZ-82.