Sub-atmospheric Extractive Distillation for Ethylbenzene Separation

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Current methods for separating ethylbenzene from close-boiling C8 aromatic compounds, such as xylene isomers, are either energy-intensive or require complex operations, and existing extractive distillation processes face challenges in achieving high separation efficiency and purity.

Innovation Solution

An extractive distillation process operating at sub-atmospheric pressure (50-500 mbar) and temperature (70-180°C) in a distillation column with a mass ratio of extractive solvent to ethylbenzene mixture of 3:1 to 70:1, using a solvent like 1,2,4-trichlorobenzene, which alters the relative volatility and enhances separation efficiency.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional fractionation methods are used to separate ethylbenzene from C8 aromatic compounds, then separation can be achieved, but the process becomes energy intensive and requires intricate systems

Engineering Contradiction:
Improveseparation efficiencyVSAvoidenergy consumption
Core Design Contradiction:
Manufacturing precisionVSUse of energy by moving object

Solution Approach 1:

The patent introduces an extractive solvent as an intermediary substance that selectively interacts with C8 aromatic compounds in the mixture. This solvent alters the relative volatility between ethylbenzene and C8 aromatics, enabling separation at lower energy costs by modifying the thermal properties of the mixture rather than relying on direct high-energy fractionation

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent changes the operating parameters by conducting distillation at sub-atmospheric pressures (50-500 mbar) and controlled temperatures (70-180°C). These parameter modifications optimize the separation process, reducing energy consumption while maintaining high separation efficiency through enhanced volatility differences under reduced pressure conditions

Inventive Principle:
Principle #35Parameter changes

2Device complexity

If a single polyfunctional distillation column is used to separate C8 aromatic isomers, then device complexity is reduced, but the system requires high reflux ratios (100-250:1) achieving commercially acceptable purity

Engineering Contradiction:
Improvecolumn structureVSAvoidreflux ratio
Core Design Contradiction:
Device complexityVSUse of energy by moving object

Solution Approach 1:

The extractive solvent acts as a mediator that enhances the separation capability of the distillation column, allowing for reduced reflux ratios while maintaining high purity. The solvent selectively interacts with C8 aromatic compounds, creating sharper separation fronts that reduce the energy-intensive reflux operation

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

By operating at sub-atmospheric pressures and optimized temperatures, the patent changes the thermodynamic parameters of the system. This enables more efficient mass transfer and sharper component separation, reducing the required reflux ratio from conventional 100-250:1 to lower values while maintaining commercial purity standards

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If adsorptive separation using crystalline aluminosilicate adsorbent is used, then ethylbenzene can be separated from xylene isomers, but the process requires complex countercurrent moving-bed systems and careful control of impurity content

Engineering Contradiction:
Improveseparation purityVSAvoidprocess operation
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent uses an extractive solvent as an intermediary that provides selective interaction with C8 aromatic compounds through altered relative volatility. This approach achieves high separation purity without requiring complex moving-bed adsorption systems, simplifying the overall process operation while maintaining effective separation

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent replaces the mechanical complexity of countercurrent moving-bed adsorption systems with a simpler extractive distillation process. By using thermal separation enhanced by the extractive solvent, the system achieves comparable or superior separation purity with significantly reduced operational complexity and fewer control requirements

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process significantly improves the separation efficiency of ethylbenzene from C8 aromatic compounds, reducing energy requirements and increasing the concentration of ethylbenzene in the overhead stream, while allowing for efficient recycling of the solvent and reducing the reflux ratio.

Implementation Method 1

Extractive distillation is the method of separating close boiling compounds from each other by carrying out the distillation in the presence of an added solvent or so called an extractive agent. The presence of the said extractive agent in the distillation system alters the relative volatility and therefore makes possible a greater degree of separation of the close boiling compounds.

Methodology Applied
Scientific EffectExtractive distillation: Distillation

Implementation Method 2

The process comprises distilling a mixture comprising ethylbenzene and a C8 aromatic compound in a distillation column in the presence of an extractive solvent

Methodology Applied
Scientific EffectDistillation: Distillation

Implementation Method 3

the distillation column is operated and operating at a sub-atmospheric pressure in a range between 50 to 500 mbar

Methodology Applied
Scientific EffectVapor pressure: Vapour Pressure

Data Source

PatentEP3189022B1Separation process for c8 aromatics mixture
Publication Date: 2021.01.06 SCG CHEM CO LTD

AI summary

Process for the distillative separation of ethylbenzene from a mixture comprising ethylbenzene and at least one other C8 aromatic compound, comprising distilling said mixture in a distillation column in the presence of an extractive solvent, characterized in that the distillation column is operated at a sub-atmospheric pressure.