Thioesterase Enzymes for Natural Thioester Production

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Solution Overview

Problem

Current methods for producing thioesters, such as methyl butanethioate, methyl thioacetate, and methyl thiopropionate, are not predictable and economically viable, making it difficult to label these compounds as 'natural' for use in food products.

Innovation Solution

Identification of nucleotide sequences encoding thioesterase enzymes, which can be used to produce thioesters efficiently and label them as 'natural' by encoding enzymes with specific amino acid sequences, enabling their use in consumable products and screening for wild-type bacteria capable of forming thioesters.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If thioesters are produced synthetically, then production efficiency is improved, but the ability to label as 'natural' deteriorates

Engineering Contradiction:
Improveproduction efficiencyVSAvoidnatural labeling capability
Core Design Contradiction:
ProductivityVSEase of manufacture

Solution Approach 1:

The patent replaces chemical synthesis methods with biological enzymatic methods. Specifically, thioesterases (enzymes) are used to catalyze the formation of thioesters from thiol and carboxylic acid substrates, substituting the mechanical/chemical synthesis process with a biological system that produces 'natural' labeled compounds while maintaining efficient production

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

2Ease of manufacture

If thioesters are produced via existing bacterial fermentation, then natural labeling is improved, but production predictability and economic viability deteriorate

Engineering Contradiction:
Improvenatural labeling capabilityVSAvoidproduction predictability
Core Design Contradiction:
Ease of manufactureVSProductivity

Solution Approach 1:

The patent changes key parameters of the fermentation process by introducing specifically identified thioesterase enzymes with known amino acid sequences and nucleotide sequences. This allows control over enzyme activity, substrate specificity, and reaction conditions, making the production process predictable while maintaining natural labeling capability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent identifies and copies specific nucleotide sequences (SEQ ID NOS: 1, 3, 5, and 7) that encode thioesterase enzymes. By replicating these genetic sequences in bacterial systems, the invention creates predictable, reproducible production of thioesters with consistent yields and product ratios

Inventive Principle:
Principle #26Copying

3Ease of manufacture

If existing bacterial fermentation methods are used, then natural production is improved, but yield control and product ratio predictability deteriorate

Engineering Contradiction:
Improvenatural production capabilityVSAvoidyield and product ratio control
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The patent employs feedback control by identifying specific thioesterase enzyme sequences and using them to monitor and control the fermentation process. The known enzyme sequences allow for measurement of enzyme activity and adjustment of fermentation conditions to achieve desired yield and product ratio outcomes

Inventive Principle:
Principle #23Feedback

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The use of nucleotide sequences encoding thioesterase enzymes allows for the efficient production of thioesters, enhancing the predictability and economic viability of their production, enabling their use in food products while maintaining a 'natural' label.

Implementation Method 1

nucleotide sequences encoding thioesterase enzymes, methods of their production, and their use in methods of forming thioesters

Methodology Applied
Scientific EffectEnzyme catalysis: Enzyme

Data Source

PatentUS10619139B2Thioesterases and their use
Publication Date: 2020.04.14 GIVAUDAN SA

AI summary

Disclosed are nucleotide sequences encoding thioesterase enzymes, methods for their production, their use in methods to form thioesters, and their use in methods of screening for other wild type bacteria capable of producing said thioesterase enzymes. Also disclosed are compositions comprising thioesters produced by the methods disclosed herein.